Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy

Laser frequency combs, with their unique combination of precisely defined spectral lines and broad bandwidth, are a powerful tool for basic and applied spectroscopy. Here, we report offset-free, mid-infrared frequency combs and dual-comb spectroscopy through supercontinuum generation in silicon-on-s...

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Main Authors: Nima Nader, Daniel L. Maser, Flavio C. Cruz, Abijith Kowligy, Henry Timmers, Jeff Chiles, Connor Fredrick, Daron A. Westly, Sae Woo Nam, Richard P. Mirin, Jeffrey M. Shainline, Scott Diddams
Format: Article
Language:English
Published: AIP Publishing LLC 2018-03-01
Series:APL Photonics
Online Access:http://dx.doi.org/10.1063/1.5006914
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author Nima Nader
Daniel L. Maser
Flavio C. Cruz
Abijith Kowligy
Henry Timmers
Jeff Chiles
Connor Fredrick
Daron A. Westly
Sae Woo Nam
Richard P. Mirin
Jeffrey M. Shainline
Scott Diddams
author_facet Nima Nader
Daniel L. Maser
Flavio C. Cruz
Abijith Kowligy
Henry Timmers
Jeff Chiles
Connor Fredrick
Daron A. Westly
Sae Woo Nam
Richard P. Mirin
Jeffrey M. Shainline
Scott Diddams
author_sort Nima Nader
collection DOAJ
description Laser frequency combs, with their unique combination of precisely defined spectral lines and broad bandwidth, are a powerful tool for basic and applied spectroscopy. Here, we report offset-free, mid-infrared frequency combs and dual-comb spectroscopy through supercontinuum generation in silicon-on-sapphire waveguides. We leverage robust fabrication and geometrical dispersion engineering of nanophotonic waveguides for multi-band, coherent frequency combs spanning 70 THz in the mid-infrared (2.5 μm–6.2 μm). Precise waveguide fabrication provides significant spectral broadening with engineered spectra targeted at specific mid-infrared bands. We characterize the relative-intensity-noise of different bands and show that the measured levels do not pose any limitation for spectroscopy applications. Additionally, we use the fabricated photonic devices to demonstrate dual-comb spectroscopy of a carbonyl sulfide gas sample at 5 μm. This work forms the technological basis for applications such as point sensors for fundamental spectroscopy, atmospheric chemistry, trace and hazardous gas detection, and biological microscopy.
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spelling doaj.art-c81a8be7ea9d4e7e8253ffc9df623fc52022-12-22T00:41:37ZengAIP Publishing LLCAPL Photonics2378-09672018-03-0133036102036102-1010.1063/1.5006914001803APPVersatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopyNima Nader0Daniel L. Maser1Flavio C. Cruz2Abijith Kowligy3Henry Timmers4Jeff Chiles5Connor Fredrick6Daron A. Westly7Sae Woo Nam8Richard P. Mirin9Jeffrey M. Shainline10Scott Diddams11Applied Physics Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USAApplied Physics Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USACenter for Nanoscale Science and Technology, National Institute of Standards and Technology, 100 Bureau Drive, Gaithersburg, Maryland 20899, USAApplied Physics Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USAApplied Physics Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USAApplied Physics Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USATime and Frequency Division, National Institute of Standards and Technology, 325 Broadway, Boulder, Colorado 80305, USALaser frequency combs, with their unique combination of precisely defined spectral lines and broad bandwidth, are a powerful tool for basic and applied spectroscopy. Here, we report offset-free, mid-infrared frequency combs and dual-comb spectroscopy through supercontinuum generation in silicon-on-sapphire waveguides. We leverage robust fabrication and geometrical dispersion engineering of nanophotonic waveguides for multi-band, coherent frequency combs spanning 70 THz in the mid-infrared (2.5 μm–6.2 μm). Precise waveguide fabrication provides significant spectral broadening with engineered spectra targeted at specific mid-infrared bands. We characterize the relative-intensity-noise of different bands and show that the measured levels do not pose any limitation for spectroscopy applications. Additionally, we use the fabricated photonic devices to demonstrate dual-comb spectroscopy of a carbonyl sulfide gas sample at 5 μm. This work forms the technological basis for applications such as point sensors for fundamental spectroscopy, atmospheric chemistry, trace and hazardous gas detection, and biological microscopy.http://dx.doi.org/10.1063/1.5006914
spellingShingle Nima Nader
Daniel L. Maser
Flavio C. Cruz
Abijith Kowligy
Henry Timmers
Jeff Chiles
Connor Fredrick
Daron A. Westly
Sae Woo Nam
Richard P. Mirin
Jeffrey M. Shainline
Scott Diddams
Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
APL Photonics
title Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
title_full Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
title_fullStr Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
title_full_unstemmed Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
title_short Versatile silicon-waveguide supercontinuum for coherent mid-infrared spectroscopy
title_sort versatile silicon waveguide supercontinuum for coherent mid infrared spectroscopy
url http://dx.doi.org/10.1063/1.5006914
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