Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application

In the present investigation, we prepared cellulose nanocrystal (CNC)-reinforced polyvinyl alcohol-cellulose (PVA-Cell) physical hydrogels using a simple blending method for actuator application. The prepared hydrogels were characterized by Fourier transform infrared spectroscopy, X-ray diffraction,...

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Main Authors: Jaehwan Kim, Tippabattini Jayaramudu, Lindong Zhai, Hyun Chan Kim, Dickens Owino Agumba
Format: Article
Language:English
Published: MDPI AG 2020-10-01
Series:Crystals
Subjects:
Online Access:https://www.mdpi.com/2073-4352/10/11/969
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author Jaehwan Kim
Tippabattini Jayaramudu
Lindong Zhai
Hyun Chan Kim
Dickens Owino Agumba
author_facet Jaehwan Kim
Tippabattini Jayaramudu
Lindong Zhai
Hyun Chan Kim
Dickens Owino Agumba
author_sort Jaehwan Kim
collection DOAJ
description In the present investigation, we prepared cellulose nanocrystal (CNC)-reinforced polyvinyl alcohol-cellulose (PVA-Cell) physical hydrogels using a simple blending method for actuator application. The prepared hydrogels were characterized by Fourier transform infrared spectroscopy, X-ray diffraction, and the surface and cross-section were studied by scanning electron microscopy. CNCs were well dispersed in the PVA-Cell hydrogel. In the preparation process, surface hydroxyl groups of the CNC and PVA-Cell matrix hydroxyl groups were interacted to produce uniform dispersion of CNCs in the hydrogels. Swelling behavior and compression studies revealed that the increase of the CNCs reinforced the crosslinking. The actuation test of the prepared hydrogels showed that the displacement linearly increased with the voltage, and the immense output displacement was observed at low CNC concentration. The prepared hydrogels are applicable for soft robot actuators and active lens.
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spelling doaj.art-cbd17dc118d6418a86af578869a0d15a2023-11-20T18:35:08ZengMDPI AGCrystals2073-43522020-10-01101196910.3390/cryst10110969Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator ApplicationJaehwan Kim0Tippabattini Jayaramudu1Lindong Zhai2Hyun Chan Kim3Dickens Owino Agumba4Center for Nanocellulose Future Composites, Department of Mechanical Engineering, Inha University, 100 Inha-ro, Michuhol-ku, Incheon 22212, KoreaCenter for Nanocellulose Future Composites, Department of Mechanical Engineering, Inha University, 100 Inha-ro, Michuhol-ku, Incheon 22212, KoreaCenter for Nanocellulose Future Composites, Department of Mechanical Engineering, Inha University, 100 Inha-ro, Michuhol-ku, Incheon 22212, KoreaCenter for Nanocellulose Future Composites, Department of Mechanical Engineering, Inha University, 100 Inha-ro, Michuhol-ku, Incheon 22212, KoreaCenter for Nanocellulose Future Composites, Department of Mechanical Engineering, Inha University, 100 Inha-ro, Michuhol-ku, Incheon 22212, KoreaIn the present investigation, we prepared cellulose nanocrystal (CNC)-reinforced polyvinyl alcohol-cellulose (PVA-Cell) physical hydrogels using a simple blending method for actuator application. The prepared hydrogels were characterized by Fourier transform infrared spectroscopy, X-ray diffraction, and the surface and cross-section were studied by scanning electron microscopy. CNCs were well dispersed in the PVA-Cell hydrogel. In the preparation process, surface hydroxyl groups of the CNC and PVA-Cell matrix hydroxyl groups were interacted to produce uniform dispersion of CNCs in the hydrogels. Swelling behavior and compression studies revealed that the increase of the CNCs reinforced the crosslinking. The actuation test of the prepared hydrogels showed that the displacement linearly increased with the voltage, and the immense output displacement was observed at low CNC concentration. The prepared hydrogels are applicable for soft robot actuators and active lens.https://www.mdpi.com/2073-4352/10/11/969soft actuatorsphysical hydrogelscellulose nanocrystalsphysical crosslinking
spellingShingle Jaehwan Kim
Tippabattini Jayaramudu
Lindong Zhai
Hyun Chan Kim
Dickens Owino Agumba
Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
Crystals
soft actuators
physical hydrogels
cellulose nanocrystals
physical crosslinking
title Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
title_full Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
title_fullStr Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
title_full_unstemmed Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
title_short Preparation of Cellulose Nanocrystal-Reinforced Physical Hydrogels for Actuator Application
title_sort preparation of cellulose nanocrystal reinforced physical hydrogels for actuator application
topic soft actuators
physical hydrogels
cellulose nanocrystals
physical crosslinking
url https://www.mdpi.com/2073-4352/10/11/969
work_keys_str_mv AT jaehwankim preparationofcellulosenanocrystalreinforcedphysicalhydrogelsforactuatorapplication
AT tippabattinijayaramudu preparationofcellulosenanocrystalreinforcedphysicalhydrogelsforactuatorapplication
AT lindongzhai preparationofcellulosenanocrystalreinforcedphysicalhydrogelsforactuatorapplication
AT hyunchankim preparationofcellulosenanocrystalreinforcedphysicalhydrogelsforactuatorapplication
AT dickensowinoagumba preparationofcellulosenanocrystalreinforcedphysicalhydrogelsforactuatorapplication