Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste

For the first time, tricalcium silicate (C3S) and an aqueous solution were mixed and allowed to hydrate in the microgravity environment aboard the International Space Station (ISS). The research hypothesis states that minimizing gravity-driven transport phenomena, such as buoyancy, sedimentation, an...

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Main Authors: Juliana Moraes Neves, Peter J. Collins, Ryan P. Wilkerson, Richard N. Grugel, Aleksandra Radlińska
Format: Article
Language:English
Published: Frontiers Media S.A. 2019-04-01
Series:Frontiers in Materials
Subjects:
Online Access:https://www.frontiersin.org/article/10.3389/fmats.2019.00083/full
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author Juliana Moraes Neves
Peter J. Collins
Ryan P. Wilkerson
Richard N. Grugel
Aleksandra Radlińska
author_facet Juliana Moraes Neves
Peter J. Collins
Ryan P. Wilkerson
Richard N. Grugel
Aleksandra Radlińska
author_sort Juliana Moraes Neves
collection DOAJ
description For the first time, tricalcium silicate (C3S) and an aqueous solution were mixed and allowed to hydrate in the microgravity environment aboard the International Space Station (ISS). The research hypothesis states that minimizing gravity-driven transport phenomena, such as buoyancy, sedimentation, and thermosolutal convection ensures diffusion-controlled crystal growth and, consequently, lead to unique microstructures. Results from SEM micrographs, image analysis, mercury intrusion porosimetry, thermogravimetry, and x-ray diffraction revealed that the primary differences in μg hydrated C3S paste are increased porosity and a lower aspect ratio of portlandite crystals, likely due to a more uniform phase distribution. Relevant observations led by the presence or absence of gravity, including bleeding effect, density, and crystallography are also presented and discussed.
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spelling doaj.art-cfeee56287054ff38600f4ab128d41072022-12-22T03:42:14ZengFrontiers Media S.A.Frontiers in Materials2296-80162019-04-01610.3389/fmats.2019.00083449212Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) PasteJuliana Moraes Neves0Peter J. Collins1Ryan P. Wilkerson2Richard N. Grugel3Aleksandra Radlińska4Department of Civil and Environmental Engineering, The Pennsylvania State University, University Park, PA, United StatesDepartment of Civil and Environmental Engineering, The Pennsylvania State University, University Park, PA, United StatesMarshall Space Flight Center-NASA, Huntsville, AL, United StatesMarshall Space Flight Center-NASA, Huntsville, AL, United StatesDepartment of Civil and Environmental Engineering, The Pennsylvania State University, University Park, PA, United StatesFor the first time, tricalcium silicate (C3S) and an aqueous solution were mixed and allowed to hydrate in the microgravity environment aboard the International Space Station (ISS). The research hypothesis states that minimizing gravity-driven transport phenomena, such as buoyancy, sedimentation, and thermosolutal convection ensures diffusion-controlled crystal growth and, consequently, lead to unique microstructures. Results from SEM micrographs, image analysis, mercury intrusion porosimetry, thermogravimetry, and x-ray diffraction revealed that the primary differences in μg hydrated C3S paste are increased porosity and a lower aspect ratio of portlandite crystals, likely due to a more uniform phase distribution. Relevant observations led by the presence or absence of gravity, including bleeding effect, density, and crystallography are also presented and discussed.https://www.frontiersin.org/article/10.3389/fmats.2019.00083/fullmicrogravityC3S hydrationmicrostructureporosityportlandite CHsedimentation
spellingShingle Juliana Moraes Neves
Peter J. Collins
Ryan P. Wilkerson
Richard N. Grugel
Aleksandra Radlińska
Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
Frontiers in Materials
microgravity
C3S hydration
microstructure
porosity
portlandite CH
sedimentation
title Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
title_full Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
title_fullStr Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
title_full_unstemmed Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
title_short Microgravity Effect on Microstructural Development of Tri-calcium Silicate (C3S) Paste
title_sort microgravity effect on microstructural development of tri calcium silicate c3s paste
topic microgravity
C3S hydration
microstructure
porosity
portlandite CH
sedimentation
url https://www.frontiersin.org/article/10.3389/fmats.2019.00083/full
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