A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces

Abstract We present strong enhancement of third harmonic generation in an amorphous silicon metasurface consisting of elliptical nano resonators. We show that this enhancement originates from a new type of multi-mode Fano mechanism. These ‘Super-Fano’ resonances are investigated numerically in great...

Full description

Bibliographic Details
Main Authors: David Hähnel, Christian Golla, Maximilian Albert, Thomas Zentgraf, Viktor Myroshnychenko, Jens Förstner, Cedrik Meier
Format: Article
Language:English
Published: Nature Publishing Group 2023-04-01
Series:Light: Science & Applications
Online Access:https://doi.org/10.1038/s41377-023-01134-1
_version_ 1797840816537862144
author David Hähnel
Christian Golla
Maximilian Albert
Thomas Zentgraf
Viktor Myroshnychenko
Jens Förstner
Cedrik Meier
author_facet David Hähnel
Christian Golla
Maximilian Albert
Thomas Zentgraf
Viktor Myroshnychenko
Jens Förstner
Cedrik Meier
author_sort David Hähnel
collection DOAJ
description Abstract We present strong enhancement of third harmonic generation in an amorphous silicon metasurface consisting of elliptical nano resonators. We show that this enhancement originates from a new type of multi-mode Fano mechanism. These ‘Super-Fano’ resonances are investigated numerically in great detail using full-wave simulations. The theoretically predicted behavior of the metasurface is experimentally verified by linear and nonlinear transmission spectroscopy. Moreover, quantitative nonlinear measurements are performed, in which an absolute conversion efficiency as high as η max ≈ 2.8 × 10−7 a peak power intensity of 1.2 GW cm−2 is found. Compared to an unpatterned silicon film of the same thickness amplification factors of up to ~900 are demonstrated. Our results pave the way to exploiting a strong Fano-type multi-mode coupling in metasurfaces for high THG in potential applications.
first_indexed 2024-04-09T16:20:50Z
format Article
id doaj.art-ca6d796a37084a8c93180d0c159be6c4
institution Directory Open Access Journal
issn 2047-7538
language English
last_indexed 2024-04-09T16:20:50Z
publishDate 2023-04-01
publisher Nature Publishing Group
record_format Article
series Light: Science & Applications
spelling doaj.art-ca6d796a37084a8c93180d0c159be6c42023-04-23T11:28:42ZengNature Publishing GroupLight: Science & Applications2047-75382023-04-011211810.1038/s41377-023-01134-1A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfacesDavid Hähnel0Christian Golla1Maximilian Albert2Thomas Zentgraf3Viktor Myroshnychenko4Jens Förstner5Cedrik Meier6Theoretical Electrical Engineering & CeOPP, Paderborn UniversityPhysics Department & CeOPP, Paderborn UniversityPhysics Department & CeOPP, Paderborn UniversityPhysics Department & CeOPP, Paderborn UniversityTheoretical Electrical Engineering & CeOPP, Paderborn UniversityTheoretical Electrical Engineering & CeOPP, Paderborn UniversityPhysics Department & CeOPP, Paderborn UniversityAbstract We present strong enhancement of third harmonic generation in an amorphous silicon metasurface consisting of elliptical nano resonators. We show that this enhancement originates from a new type of multi-mode Fano mechanism. These ‘Super-Fano’ resonances are investigated numerically in great detail using full-wave simulations. The theoretically predicted behavior of the metasurface is experimentally verified by linear and nonlinear transmission spectroscopy. Moreover, quantitative nonlinear measurements are performed, in which an absolute conversion efficiency as high as η max ≈ 2.8 × 10−7 a peak power intensity of 1.2 GW cm−2 is found. Compared to an unpatterned silicon film of the same thickness amplification factors of up to ~900 are demonstrated. Our results pave the way to exploiting a strong Fano-type multi-mode coupling in metasurfaces for high THG in potential applications.https://doi.org/10.1038/s41377-023-01134-1
spellingShingle David Hähnel
Christian Golla
Maximilian Albert
Thomas Zentgraf
Viktor Myroshnychenko
Jens Förstner
Cedrik Meier
A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
Light: Science & Applications
title A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
title_full A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
title_fullStr A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
title_full_unstemmed A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
title_short A multi-mode super-fano mechanism for enhanced third harmonic generation in silicon metasurfaces
title_sort multi mode super fano mechanism for enhanced third harmonic generation in silicon metasurfaces
url https://doi.org/10.1038/s41377-023-01134-1
work_keys_str_mv AT davidhahnel amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT christiangolla amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT maximilianalbert amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT thomaszentgraf amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT viktormyroshnychenko amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT jensforstner amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT cedrikmeier amultimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT davidhahnel multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT christiangolla multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT maximilianalbert multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT thomaszentgraf multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT viktormyroshnychenko multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT jensforstner multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces
AT cedrikmeier multimodesuperfanomechanismforenhancedthirdharmonicgenerationinsiliconmetasurfaces