Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals
Two-photon absorption has been systematically studied in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> crystals, both of which are prospective nonlinear o...
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2023-04-01
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author | Igor O. Kinyaevskiy Valery I. Kovalev Nikita S. Semin Pavel A. Danilov Sergey I. Kudryashov Andrey V. Koribut Elizaveta E. Dunaeva |
author_facet | Igor O. Kinyaevskiy Valery I. Kovalev Nikita S. Semin Pavel A. Danilov Sergey I. Kudryashov Andrey V. Koribut Elizaveta E. Dunaeva |
author_sort | Igor O. Kinyaevskiy |
collection | DOAJ |
description | Two-photon absorption has been systematically studied in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> crystals, both of which are prospective nonlinear optical and laser host materials. A strong dependence of the two-photon absorption coefficients on the orientation of the laser beam polarization with respect to the optical c-axis of the crystals is revealed. The measured coefficients for perpendicular and parallel orientations were 50 ± 10 cm/TW and 19 ± 4 cm/TW in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub>, and 18 ± 3 cm/TW and 10 ± 2 cm/TW in Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub>, respectively. Thus, to minimize optical losses caused by two-photon absorption, an orientation of Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> crystals with the laser beam polarization parallel to the crystal optical c-axis is preferred. |
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spelling | doaj.art-d0aafd0e5e314abdad640e7ecf77f01f2023-11-17T20:58:28ZengMDPI AGPhotonics2304-67322023-04-0110446610.3390/photonics10040466Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> CrystalsIgor O. Kinyaevskiy0Valery I. Kovalev1Nikita S. Semin2Pavel A. Danilov3Sergey I. Kudryashov4Andrey V. Koribut5Elizaveta E. Dunaeva6P.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaP.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaP.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaP.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaP.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaP.N. Lebedev Physical Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaProkhorov General Physics Institute of the Russian Academy of Sciences, 119991 Moscow, RussiaTwo-photon absorption has been systematically studied in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> crystals, both of which are prospective nonlinear optical and laser host materials. A strong dependence of the two-photon absorption coefficients on the orientation of the laser beam polarization with respect to the optical c-axis of the crystals is revealed. The measured coefficients for perpendicular and parallel orientations were 50 ± 10 cm/TW and 19 ± 4 cm/TW in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub>, and 18 ± 3 cm/TW and 10 ± 2 cm/TW in Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub>, respectively. Thus, to minimize optical losses caused by two-photon absorption, an orientation of Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> crystals with the laser beam polarization parallel to the crystal optical c-axis is preferred.https://www.mdpi.com/2304-6732/10/4/466two-photon absorptioncalcium orthovanadateCa<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub>Ca<sub>3-x</sub>Sr<sub>x</sub>(VO<sub>4</sub>)<sub>2</sub>orientation effects |
spellingShingle | Igor O. Kinyaevskiy Valery I. Kovalev Nikita S. Semin Pavel A. Danilov Sergey I. Kudryashov Andrey V. Koribut Elizaveta E. Dunaeva Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals Photonics two-photon absorption calcium orthovanadate Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> Ca<sub>3-x</sub>Sr<sub>x</sub>(VO<sub>4</sub>)<sub>2</sub> orientation effects |
title | Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals |
title_full | Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals |
title_fullStr | Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals |
title_full_unstemmed | Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals |
title_short | Two-Photon Absorption in Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> and Ca<sub>2.7</sub>Sr<sub>0.3</sub>(VO<sub>4</sub>)<sub>2</sub> Crystals |
title_sort | two photon absorption in ca sub 3 sub vo sub 4 sub sub 2 sub and ca sub 2 7 sub sr sub 0 3 sub vo sub 4 sub sub 2 sub crystals |
topic | two-photon absorption calcium orthovanadate Ca<sub>3</sub>(VO<sub>4</sub>)<sub>2</sub> Ca<sub>3-x</sub>Sr<sub>x</sub>(VO<sub>4</sub>)<sub>2</sub> orientation effects |
url | https://www.mdpi.com/2304-6732/10/4/466 |
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