New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau

Atmospheric heavy metals have important environmental and health threats. To investigate atmospheric deposition and contamination of heavy metal elements in the glaciers of the eastern Tibetan Plateau (ETP), we collected the surface snow (cryoconites) samples in the Lenglongling Glacier (LG), the Ga...

Full description

Bibliographic Details
Main Authors: Xiaoyu Jiao, Zhiwen Dong, Shichang Kang, Yifan Li, Cong Jiang, Masoud Rostami
Format: Article
Language:English
Published: Elsevier 2021-01-01
Series:Ecotoxicology and Environmental Safety
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S0147651320310666
_version_ 1819315729108828160
author Xiaoyu Jiao
Zhiwen Dong
Shichang Kang
Yifan Li
Cong Jiang
Masoud Rostami
author_facet Xiaoyu Jiao
Zhiwen Dong
Shichang Kang
Yifan Li
Cong Jiang
Masoud Rostami
author_sort Xiaoyu Jiao
collection DOAJ
description Atmospheric heavy metals have important environmental and health threats. To investigate atmospheric deposition and contamination of heavy metal elements in the glaciers of the eastern Tibetan Plateau (ETP), we collected the surface snow (cryoconites) samples in the Lenglongling Glacier (LG), the Gannan Snowpack (GS), the Dagu Glacier (DG), the Hailuogou Glacier (HG) and Yulong Snow-mountain Glacier (YG) in summer 2017. Samples were analyzed for concentrations and enrichment factors (EFs) of Al and trace elements (Pb, Co, Cd, Ba, Mn, Ga, Sc, V, Zn, Cr, Ni, Cu, Rb, Sb, Cs, As, Mo, Li) using inductively coupled plasma-mass spectrometry (ICP-MS). Results showed that the concentrations and EFs of heavy metals (e.g. Sb, Cu, Cr, Ni, As, Mo) were generally high value in YG, GS and LG, while were relatively low value in DG and HG, implying that ETP glaciers may have been affected by atmospheric anthropogenic pollutants deposition to varying degrees. Comparing the heavy metal concentrations in the glaciers with those in the precipitation of middle/eastern China cities and also the South Asian cities, we find that the glacial heavy metal concentrations were generally low level, though the anthropogenic pollutants were still significantly enriched. Taking the spatial distribution of As and Ni concentration/EFs in the glaciers and surrounding urban precipitation as an example, we find that the heavy metal pollutants were probably transported to the glaciers through three routes from the surrounding densely populated area of Asia. The MODIS AOD and NCEP/NCAR wind vector also demonstrated that the atmospheric pollutants originated from anthropogenic emissions of urban areas of both South Asia, and northwest and east China, mainly caused by the large scale atmospheric circulation (e.g. the South Asian Monsoon, westerlies and Eastern Asian Summer Monsoon). Therefore, control of these potential pollution emission sources of the surrounding densely populated areas in Asia could be important to ETP glaciers in future perspectives.
first_indexed 2024-12-24T10:04:44Z
format Article
id doaj.art-cd8b4ee32bcb4b30b4718d2df7d09f1a
institution Directory Open Access Journal
issn 0147-6513
language English
last_indexed 2024-12-24T10:04:44Z
publishDate 2021-01-01
publisher Elsevier
record_format Article
series Ecotoxicology and Environmental Safety
spelling doaj.art-cd8b4ee32bcb4b30b4718d2df7d09f1a2022-12-21T17:00:53ZengElsevierEcotoxicology and Environmental Safety0147-65132021-01-01207111228New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan PlateauXiaoyu Jiao0Zhiwen Dong1Shichang Kang2Yifan Li3Cong Jiang4Masoud Rostami5State Key Laboratory of Cryosphere Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou, 730000, China; University of Chinese Academy of Sciences, Beijing, 100049, ChinaState Key Laboratory of Cryosphere Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou, 730000, China; CAS Center for Excellence in Tibetan Plateau Earth Sciences, Chinese Academy of Sciences (CAS), Beijing, 100101, China; Corresponding author. State Key Laboratory of Cryosphere Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou, 730000, China.State Key Laboratory of Cryosphere Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou, 730000, China; CAS Center for Excellence in Tibetan Plateau Earth Sciences, Chinese Academy of Sciences (CAS), Beijing, 100101, ChinaInstitute for Geophysics and Meteorology, University of Cologne, Cologne, D-50923, GermanyInstitute for Geophysics and Meteorology, University of Cologne, Cologne, D-50923, GermanyInstitute for Geophysics and Meteorology, University of Cologne, Cologne, D-50923, GermanyAtmospheric heavy metals have important environmental and health threats. To investigate atmospheric deposition and contamination of heavy metal elements in the glaciers of the eastern Tibetan Plateau (ETP), we collected the surface snow (cryoconites) samples in the Lenglongling Glacier (LG), the Gannan Snowpack (GS), the Dagu Glacier (DG), the Hailuogou Glacier (HG) and Yulong Snow-mountain Glacier (YG) in summer 2017. Samples were analyzed for concentrations and enrichment factors (EFs) of Al and trace elements (Pb, Co, Cd, Ba, Mn, Ga, Sc, V, Zn, Cr, Ni, Cu, Rb, Sb, Cs, As, Mo, Li) using inductively coupled plasma-mass spectrometry (ICP-MS). Results showed that the concentrations and EFs of heavy metals (e.g. Sb, Cu, Cr, Ni, As, Mo) were generally high value in YG, GS and LG, while were relatively low value in DG and HG, implying that ETP glaciers may have been affected by atmospheric anthropogenic pollutants deposition to varying degrees. Comparing the heavy metal concentrations in the glaciers with those in the precipitation of middle/eastern China cities and also the South Asian cities, we find that the glacial heavy metal concentrations were generally low level, though the anthropogenic pollutants were still significantly enriched. Taking the spatial distribution of As and Ni concentration/EFs in the glaciers and surrounding urban precipitation as an example, we find that the heavy metal pollutants were probably transported to the glaciers through three routes from the surrounding densely populated area of Asia. The MODIS AOD and NCEP/NCAR wind vector also demonstrated that the atmospheric pollutants originated from anthropogenic emissions of urban areas of both South Asia, and northwest and east China, mainly caused by the large scale atmospheric circulation (e.g. the South Asian Monsoon, westerlies and Eastern Asian Summer Monsoon). Therefore, control of these potential pollution emission sources of the surrounding densely populated areas in Asia could be important to ETP glaciers in future perspectives.http://www.sciencedirect.com/science/article/pii/S0147651320310666Heavy metal elementsAtmospheric pollutantsTransport routesEastern Tibetan plateau glaciers
spellingShingle Xiaoyu Jiao
Zhiwen Dong
Shichang Kang
Yifan Li
Cong Jiang
Masoud Rostami
New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
Ecotoxicology and Environmental Safety
Heavy metal elements
Atmospheric pollutants
Transport routes
Eastern Tibetan plateau glaciers
title New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
title_full New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
title_fullStr New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
title_full_unstemmed New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
title_short New insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern Tibetan Plateau
title_sort new insights into heavy metal elements deposition in the snowpacks of mountain glaciers in the eastern tibetan plateau
topic Heavy metal elements
Atmospheric pollutants
Transport routes
Eastern Tibetan plateau glaciers
url http://www.sciencedirect.com/science/article/pii/S0147651320310666
work_keys_str_mv AT xiaoyujiao newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau
AT zhiwendong newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau
AT shichangkang newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau
AT yifanli newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau
AT congjiang newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau
AT masoudrostami newinsightsintoheavymetalelementsdepositioninthesnowpacksofmountainglaciersintheeasterntibetanplateau