In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology

After the accident at the Fukushima Dai-ichi Nuclear Power Station, a large amount of contaminated water was treated using several decontamination systems with different natures of adsorbents and chemicals. The resulting wastes, called Fukushima Effluent Treatment Wastes (FETW), were stored at the F...

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Main Authors: Vernay Aliénor, Michel Caroline, Hollebecque Jean-François, Nonnet Hélène, Fournier Maxime, Didierlaurent Régis
Format: Article
Language:English
Published: EDP Sciences 2022-01-01
Series:EPJ Nuclear Sciences & Technologies
Online Access:https://www.epj-n.org/articles/epjn/full_html/2022/01/epjn220052/epjn220052.html
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author Vernay Aliénor
Michel Caroline
Hollebecque Jean-François
Nonnet Hélène
Fournier Maxime
Didierlaurent Régis
author_facet Vernay Aliénor
Michel Caroline
Hollebecque Jean-François
Nonnet Hélène
Fournier Maxime
Didierlaurent Régis
author_sort Vernay Aliénor
collection DOAJ
description After the accident at the Fukushima Dai-ichi Nuclear Power Station, a large amount of contaminated water was treated using several decontamination systems with different natures of adsorbents and chemicals. The resulting wastes, called Fukushima Effluent Treatment Wastes (FETW), were stored at the Fukushima Dai-ichi site. Vitrification could be the most promising treatment method to package these wastes. The consortium gathering CEA, Orano, ECM Technologies and ANDRA, implemented an in situ, robust, simple and versatile In-Can vitrification process, the DEM&MELT technology. Since 2018, the applicability of this technology for FETW treatment and conditioning has been evaluated. In 2021–2022, studies focused on one particular waste, coming from the ALPS system (Advanced Liquid Processing System-Multi Radionuclides Removal) generating around 70%vol. of FETW. This waste is composed of two co-precipitation slurries: one mainly composed of iron hydroxide, and one of calcium carbonate and magnesium hydroxide. The purpose of this article is to highlight the feasibility of ALPS slurries vitrification with DEM&MELT, relying on tests performed from laboratory-scale to full-scale. Macroscopically homogeneous glasses were produced using the DEM&MELT demonstrator, with a waste loading of 60 wt.% (expressed as waste dry mass) and microstructural analyses were performed. It gives promising results for FETW conditioning with the DEM&MELT process.
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spelling doaj.art-d0495c12eeb749a1ab1d6b747a9ce4e42022-12-22T03:49:32ZengEDP SciencesEPJ Nuclear Sciences & Technologies2491-92922022-01-0183310.1051/epjn/2022045epjn220052In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technologyVernay Aliénor0https://orcid.org/0000-0002-6442-6719Michel Caroline1Hollebecque Jean-François2Nonnet Hélène3Fournier Maxime4Didierlaurent Régis5CEA, DES, ISEC, DE2D, Univ. MontpellierCEA, DES, ISEC, DE2D, Univ. MontpellierCEA, DES, ISEC, DE2D, Univ. MontpellierCEA, DES, ISEC, DE2D, Univ. MontpellierCEA, DES, ISEC, DE2D, Univ. MontpellierOrano RecyclageAfter the accident at the Fukushima Dai-ichi Nuclear Power Station, a large amount of contaminated water was treated using several decontamination systems with different natures of adsorbents and chemicals. The resulting wastes, called Fukushima Effluent Treatment Wastes (FETW), were stored at the Fukushima Dai-ichi site. Vitrification could be the most promising treatment method to package these wastes. The consortium gathering CEA, Orano, ECM Technologies and ANDRA, implemented an in situ, robust, simple and versatile In-Can vitrification process, the DEM&MELT technology. Since 2018, the applicability of this technology for FETW treatment and conditioning has been evaluated. In 2021–2022, studies focused on one particular waste, coming from the ALPS system (Advanced Liquid Processing System-Multi Radionuclides Removal) generating around 70%vol. of FETW. This waste is composed of two co-precipitation slurries: one mainly composed of iron hydroxide, and one of calcium carbonate and magnesium hydroxide. The purpose of this article is to highlight the feasibility of ALPS slurries vitrification with DEM&MELT, relying on tests performed from laboratory-scale to full-scale. Macroscopically homogeneous glasses were produced using the DEM&MELT demonstrator, with a waste loading of 60 wt.% (expressed as waste dry mass) and microstructural analyses were performed. It gives promising results for FETW conditioning with the DEM&MELT process.https://www.epj-n.org/articles/epjn/full_html/2022/01/epjn220052/epjn220052.html
spellingShingle Vernay Aliénor
Michel Caroline
Hollebecque Jean-François
Nonnet Hélène
Fournier Maxime
Didierlaurent Régis
In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
EPJ Nuclear Sciences & Technologies
title In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
title_full In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
title_fullStr In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
title_full_unstemmed In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
title_short In-Can vitrification of ALPS slurries from Fukushima Daiichi effluent treatment using DEM&MELT technology
title_sort in can vitrification of alps slurries from fukushima daiichi effluent treatment using dem melt technology
url https://www.epj-n.org/articles/epjn/full_html/2022/01/epjn220052/epjn220052.html
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