Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering

Growth at liquid-liquid interfaces differ inherently from that on solids, making it attractive for nanomaterial formation. Here, the authors use X-ray scattering to derive a detailed microscopic picture of lead-halide growth on liquid mercury that reveals the key importance of anion adsorption.

Bibliographic Details
Main Authors: Andrea Sartori, Rajendra P. Giri, Hiromasa Fujii, Svenja C. Hövelmann, Jonas E. Warias, Philipp Jordt, Chen Shen, Bridget M. Murphy, Olaf M. Magnussen
Format: Article
Language:English
Published: Nature Portfolio 2022-09-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-32932-7
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author Andrea Sartori
Rajendra P. Giri
Hiromasa Fujii
Svenja C. Hövelmann
Jonas E. Warias
Philipp Jordt
Chen Shen
Bridget M. Murphy
Olaf M. Magnussen
author_facet Andrea Sartori
Rajendra P. Giri
Hiromasa Fujii
Svenja C. Hövelmann
Jonas E. Warias
Philipp Jordt
Chen Shen
Bridget M. Murphy
Olaf M. Magnussen
author_sort Andrea Sartori
collection DOAJ
description Growth at liquid-liquid interfaces differ inherently from that on solids, making it attractive for nanomaterial formation. Here, the authors use X-ray scattering to derive a detailed microscopic picture of lead-halide growth on liquid mercury that reveals the key importance of anion adsorption.
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spelling doaj.art-c82c62d59ba54701baab8fff831a508a2022-12-22T04:03:01ZengNature PortfolioNature Communications2041-17232022-09-0113111110.1038/s41467-022-32932-7Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scatteringAndrea Sartori0Rajendra P. Giri1Hiromasa Fujii2Svenja C. Hövelmann3Jonas E. Warias4Philipp Jordt5Chen Shen6Bridget M. Murphy7Olaf M. Magnussen8Institute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityDeutsches Elektronen-Synchrotron DESYInstitute for Experimental and Applied Physics, Kiel UniversityInstitute for Experimental and Applied Physics, Kiel UniversityGrowth at liquid-liquid interfaces differ inherently from that on solids, making it attractive for nanomaterial formation. Here, the authors use X-ray scattering to derive a detailed microscopic picture of lead-halide growth on liquid mercury that reveals the key importance of anion adsorption.https://doi.org/10.1038/s41467-022-32932-7
spellingShingle Andrea Sartori
Rajendra P. Giri
Hiromasa Fujii
Svenja C. Hövelmann
Jonas E. Warias
Philipp Jordt
Chen Shen
Bridget M. Murphy
Olaf M. Magnussen
Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
Nature Communications
title Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
title_full Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
title_fullStr Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
title_full_unstemmed Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
title_short Role of chemisorbing species in growth at liquid metal-electrolyte interfaces revealed by in situ X-ray scattering
title_sort role of chemisorbing species in growth at liquid metal electrolyte interfaces revealed by in situ x ray scattering
url https://doi.org/10.1038/s41467-022-32932-7
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