Direct observation of nuclear reorganization driven by ultrafast spin transitions
Electron spin is a fundamental property of molecules, and changes in spin state affect both molecular structure and dynamics. Here, the authors resolve, by ultrafast electron diffraction, the nuclear reorganization stabilizing spin transitions in a [FeII(bpy)3](PF6)2 crystal.
| Main Authors: | , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2020-03-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-020-15187-y |
| _version_ | 1818400489726803968 |
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| author | Yifeng Jiang Lai Chung Liu Antoine Sarracini Kamil M. Krawczyk Jordan S. Wentzell Cheng Lu Ryan L. Field Samir F. Matar Wojciech Gawelda Henrike M. Müller-Werkmeister R. J. Dwayne Miller |
| author_facet | Yifeng Jiang Lai Chung Liu Antoine Sarracini Kamil M. Krawczyk Jordan S. Wentzell Cheng Lu Ryan L. Field Samir F. Matar Wojciech Gawelda Henrike M. Müller-Werkmeister R. J. Dwayne Miller |
| author_sort | Yifeng Jiang |
| collection | DOAJ |
| description | Electron spin is a fundamental property of molecules, and changes in spin state affect both molecular structure and dynamics. Here, the authors resolve, by ultrafast electron diffraction, the nuclear reorganization stabilizing spin transitions in a [FeII(bpy)3](PF6)2 crystal. |
| first_indexed | 2024-12-14T07:37:23Z |
| format | Article |
| id | doaj.art-cc1c2628961b4f3698e25d91530b557a |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-12-14T07:37:23Z |
| publishDate | 2020-03-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-cc1c2628961b4f3698e25d91530b557a2022-12-21T23:11:08ZengNature PortfolioNature Communications2041-17232020-03-011111810.1038/s41467-020-15187-yDirect observation of nuclear reorganization driven by ultrafast spin transitionsYifeng Jiang0Lai Chung Liu1Antoine Sarracini2Kamil M. Krawczyk3Jordan S. Wentzell4Cheng Lu5Ryan L. Field6Samir F. Matar7Wojciech Gawelda8Henrike M. Müller-Werkmeister9R. J. Dwayne Miller10Max Planck Institute for the Structure and Dynamics of MatterDepartments of Chemistry and Physics, University of TorontoDepartments of Chemistry and Physics, University of TorontoDepartments of Chemistry and Physics, University of TorontoDepartments of Chemistry and Physics, University of TorontoDepartments of Chemistry and Physics, University of TorontoDepartments of Chemistry and Physics, University of TorontoLebanese German UniversityEuropean XFELInstitute of Chemistry, University of PotsdamMax Planck Institute for the Structure and Dynamics of MatterElectron spin is a fundamental property of molecules, and changes in spin state affect both molecular structure and dynamics. Here, the authors resolve, by ultrafast electron diffraction, the nuclear reorganization stabilizing spin transitions in a [FeII(bpy)3](PF6)2 crystal.https://doi.org/10.1038/s41467-020-15187-y |
| spellingShingle | Yifeng Jiang Lai Chung Liu Antoine Sarracini Kamil M. Krawczyk Jordan S. Wentzell Cheng Lu Ryan L. Field Samir F. Matar Wojciech Gawelda Henrike M. Müller-Werkmeister R. J. Dwayne Miller Direct observation of nuclear reorganization driven by ultrafast spin transitions Nature Communications |
| title | Direct observation of nuclear reorganization driven by ultrafast spin transitions |
| title_full | Direct observation of nuclear reorganization driven by ultrafast spin transitions |
| title_fullStr | Direct observation of nuclear reorganization driven by ultrafast spin transitions |
| title_full_unstemmed | Direct observation of nuclear reorganization driven by ultrafast spin transitions |
| title_short | Direct observation of nuclear reorganization driven by ultrafast spin transitions |
| title_sort | direct observation of nuclear reorganization driven by ultrafast spin transitions |
| url | https://doi.org/10.1038/s41467-020-15187-y |
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