Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide

Abstract The realization of compact and efficient broadband mid-infrared (MIR) lasers has enormous impacts in promoting MIR spectroscopy for various important applications. A number of well-designed waveguide platforms have been demonstrated for MIR supercontinuum and frequency comb generations base...

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Main Authors: Bo Hu, Xuemei Yang, Jiangen Wu, Siyi Lu, Hang Yang, Zhe Long, Linzhen He, Xing Luo, Kan Tian, Weizhe Wang, Yang Li, Han Wu, Wenlong Li, Chunyu Guo, Huan Yang, Qi Jie Wang, Houkun Liang
Format: Article
Language:English
Published: Nature Portfolio 2023-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-42912-0
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author Bo Hu
Xuemei Yang
Jiangen Wu
Siyi Lu
Hang Yang
Zhe Long
Linzhen He
Xing Luo
Kan Tian
Weizhe Wang
Yang Li
Han Wu
Wenlong Li
Chunyu Guo
Huan Yang
Qi Jie Wang
Houkun Liang
author_facet Bo Hu
Xuemei Yang
Jiangen Wu
Siyi Lu
Hang Yang
Zhe Long
Linzhen He
Xing Luo
Kan Tian
Weizhe Wang
Yang Li
Han Wu
Wenlong Li
Chunyu Guo
Huan Yang
Qi Jie Wang
Houkun Liang
author_sort Bo Hu
collection DOAJ
description Abstract The realization of compact and efficient broadband mid-infrared (MIR) lasers has enormous impacts in promoting MIR spectroscopy for various important applications. A number of well-designed waveguide platforms have been demonstrated for MIR supercontinuum and frequency comb generations based on cubic nonlinearities, but unfortunately third-order nonlinear response is inherently weak. Here, we propose and demonstrate for the first time a χ (2) micrometer waveguide platform based on birefringence phase matching for long-wavelength infrared (LWIR) laser generation with a high quantum efficiency. In a ZnGeP2-based waveguide platform, an octave-spanning spectrum covering 5–11 μm is generated through optical parametric generation (OPG). A quantum conversion efficiency of 74% as a new record in LWIR single-pass parametric processes is achieved. The threshold energy is measured as ~616 pJ, reduced by more than 1-order of magnitude as compared to those of MIR OPGs in bulk media. Our prototype micro-waveguide platform could be extended to other χ (2) birefringence crystals and trigger new frontiers of MIR integrated nonlinear photonics.
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spelling doaj.art-cb75d2f0f01a41b6875b4b2bf9b1a8f82023-11-12T12:23:05ZengNature PortfolioNature Communications2041-17232023-11-0114111010.1038/s41467-023-42912-0Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguideBo Hu0Xuemei Yang1Jiangen Wu2Siyi Lu3Hang Yang4Zhe Long5Linzhen He6Xing Luo7Kan Tian8Weizhe Wang9Yang Li10Han Wu11Wenlong Li12Chunyu Guo13Huan Yang14Qi Jie Wang15Houkun Liang16School of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySino-German College of Intelligent Manufacturing, Shenzhen Technology UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversityCollege of Physics and Optoelectronic Engineering, Shenzhen UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversitySchool of Electronics and Information Engineering, Sichuan UniversityChengdu Dien PHOTOELECTRIC Technology Co., Ltd.College of Physics and Optoelectronic Engineering, Shenzhen UniversitySino-German College of Intelligent Manufacturing, Shenzhen Technology UniversitySchool of Electrical & Electronic Engineering & The Photonics Institute, Nanyang Technological UniversitySchool of Electronics and Information Engineering, Sichuan UniversityAbstract The realization of compact and efficient broadband mid-infrared (MIR) lasers has enormous impacts in promoting MIR spectroscopy for various important applications. A number of well-designed waveguide platforms have been demonstrated for MIR supercontinuum and frequency comb generations based on cubic nonlinearities, but unfortunately third-order nonlinear response is inherently weak. Here, we propose and demonstrate for the first time a χ (2) micrometer waveguide platform based on birefringence phase matching for long-wavelength infrared (LWIR) laser generation with a high quantum efficiency. In a ZnGeP2-based waveguide platform, an octave-spanning spectrum covering 5–11 μm is generated through optical parametric generation (OPG). A quantum conversion efficiency of 74% as a new record in LWIR single-pass parametric processes is achieved. The threshold energy is measured as ~616 pJ, reduced by more than 1-order of magnitude as compared to those of MIR OPGs in bulk media. Our prototype micro-waveguide platform could be extended to other χ (2) birefringence crystals and trigger new frontiers of MIR integrated nonlinear photonics.https://doi.org/10.1038/s41467-023-42912-0
spellingShingle Bo Hu
Xuemei Yang
Jiangen Wu
Siyi Lu
Hang Yang
Zhe Long
Linzhen He
Xing Luo
Kan Tian
Weizhe Wang
Yang Li
Han Wu
Wenlong Li
Chunyu Guo
Huan Yang
Qi Jie Wang
Houkun Liang
Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
Nature Communications
title Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
title_full Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
title_fullStr Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
title_full_unstemmed Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
title_short Highly efficient octave-spanning long-wavelength infrared generation with a 74% quantum efficiency in a χ (2) waveguide
title_sort highly efficient octave spanning long wavelength infrared generation with a 74 quantum efficiency in a χ 2 waveguide
url https://doi.org/10.1038/s41467-023-42912-0
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