Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements

The satellite-based cloud condensation nuclei (CCN) proxies used to quantify the aerosol-cloud interactions (ACIs) are column integrated and do not guarantee the vertical co-location of aerosols and clouds. This has encouraged the use of height-resolved measurements of spaceborne lidars for ACI stud...

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Main Authors: Goutam Choudhury, Matthias Tesche
Format: Article
Language:English
Published: MDPI AG 2022-07-01
Series:Remote Sensing
Subjects:
Online Access:https://www.mdpi.com/2072-4292/14/14/3342
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author Goutam Choudhury
Matthias Tesche
author_facet Goutam Choudhury
Matthias Tesche
author_sort Goutam Choudhury
collection DOAJ
description The satellite-based cloud condensation nuclei (CCN) proxies used to quantify the aerosol-cloud interactions (ACIs) are column integrated and do not guarantee the vertical co-location of aerosols and clouds. This has encouraged the use of height-resolved measurements of spaceborne lidars for ACI studies and led to advancements in lidar-based CCN retrieval algorithms. In this study, we present a comparison between the number concentration of CCN (<i>n</i><sub>CCN</sub>) derived from ground-based in situ and spaceborne lidar cloud-aerosol lidar with orthogonal polarization (CALIOP) measurements. On analysing their monthly time series, we found that about 88% of CALIOP <i>n</i><sub>CCN</sub> estimates remained within a factor of 1.5 of the in situ measurements. Overall, the CALIOP estimates of monthly <i>n</i><sub>CCN</sub> were in good agreement with the in situ measurements with a normalized mean error of 71%, normalized mean bias of 39% and correlation coefficient of 0.68. Based on our comparison results, we point out the necessary measures that should be considered for global <i>n</i><sub>CCN</sub> retrieval. Our results show the competence of CALIOP in compiling a global height- and type-resolved <i>n</i><sub>CCN</sub> dataset for use in ACI studies.
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spelling doaj.art-ce657b4b553e4582a49b404ecc1319762023-11-30T21:48:52ZengMDPI AGRemote Sensing2072-42922022-07-011414334210.3390/rs14143342Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface MeasurementsGoutam Choudhury0Matthias Tesche1Leipzig Institute for Meteorology, Leipzig University, 04103 Leipzig, GermanyLeipzig Institute for Meteorology, Leipzig University, 04103 Leipzig, GermanyThe satellite-based cloud condensation nuclei (CCN) proxies used to quantify the aerosol-cloud interactions (ACIs) are column integrated and do not guarantee the vertical co-location of aerosols and clouds. This has encouraged the use of height-resolved measurements of spaceborne lidars for ACI studies and led to advancements in lidar-based CCN retrieval algorithms. In this study, we present a comparison between the number concentration of CCN (<i>n</i><sub>CCN</sub>) derived from ground-based in situ and spaceborne lidar cloud-aerosol lidar with orthogonal polarization (CALIOP) measurements. On analysing their monthly time series, we found that about 88% of CALIOP <i>n</i><sub>CCN</sub> estimates remained within a factor of 1.5 of the in situ measurements. Overall, the CALIOP estimates of monthly <i>n</i><sub>CCN</sub> were in good agreement with the in situ measurements with a normalized mean error of 71%, normalized mean bias of 39% and correlation coefficient of 0.68. Based on our comparison results, we point out the necessary measures that should be considered for global <i>n</i><sub>CCN</sub> retrieval. Our results show the competence of CALIOP in compiling a global height- and type-resolved <i>n</i><sub>CCN</sub> dataset for use in ACI studies.https://www.mdpi.com/2072-4292/14/14/3342CCN validationCALIPSO validationOMCAMPOLIPHONaerosol-cloud interactions
spellingShingle Goutam Choudhury
Matthias Tesche
Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
Remote Sensing
CCN validation
CALIPSO validation
OMCAM
POLIPHON
aerosol-cloud interactions
title Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
title_full Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
title_fullStr Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
title_full_unstemmed Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
title_short Assessment of CALIOP-Derived CCN Concentrations by In Situ Surface Measurements
title_sort assessment of caliop derived ccn concentrations by in situ surface measurements
topic CCN validation
CALIPSO validation
OMCAM
POLIPHON
aerosol-cloud interactions
url https://www.mdpi.com/2072-4292/14/14/3342
work_keys_str_mv AT goutamchoudhury assessmentofcaliopderivedccnconcentrationsbyinsitusurfacemeasurements
AT matthiastesche assessmentofcaliopderivedccnconcentrationsbyinsitusurfacemeasurements