Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties

Laboratory measurements using nuclear magnetic resonance, scanning electron microscopy, and gas porosity and permeability analysis were conducted to acquire a petrophysical interpretation of the Carbon Tan Sandstone and Savonnieres Carbonate for potential carbon dioxide storage in subsurface formati...

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Main Authors: Hisham Ben Mahmud, Mohamed Khalifa, Mian Shafiq, Ausama Giwelli
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2023-09-01
Series:Petroleum Research
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2096249522000710
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author Hisham Ben Mahmud
Mohamed Khalifa
Mian Shafiq
Ausama Giwelli
author_facet Hisham Ben Mahmud
Mohamed Khalifa
Mian Shafiq
Ausama Giwelli
author_sort Hisham Ben Mahmud
collection DOAJ
description Laboratory measurements using nuclear magnetic resonance, scanning electron microscopy, and gas porosity and permeability analysis were conducted to acquire a petrophysical interpretation of the Carbon Tan Sandstone and Savonnieres Carbonate for potential carbon dioxide storage in subsurface formations. The relationships between pore structures, such as pore-size distribution, pore geometry, and porosity/permeability, were investigated near and far from the wellbore. At operating pressures of 2500psi (17.24 MPa) and temperatures of 176 °F (50 °C), carbonated water was injected into a composite core constructed of two similar core samples bounded by a compact disc located between them. The current results showed that a strong calcite dissolution took place near the injection position of both rock samples and led to improvements in the primary intergranular permeability and porosity, while the carbonate sample showed significant improvement compared to sandstone. The durable heterogeneous dissolution of calcite grains also led to the creation of new pores as intra-granular micro-pores. While at deeper depths from the injection position, it noticed an insignificant development in pore structure and its populations as well as rock hydraulic properties of both rock samples. In conclusion, the study revealed that the injected carbonated brine had a valuable impact on fluid-formation interactive, which improved rock's inlet properties compared with outlet.
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spelling doaj.art-d0914b0df4ee4d7bb910b3453e6e1bd02023-09-28T05:25:43ZengKeAi Communications Co., Ltd.Petroleum Research2096-24952023-09-0183316323Experimental investigation of the influence of carbonated water on sandstone and carbonate rock propertiesHisham Ben Mahmud0Mohamed Khalifa1Mian Shafiq2Ausama Giwelli3Department of Chemical and Energy Engineering, Curtin University Malaysia, Faculty of Engineering and Science, Miri, 98009, Sarawak, Malaysia; Energy and Environmental Research Cluster, Faculty of Engineering and Science, Curtin University Malaysia, Sarawak, 98009, Malaysia; Corresponding author. Department of Chemical and Energy Engineering, Curtin University Malaysia, Faculty of Engineering and Science, Miri, 98009, Sarawak, Malaysia.Department of Earth Sciences, School of Basic Sciences, Libyan Academy of Postgraduate Studies, PO Box, 79031, Janzour, LibyaDepartment of Chemical and Petroleum Engineering, UCSI University, 56000, MalaysiaAustralian Resources Research Centre, CSIRO, Kensington, AustraliaLaboratory measurements using nuclear magnetic resonance, scanning electron microscopy, and gas porosity and permeability analysis were conducted to acquire a petrophysical interpretation of the Carbon Tan Sandstone and Savonnieres Carbonate for potential carbon dioxide storage in subsurface formations. The relationships between pore structures, such as pore-size distribution, pore geometry, and porosity/permeability, were investigated near and far from the wellbore. At operating pressures of 2500psi (17.24 MPa) and temperatures of 176 °F (50 °C), carbonated water was injected into a composite core constructed of two similar core samples bounded by a compact disc located between them. The current results showed that a strong calcite dissolution took place near the injection position of both rock samples and led to improvements in the primary intergranular permeability and porosity, while the carbonate sample showed significant improvement compared to sandstone. The durable heterogeneous dissolution of calcite grains also led to the creation of new pores as intra-granular micro-pores. While at deeper depths from the injection position, it noticed an insignificant development in pore structure and its populations as well as rock hydraulic properties of both rock samples. In conclusion, the study revealed that the injected carbonated brine had a valuable impact on fluid-formation interactive, which improved rock's inlet properties compared with outlet.http://www.sciencedirect.com/science/article/pii/S2096249522000710CO2–brine injectionFluid-carbonate/sandstone interactionPetrophysical propertiesPore structureNMRSEM analysis
spellingShingle Hisham Ben Mahmud
Mohamed Khalifa
Mian Shafiq
Ausama Giwelli
Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
Petroleum Research
CO2–brine injection
Fluid-carbonate/sandstone interaction
Petrophysical properties
Pore structure
NMR
SEM analysis
title Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
title_full Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
title_fullStr Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
title_full_unstemmed Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
title_short Experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
title_sort experimental investigation of the influence of carbonated water on sandstone and carbonate rock properties
topic CO2–brine injection
Fluid-carbonate/sandstone interaction
Petrophysical properties
Pore structure
NMR
SEM analysis
url http://www.sciencedirect.com/science/article/pii/S2096249522000710
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AT mohamedkhalifa experimentalinvestigationoftheinfluenceofcarbonatedwateronsandstoneandcarbonaterockproperties
AT mianshafiq experimentalinvestigationoftheinfluenceofcarbonatedwateronsandstoneandcarbonaterockproperties
AT ausamagiwelli experimentalinvestigationoftheinfluenceofcarbonatedwateronsandstoneandcarbonaterockproperties