Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters
Cu, which exhibits excellent corrosion resistance in underground environments, has been investigated as a canister material for use in the deep geological disposal of spent nuclear fuels. In this study, the technical viability of atmospheric plasma spraying for producing Cu-coated canisters was inve...
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Format: | Article |
Language: | English |
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Elsevier
2023-11-01
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Series: | Nuclear Engineering and Technology |
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Online Access: | http://www.sciencedirect.com/science/article/pii/S1738573323003339 |
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author | Sung-Wook Kim Gha-Young Kim Young-Ho Lee Jun-Hyuk Jang Chung-Won Lee Jeong-Hyun Woo Seok Yoon |
author_facet | Sung-Wook Kim Gha-Young Kim Young-Ho Lee Jun-Hyuk Jang Chung-Won Lee Jeong-Hyun Woo Seok Yoon |
author_sort | Sung-Wook Kim |
collection | DOAJ |
description | Cu, which exhibits excellent corrosion resistance in underground environments, has been investigated as a canister material for use in the deep geological disposal of spent nuclear fuels. In this study, the technical viability of atmospheric plasma spraying for producing Cu-coated canisters was investigated. A high-purity Cu film (millimeter scale) was deposited onto a stainless-steel substrate using a plasma gun with a shroud structure. Potentiodynamic polarization studies revealed that the Cu film exhibited a sufficiently low corrosion rate in the groundwater electrolyte. In addition, no pitting corrosion was observed on the Cu film surface after accelerated corrosion studies. A prototype cylindrical Cu film was fabricated on a 1/20 scale on a stainless-steel tube to demonstrate the scalability of atmospheric plasma spraying in producing Cu-coated canisters. |
first_indexed | 2024-03-11T16:48:35Z |
format | Article |
id | doaj.art-ce2248d4d661423699bf592525a393bd |
institution | Directory Open Access Journal |
issn | 1738-5733 |
language | English |
last_indexed | 2024-03-11T16:48:35Z |
publishDate | 2023-11-01 |
publisher | Elsevier |
record_format | Article |
series | Nuclear Engineering and Technology |
spelling | doaj.art-ce2248d4d661423699bf592525a393bd2023-10-22T04:48:28ZengElsevierNuclear Engineering and Technology1738-57332023-11-01551140324038Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canistersSung-Wook Kim0Gha-Young Kim1Young-Ho Lee2Jun-Hyuk Jang3Chung-Won Lee4Jeong-Hyun Woo5Seok Yoon6Corresponding author.; Korea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaKorea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon, 34057, Republic of KoreaCu, which exhibits excellent corrosion resistance in underground environments, has been investigated as a canister material for use in the deep geological disposal of spent nuclear fuels. In this study, the technical viability of atmospheric plasma spraying for producing Cu-coated canisters was investigated. A high-purity Cu film (millimeter scale) was deposited onto a stainless-steel substrate using a plasma gun with a shroud structure. Potentiodynamic polarization studies revealed that the Cu film exhibited a sufficiently low corrosion rate in the groundwater electrolyte. In addition, no pitting corrosion was observed on the Cu film surface after accelerated corrosion studies. A prototype cylindrical Cu film was fabricated on a 1/20 scale on a stainless-steel tube to demonstrate the scalability of atmospheric plasma spraying in producing Cu-coated canisters.http://www.sciencedirect.com/science/article/pii/S1738573323003339Deep geological disposalCanisterCopperAdditive manufacturingAtmospheric plasma sprayingElectrochemistry |
spellingShingle | Sung-Wook Kim Gha-Young Kim Young-Ho Lee Jun-Hyuk Jang Chung-Won Lee Jeong-Hyun Woo Seok Yoon Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters Nuclear Engineering and Technology Deep geological disposal Canister Copper Additive manufacturing Atmospheric plasma spraying Electrochemistry |
title | Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters |
title_full | Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters |
title_fullStr | Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters |
title_full_unstemmed | Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters |
title_short | Electrochemical corrosion behavior of atmospheric-plasma-sprayed copper as a coating material for deep geological disposal canisters |
title_sort | electrochemical corrosion behavior of atmospheric plasma sprayed copper as a coating material for deep geological disposal canisters |
topic | Deep geological disposal Canister Copper Additive manufacturing Atmospheric plasma spraying Electrochemistry |
url | http://www.sciencedirect.com/science/article/pii/S1738573323003339 |
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