Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation
Quantitatively describing the atomic configuration of the catalytically active sites is challenging. Here the authors demonstrate that tuning crystal-phase of metal single-particle enables to precisely describe the atomic structure of the active sites and accurately identify the activation routes of...
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2022-08-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-32274-4 |
| _version_ | 1798038063984672768 |
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| author | Shuang Liu Yong Li Xiaojuan Yu Shaobo Han Yan Zhou Yuqi Yang Hao Zhang Zheng Jiang Chuwei Zhu Wei-Xue Li Christof Wöll Yuemin Wang Wenjie Shen |
| author_facet | Shuang Liu Yong Li Xiaojuan Yu Shaobo Han Yan Zhou Yuqi Yang Hao Zhang Zheng Jiang Chuwei Zhu Wei-Xue Li Christof Wöll Yuemin Wang Wenjie Shen |
| author_sort | Shuang Liu |
| collection | DOAJ |
| description | Quantitatively describing the atomic configuration of the catalytically active sites is challenging. Here the authors demonstrate that tuning crystal-phase of metal single-particle enables to precisely describe the atomic structure of the active sites and accurately identify the activation routes of the reacting molecules. |
| first_indexed | 2024-04-11T21:36:10Z |
| format | Article |
| id | doaj.art-c859368a7c4547aabe4ace47bd76c72c |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-11T21:36:10Z |
| publishDate | 2022-08-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-c859368a7c4547aabe4ace47bd76c72c2022-12-22T04:01:46ZengNature PortfolioNature Communications2041-17232022-08-0113111010.1038/s41467-022-32274-4Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenationShuang Liu0Yong Li1Xiaojuan Yu2Shaobo Han3Yan Zhou4Yuqi Yang5Hao Zhang6Zheng Jiang7Chuwei Zhu8Wei-Xue Li9Christof Wöll10Yuemin Wang11Wenjie Shen12State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of SciencesInstitute of Functional Interfaces, Karlsruhe Institute of TechnologyState Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of SciencesShanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of SciencesShanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of SciencesShanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of SciencesSchool of Chemistry and Materials Science, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of ChinaSchool of Chemistry and Materials Science, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of ChinaInstitute of Functional Interfaces, Karlsruhe Institute of TechnologyInstitute of Functional Interfaces, Karlsruhe Institute of TechnologyState Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of SciencesQuantitatively describing the atomic configuration of the catalytically active sites is challenging. Here the authors demonstrate that tuning crystal-phase of metal single-particle enables to precisely describe the atomic structure of the active sites and accurately identify the activation routes of the reacting molecules.https://doi.org/10.1038/s41467-022-32274-4 |
| spellingShingle | Shuang Liu Yong Li Xiaojuan Yu Shaobo Han Yan Zhou Yuqi Yang Hao Zhang Zheng Jiang Chuwei Zhu Wei-Xue Li Christof Wöll Yuemin Wang Wenjie Shen Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation Nature Communications |
| title | Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation |
| title_full | Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation |
| title_fullStr | Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation |
| title_full_unstemmed | Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation |
| title_short | Tuning crystal-phase of bimetallic single-nanoparticle for catalytic hydrogenation |
| title_sort | tuning crystal phase of bimetallic single nanoparticle for catalytic hydrogenation |
| url | https://doi.org/10.1038/s41467-022-32274-4 |
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