Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles

The Fe-doped NiO nanoparticles that were synthesized using a co-precipitation method are characterized by enhanced room-temperature ferromagnetic property evident from magnetic measurements. Neutron powder diffraction experiments suggested an increment of the magnetic moment of 3<i>d</i>...

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Main Authors: Ashish Chhaganlal Gandhi, Tai-Yue Li, B. Vijaya Kumar, P. Muralidhar Reddy, Jen-Chih Peng, Chun-Ming Wu, Sheng Yun Wu
Format: Article
Language:English
Published: MDPI AG 2020-07-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/10/7/1318
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author Ashish Chhaganlal Gandhi
Tai-Yue Li
B. Vijaya Kumar
P. Muralidhar Reddy
Jen-Chih Peng
Chun-Ming Wu
Sheng Yun Wu
author_facet Ashish Chhaganlal Gandhi
Tai-Yue Li
B. Vijaya Kumar
P. Muralidhar Reddy
Jen-Chih Peng
Chun-Ming Wu
Sheng Yun Wu
author_sort Ashish Chhaganlal Gandhi
collection DOAJ
description The Fe-doped NiO nanoparticles that were synthesized using a co-precipitation method are characterized by enhanced room-temperature ferromagnetic property evident from magnetic measurements. Neutron powder diffraction experiments suggested an increment of the magnetic moment of 3<i>d</i> ions in the nanoparticles as a function of Fe-concentration. The temperature, time, and field-dependent magnetization measurements show that the effect of Fe-doping in NiO has enhanced the intraparticle interactions due to formed defect clusters. The intraparticle interactions are proposed to bring additional magnetic anisotropy energy barriers that affect the overall magnetic moment relaxation process and emerging as room temperature magnetic memory. The outcome of this study is attractive for the future development of the room temperature ferromagnetic oxide system to facilitate the integration of spintronic devices and understanding of their fundamental physics.
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spelling doaj.art-cf1a2ba419c14db2828aad77f87827a52023-11-20T05:51:26ZengMDPI AGNanomaterials2079-49912020-07-01107131810.3390/nano10071318Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO NanoparticlesAshish Chhaganlal Gandhi0Tai-Yue Li1B. Vijaya Kumar2P. Muralidhar Reddy3Jen-Chih Peng4Chun-Ming Wu5Sheng Yun Wu6Department of Physics, National Dong Hwa University, Hualien 97401, TaiwanDepartment of Physics, National Dong Hwa University, Hualien 97401, TaiwanDepartment of Chemistry, Nizam College, Osmania University, Hyderabad 500001, IndiaDepartment of Chemistry, University College of Science, Osmania University, Hyderabad 500007, Telangana, IndiaSIKA, National Synchrotron Radiation Research Center, Hsinchu 30076, TaiwanSIKA, National Synchrotron Radiation Research Center, Hsinchu 30076, TaiwanDepartment of Physics, National Dong Hwa University, Hualien 97401, TaiwanThe Fe-doped NiO nanoparticles that were synthesized using a co-precipitation method are characterized by enhanced room-temperature ferromagnetic property evident from magnetic measurements. Neutron powder diffraction experiments suggested an increment of the magnetic moment of 3<i>d</i> ions in the nanoparticles as a function of Fe-concentration. The temperature, time, and field-dependent magnetization measurements show that the effect of Fe-doping in NiO has enhanced the intraparticle interactions due to formed defect clusters. The intraparticle interactions are proposed to bring additional magnetic anisotropy energy barriers that affect the overall magnetic moment relaxation process and emerging as room temperature magnetic memory. The outcome of this study is attractive for the future development of the room temperature ferromagnetic oxide system to facilitate the integration of spintronic devices and understanding of their fundamental physics.https://www.mdpi.com/2079-4991/10/7/1318room temperaturemagnetic memory effectintraparticle interactions4:1 defect clusterFe-doped NiO
spellingShingle Ashish Chhaganlal Gandhi
Tai-Yue Li
B. Vijaya Kumar
P. Muralidhar Reddy
Jen-Chih Peng
Chun-Ming Wu
Sheng Yun Wu
Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
Nanomaterials
room temperature
magnetic memory effect
intraparticle interactions
4:1 defect cluster
Fe-doped NiO
title Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
title_full Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
title_fullStr Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
title_full_unstemmed Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
title_short Room Temperature Magnetic Memory Effect in Cluster-Glassy Fe-Doped NiO Nanoparticles
title_sort room temperature magnetic memory effect in cluster glassy fe doped nio nanoparticles
topic room temperature
magnetic memory effect
intraparticle interactions
4:1 defect cluster
Fe-doped NiO
url https://www.mdpi.com/2079-4991/10/7/1318
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