Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China

This study investigated the hydrochemical characteristics and human health risks of groundwater in a pollution accident site. By collecting 27 samples, the content of the heavy metal(oid)s (As, Cd, Cr, Cu, Hg, Ni, Pb, and Zn) was tested, statistical analysis of heavy metal ion concentration was cond...

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Main Authors: Yu Han, Yuxiang Liu, Shanming Wei, Min Wang, Guantao Ding, Xiaoyu Song, Dandan Shen, Shuai Gao, Cui Tang, Guanqun Ma
Format: Article
Language:English
Published: MDPI AG 2023-09-01
Series:Water
Subjects:
Online Access:https://www.mdpi.com/2073-4441/15/19/3440
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author Yu Han
Yuxiang Liu
Shanming Wei
Min Wang
Guantao Ding
Xiaoyu Song
Dandan Shen
Shuai Gao
Cui Tang
Guanqun Ma
author_facet Yu Han
Yuxiang Liu
Shanming Wei
Min Wang
Guantao Ding
Xiaoyu Song
Dandan Shen
Shuai Gao
Cui Tang
Guanqun Ma
author_sort Yu Han
collection DOAJ
description This study investigated the hydrochemical characteristics and human health risks of groundwater in a pollution accident site. By collecting 27 samples, the content of the heavy metal(oid)s (As, Cd, Cr, Cu, Hg, Ni, Pb, and Zn) was tested, statistical analysis of heavy metal ion concentration was conducted, and the Nemerow comprehensive contamination index was determined. The health risk assessment was conducted based on the test results, and correlation analysis, as well as principal component analysis, were used to resolve the possible sources of heavy metal contamination. The results showed that the total hardness and total dissolved solids were significantly higher, and the potassium permanganate index and ammonia nitrogen content were higher in some samples. The heavy metal content was higher than the Class III groundwater quality standard (GB/T14848-2017). The health risk assessment showed that the total health risks posed by the eight heavy metal(oid)s in the study area through drinking water and dermal contact exceeded the maximum acceptable level. In general, the health risk is slightly higher for adults than for children. The groundwater in the abandoned mines has unsafe levels of heavy metal(oid)s for human health, but the normal drinking water remains safe for surrounding residents. Carcinogenic heavy metal(oid)s are the main source of health risks in the region, and the impact of Cr on human health requires further attention.
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spelling doaj.art-cd8cfcbda03e499fb99d31f571ba7b352023-11-30T20:49:58ZengMDPI AGWater2073-44412023-09-011519344010.3390/w15193440Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, ChinaYu Han0Yuxiang Liu1Shanming Wei2Min Wang3Guantao Ding4Xiaoyu Song5Dandan Shen6Shuai Gao7Cui Tang8Guanqun Ma9801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, ChinaCollege of Energy and Mining Engineering, Shandong University of Science and Technology, Qingdao 266590, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, ChinaCollege of Energy and Mining Engineering, Shandong University of Science and Technology, Qingdao 266590, ChinaShandong Transportation Institute, Jinan 250000, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, China801 Institute of Hydrogeology and Engineering Geology, Shandong Provincial Bureau of Geology & Mineral Resources, Jinan 250014, ChinaThis study investigated the hydrochemical characteristics and human health risks of groundwater in a pollution accident site. By collecting 27 samples, the content of the heavy metal(oid)s (As, Cd, Cr, Cu, Hg, Ni, Pb, and Zn) was tested, statistical analysis of heavy metal ion concentration was conducted, and the Nemerow comprehensive contamination index was determined. The health risk assessment was conducted based on the test results, and correlation analysis, as well as principal component analysis, were used to resolve the possible sources of heavy metal contamination. The results showed that the total hardness and total dissolved solids were significantly higher, and the potassium permanganate index and ammonia nitrogen content were higher in some samples. The heavy metal content was higher than the Class III groundwater quality standard (GB/T14848-2017). The health risk assessment showed that the total health risks posed by the eight heavy metal(oid)s in the study area through drinking water and dermal contact exceeded the maximum acceptable level. In general, the health risk is slightly higher for adults than for children. The groundwater in the abandoned mines has unsafe levels of heavy metal(oid)s for human health, but the normal drinking water remains safe for surrounding residents. Carcinogenic heavy metal(oid)s are the main source of health risks in the region, and the impact of Cr on human health requires further attention.https://www.mdpi.com/2073-4441/15/19/3440groundwaterhealth risk assessmentheavy metal(oid)swater quality evaluation
spellingShingle Yu Han
Yuxiang Liu
Shanming Wei
Min Wang
Guantao Ding
Xiaoyu Song
Dandan Shen
Shuai Gao
Cui Tang
Guanqun Ma
Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
Water
groundwater
health risk assessment
heavy metal(oid)s
water quality evaluation
title Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
title_full Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
title_fullStr Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
title_full_unstemmed Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
title_short Source Apportionment and Health Risk Assessment of Heavy Metals in Karst Water from Abandoned Mines in Zhangqiu, China
title_sort source apportionment and health risk assessment of heavy metals in karst water from abandoned mines in zhangqiu china
topic groundwater
health risk assessment
heavy metal(oid)s
water quality evaluation
url https://www.mdpi.com/2073-4441/15/19/3440
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