Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest

<p>The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to me...

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Main Authors: R. Herbert, P. Stier
Format: Article
Language:English
Published: Copernicus Publications 2023-04-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/23/4595/2023/acp-23-4595-2023.pdf
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author R. Herbert
P. Stier
author_facet R. Herbert
P. Stier
author_sort R. Herbert
collection DOAJ
description <p>The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to measure for purposes of gaining a representative understanding of smoke impacts on the Amazonian atmosphere. In this study, we use multiple collocated satellite sensors on board AQUA and TERRA platforms to study the underlying smoke–cloud–radiation interactions during the diurnal cycle. An 18-year time series for both morning and afternoon overpasses is constructed, providing collocated measurements of aerosol optical depth (AOD; column-integrated aerosol extinction), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water vapour content from independent sources.</p> <p>The long-term time series reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD <span class="inline-formula">≤</span> 0.4) enhance convective activity, cloudiness, and precipitation, but higher loadings (AOD <span class="inline-formula">&gt;</span> 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings, suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 W m<span class="inline-formula"><sup>−2</sup></span> for an AOD perturbation of <span class="inline-formula">+</span>1.0.</p> <p>The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning and afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land use change, and deforestation will have important and widespread impacts on the region over the coming decades. Based on this analysis, we anticipate that further increases in anthropogenic fire activity will associated with an overall reduction in regional precipitation and a negative forcing (cooling) on the Earth's energy budget.</p>
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spelling doaj.art-cb4a448dd0694520a8ee19539d2bcf6f2023-04-17T10:32:41ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242023-04-01234595461610.5194/acp-23-4595-2023Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforestR. HerbertP. Stier<p>The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to measure for purposes of gaining a representative understanding of smoke impacts on the Amazonian atmosphere. In this study, we use multiple collocated satellite sensors on board AQUA and TERRA platforms to study the underlying smoke–cloud–radiation interactions during the diurnal cycle. An 18-year time series for both morning and afternoon overpasses is constructed, providing collocated measurements of aerosol optical depth (AOD; column-integrated aerosol extinction), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water vapour content from independent sources.</p> <p>The long-term time series reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD <span class="inline-formula">≤</span> 0.4) enhance convective activity, cloudiness, and precipitation, but higher loadings (AOD <span class="inline-formula">&gt;</span> 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings, suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 W m<span class="inline-formula"><sup>−2</sup></span> for an AOD perturbation of <span class="inline-formula">+</span>1.0.</p> <p>The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning and afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land use change, and deforestation will have important and widespread impacts on the region over the coming decades. Based on this analysis, we anticipate that further increases in anthropogenic fire activity will associated with an overall reduction in regional precipitation and a negative forcing (cooling) on the Earth's energy budget.</p>https://acp.copernicus.org/articles/23/4595/2023/acp-23-4595-2023.pdf
spellingShingle R. Herbert
P. Stier
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Atmospheric Chemistry and Physics
title Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
title_full Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
title_fullStr Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
title_full_unstemmed Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
title_short Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
title_sort satellite observations of smoke cloud radiation interactions over the amazon rainforest
url https://acp.copernicus.org/articles/23/4595/2023/acp-23-4595-2023.pdf
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