Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films

All-solid-state batteries (SSBs) are one of the most fascinating next-generation energy storage systems that can provide improved energy density and safety for a wide range of applications from portable electronics to electric vehicles. The development of SSBs was accelerated by the discovery of new...

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Main Authors: Gene Yang, Corey Abraham, Yuxi Ma, Myoungseok Lee, Evan Helfrick, Dahyun Oh, Dongkyu Lee
Format: Article
Language:English
Published: MDPI AG 2020-07-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/10/14/4727
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author Gene Yang
Corey Abraham
Yuxi Ma
Myoungseok Lee
Evan Helfrick
Dahyun Oh
Dongkyu Lee
author_facet Gene Yang
Corey Abraham
Yuxi Ma
Myoungseok Lee
Evan Helfrick
Dahyun Oh
Dongkyu Lee
author_sort Gene Yang
collection DOAJ
description All-solid-state batteries (SSBs) are one of the most fascinating next-generation energy storage systems that can provide improved energy density and safety for a wide range of applications from portable electronics to electric vehicles. The development of SSBs was accelerated by the discovery of new materials and the design of nanostructures. In particular, advances in the growth of thin-film battery materials facilitated the development of all solid-state thin-film batteries (SSTFBs)—expanding their applications to microelectronics such as flexible devices and implantable medical devices. However, critical challenges still remain, such as low ionic conductivity of solid electrolytes, interfacial instability and difficulty in controlling thin-film growth. In this review, we discuss the evolution of electrode and electrolyte materials for lithium-based batteries and their adoption in SSBs and SSTFBs. We highlight novel design strategies of bulk and thin-film materials to solve the issues in lithium-based batteries. We also focus on the important advances in thin-film electrodes, electrolytes and interfacial layers with the aim of providing insight into the future design of batteries. Furthermore, various thin-film fabrication techniques are also covered in this review.
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spelling doaj.art-ca2c091d48b4481d99caa69239d937aa2023-11-20T06:16:45ZengMDPI AGApplied Sciences2076-34172020-07-011014472710.3390/app10144727Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin FilmsGene Yang0Corey Abraham1Yuxi Ma2Myoungseok Lee3Evan Helfrick4Dahyun Oh5Dongkyu Lee6Department of Mechanical Engineering, College of Engineering and Computing, University of South Carolina, Columbia, SC 29208, USAChemical and Materials Engineering Department, Charles W. Davidson College of Engineering, San José State University, San José, CA 95192-0080, USADepartment of Mechanical Engineering, College of Engineering and Computing, University of South Carolina, Columbia, SC 29208, USADepartment of Mechanical Engineering, College of Engineering and Computing, University of South Carolina, Columbia, SC 29208, USADepartment of Mechanical Engineering, College of Engineering and Computing, University of South Carolina, Columbia, SC 29208, USAChemical and Materials Engineering Department, Charles W. Davidson College of Engineering, San José State University, San José, CA 95192-0080, USADepartment of Mechanical Engineering, College of Engineering and Computing, University of South Carolina, Columbia, SC 29208, USAAll-solid-state batteries (SSBs) are one of the most fascinating next-generation energy storage systems that can provide improved energy density and safety for a wide range of applications from portable electronics to electric vehicles. The development of SSBs was accelerated by the discovery of new materials and the design of nanostructures. In particular, advances in the growth of thin-film battery materials facilitated the development of all solid-state thin-film batteries (SSTFBs)—expanding their applications to microelectronics such as flexible devices and implantable medical devices. However, critical challenges still remain, such as low ionic conductivity of solid electrolytes, interfacial instability and difficulty in controlling thin-film growth. In this review, we discuss the evolution of electrode and electrolyte materials for lithium-based batteries and their adoption in SSBs and SSTFBs. We highlight novel design strategies of bulk and thin-film materials to solve the issues in lithium-based batteries. We also focus on the important advances in thin-film electrodes, electrolytes and interfacial layers with the aim of providing insight into the future design of batteries. Furthermore, various thin-film fabrication techniques are also covered in this review.https://www.mdpi.com/2076-3417/10/14/4727lithium-ion batteriessolid electrolytesall solid-state batteriesall solid-state thin-film batteriesnanostructured thin filmsinterfacial buffer layers
spellingShingle Gene Yang
Corey Abraham
Yuxi Ma
Myoungseok Lee
Evan Helfrick
Dahyun Oh
Dongkyu Lee
Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
Applied Sciences
lithium-ion batteries
solid electrolytes
all solid-state batteries
all solid-state thin-film batteries
nanostructured thin films
interfacial buffer layers
title Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
title_full Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
title_fullStr Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
title_full_unstemmed Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
title_short Advances in Materials Design for All-Solid-state Batteries: From Bulk to Thin Films
title_sort advances in materials design for all solid state batteries from bulk to thin films
topic lithium-ion batteries
solid electrolytes
all solid-state batteries
all solid-state thin-film batteries
nanostructured thin films
interfacial buffer layers
url https://www.mdpi.com/2076-3417/10/14/4727
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