Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N
<p>We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a...
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Copernicus Publications
2021-01-01
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| Series: | Atmospheric Chemistry and Physics |
| Online Access: | https://acp.copernicus.org/articles/21/989/2021/acp-21-989-2021.pdf |
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| author | J. Schneider R. Weigel T. Klimach A. Dragoneas A. Dragoneas O. Appel O. Appel A. Hünig A. Hünig S. Molleker S. Molleker F. Köllner F. Köllner H.-C. Clemen O. Eppers O. Eppers P. Hoppe P. Hoor C. Mahnke C. Mahnke C. Mahnke M. Krämer M. Krämer C. Rolf J.-U. Grooß A. Zahn F. Obersteiner F. Ravegnani A. Ulanovsky H. Schlager M. Scheibe G. S. Diskin J. P. DiGangi J. B. Nowak M. Zöger S. Borrmann S. Borrmann |
| author_facet | J. Schneider R. Weigel T. Klimach A. Dragoneas A. Dragoneas O. Appel O. Appel A. Hünig A. Hünig S. Molleker S. Molleker F. Köllner F. Köllner H.-C. Clemen O. Eppers O. Eppers P. Hoppe P. Hoor C. Mahnke C. Mahnke C. Mahnke M. Krämer M. Krämer C. Rolf J.-U. Grooß A. Zahn F. Obersteiner F. Ravegnani A. Ulanovsky H. Schlager M. Scheibe G. S. Diskin J. P. DiGangi J. B. Nowak M. Zöger S. Borrmann S. Borrmann |
| author_sort | J. Schneider |
| collection | DOAJ |
| description | <p>We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles
containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a
low-altitude aircraft mission show that meteoric material is also present within middle- and lower-tropospheric aerosol but within only a very small
proportion of particles. For both the UTLS campaigns and the lower- and mid-troposphere observations, the measurements were conducted with single-particle laser ablation mass spectrometers with bipolar-ion detection, which enabled us to measure the chemical composition of particles in a diameter
range of approximately 150 <span class="inline-formula">nm</span> to 3 <span class="inline-formula">µm</span>. The five UTLS aircraft missions cover a latitude range from 15 to 68<span class="inline-formula"><sup>∘</sup></span> N,
altitudes up to 21 <span class="inline-formula">km</span>, and a potential temperature range from 280 to 480 <span class="inline-formula">K</span>. In total, 338 363 single particles were analysed, of
which 147 338 were measured in the stratosphere. Of these total particles, 50 688 were characterized by high abundances of magnesium and iron,
together with sulfuric ions, the vast majority (48 610) in the stratosphere, and are interpreted as meteoric material immersed or dissolved within
sulfuric acid. It must be noted that the relative abundance of such meteoric particles may be overestimated by about 10 % to 30 % due to the
presence of pure sulfuric acid particles in the stratosphere which are not detected by the instruments used here. Below the tropopause, the observed
fraction of the meteoric particle type decreased sharply with 0.2 %–1 % abundance at Jungfraujoch, and smaller abundances
(0.025 %–0.05 %) were observed during the lower-altitude Canadian Arctic aircraft measurements. The size distribution of the meteoric sulfuric
particles measured in the UTLS campaigns is consistent with earlier aircraft-based mass-spectrometric measurements, with only 5 %–10 %
fractions in the smallest particles detected (200–300 <span class="inline-formula">nm</span> diameter) but with substantial (<span class="inline-formula">></span> 40 %) abundance fractions for particles
from 300–350 up to 900 <span class="inline-formula">nm</span> in diameter, suggesting sedimentation is the primary loss mechanism. In the tropical lower stratosphere, only a
small fraction (<span class="inline-formula"><</span> 10 %) of the analysed particles contained meteoric material. In contrast, in the extratropics the<span id="page990"/> observed fraction of
meteoric particles reached 20 %–40 % directly above the tropopause. At potential temperature levels of more than 40 <span class="inline-formula">K</span> above the
thermal tropopause, particles containing meteoric material were observed in much higher relative abundances than near the tropopause, and, at these
altitudes, they occurred at a similar abundance fraction across all latitudes and seasons measured. Above 440 <span class="inline-formula">K</span>, the observed fraction of meteoric
particles is above 60 % at latitudes between 20 and 42<span class="inline-formula"><sup>∘</sup></span> N. Meteoric smoke particles are transported from the mesosphere into the
stratosphere within the winter polar vortex and are subsequently distributed towards low latitudes by isentropic mixing, typically below a potential temperature of 440 <span class="inline-formula">K</span>. By contrast, the findings from the UTLS measurements show that meteoric material is found in stratospheric
aerosol particles at all latitudes and seasons, which suggests that either isentropic mixing is effective also above 440 <span class="inline-formula">K</span> or that meteoric
fragments may be the source of a substantial proportion of the observed meteoric material.</p> |
| first_indexed | 2024-12-14T22:24:31Z |
| format | Article |
| id | doaj.art-ccb3258ea0c345c5873eadf9a39a5e47 |
| institution | Directory Open Access Journal |
| issn | 1680-7316 1680-7324 |
| language | English |
| last_indexed | 2024-12-14T22:24:31Z |
| publishDate | 2021-01-01 |
| publisher | Copernicus Publications |
| record_format | Article |
| series | Atmospheric Chemistry and Physics |
| spelling | doaj.art-ccb3258ea0c345c5873eadf9a39a5e472022-12-21T22:45:24ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242021-01-0121989101310.5194/acp-21-989-2021Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° NJ. Schneider0R. Weigel1T. Klimach2A. Dragoneas3A. Dragoneas4O. Appel5O. Appel6A. Hünig7A. Hünig8S. Molleker9S. Molleker10F. Köllner11F. Köllner12H.-C. Clemen13O. Eppers14O. Eppers15P. Hoppe16P. Hoor17C. Mahnke18C. Mahnke19C. Mahnke20M. Krämer21M. Krämer22C. Rolf23J.-U. Grooß24A. Zahn25F. Obersteiner26F. Ravegnani27A. Ulanovsky28H. Schlager29M. Scheibe30G. S. Diskin31J. P. DiGangi32J. B. Nowak33M. Zöger34S. Borrmann35S. Borrmann36Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyInstitute of Energy and Climate Research, Forschungszentrum Jülich, Jülich, 52425, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, GermanyInstitute of Energy and Climate Research, Forschungszentrum Jülich, Jülich, 52425, GermanyInstitute of Energy and Climate Research, Forschungszentrum Jülich, Jülich, 52425, GermanyInstitute of Energy and Climate Research, Forschungszentrum Jülich, Jülich, 52425, GermanyInstitute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Eggenstein-Leopoldshafen, 76344, GermanyInstitute of Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Eggenstein-Leopoldshafen, 76344, GermanyInstitute of Atmospheric Sciences and Climate, ISAC-CNR, Bologna, 40129, ItalyCentral Aerological Observatory, Dolgoprudny, Moscow region, 141700, RussiaInstitute of Atmospheric Physics, German Aerospace Center (DLR) Oberpfaffenhofen, Wessling, 82234, GermanyInstitute of Atmospheric Physics, German Aerospace Center (DLR) Oberpfaffenhofen, Wessling, 82234, GermanyNASA Langley Research Center, MS 483, Hampton, VA 23681, USANASA Langley Research Center, MS 483, Hampton, VA 23681, USANASA Langley Research Center, MS 483, Hampton, VA 23681, USAFlight Experiments, German Aerospace Center (DLR) Oberpfaffenhofen, Wessling, 82234, GermanyParticle Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, GermanyInstitute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, 55128, Germany<p>We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a low-altitude aircraft mission show that meteoric material is also present within middle- and lower-tropospheric aerosol but within only a very small proportion of particles. For both the UTLS campaigns and the lower- and mid-troposphere observations, the measurements were conducted with single-particle laser ablation mass spectrometers with bipolar-ion detection, which enabled us to measure the chemical composition of particles in a diameter range of approximately 150 <span class="inline-formula">nm</span> to 3 <span class="inline-formula">µm</span>. The five UTLS aircraft missions cover a latitude range from 15 to 68<span class="inline-formula"><sup>∘</sup></span> N, altitudes up to 21 <span class="inline-formula">km</span>, and a potential temperature range from 280 to 480 <span class="inline-formula">K</span>. In total, 338 363 single particles were analysed, of which 147 338 were measured in the stratosphere. Of these total particles, 50 688 were characterized by high abundances of magnesium and iron, together with sulfuric ions, the vast majority (48 610) in the stratosphere, and are interpreted as meteoric material immersed or dissolved within sulfuric acid. It must be noted that the relative abundance of such meteoric particles may be overestimated by about 10 % to 30 % due to the presence of pure sulfuric acid particles in the stratosphere which are not detected by the instruments used here. Below the tropopause, the observed fraction of the meteoric particle type decreased sharply with 0.2 %–1 % abundance at Jungfraujoch, and smaller abundances (0.025 %–0.05 %) were observed during the lower-altitude Canadian Arctic aircraft measurements. The size distribution of the meteoric sulfuric particles measured in the UTLS campaigns is consistent with earlier aircraft-based mass-spectrometric measurements, with only 5 %–10 % fractions in the smallest particles detected (200–300 <span class="inline-formula">nm</span> diameter) but with substantial (<span class="inline-formula">></span> 40 %) abundance fractions for particles from 300–350 up to 900 <span class="inline-formula">nm</span> in diameter, suggesting sedimentation is the primary loss mechanism. In the tropical lower stratosphere, only a small fraction (<span class="inline-formula"><</span> 10 %) of the analysed particles contained meteoric material. In contrast, in the extratropics the<span id="page990"/> observed fraction of meteoric particles reached 20 %–40 % directly above the tropopause. At potential temperature levels of more than 40 <span class="inline-formula">K</span> above the thermal tropopause, particles containing meteoric material were observed in much higher relative abundances than near the tropopause, and, at these altitudes, they occurred at a similar abundance fraction across all latitudes and seasons measured. Above 440 <span class="inline-formula">K</span>, the observed fraction of meteoric particles is above 60 % at latitudes between 20 and 42<span class="inline-formula"><sup>∘</sup></span> N. Meteoric smoke particles are transported from the mesosphere into the stratosphere within the winter polar vortex and are subsequently distributed towards low latitudes by isentropic mixing, typically below a potential temperature of 440 <span class="inline-formula">K</span>. By contrast, the findings from the UTLS measurements show that meteoric material is found in stratospheric aerosol particles at all latitudes and seasons, which suggests that either isentropic mixing is effective also above 440 <span class="inline-formula">K</span> or that meteoric fragments may be the source of a substantial proportion of the observed meteoric material.</p>https://acp.copernicus.org/articles/21/989/2021/acp-21-989-2021.pdf |
| spellingShingle | J. Schneider R. Weigel T. Klimach A. Dragoneas A. Dragoneas O. Appel O. Appel A. Hünig A. Hünig S. Molleker S. Molleker F. Köllner F. Köllner H.-C. Clemen O. Eppers O. Eppers P. Hoppe P. Hoor C. Mahnke C. Mahnke C. Mahnke M. Krämer M. Krämer C. Rolf J.-U. Grooß A. Zahn F. Obersteiner F. Ravegnani A. Ulanovsky H. Schlager M. Scheibe G. S. Diskin J. P. DiGangi J. B. Nowak M. Zöger S. Borrmann S. Borrmann Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N Atmospheric Chemistry and Physics |
| title | Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N |
| title_full | Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N |
| title_fullStr | Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N |
| title_full_unstemmed | Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N |
| title_short | Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N |
| title_sort | aircraft based observation of meteoric material in lower stratospheric aerosol particles between 15 and 68° thinsp n |
| url | https://acp.copernicus.org/articles/21/989/2021/acp-21-989-2021.pdf |
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