Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films

Abstract The rapid development of 2D magnetic materials has opened new possibilities in the field of spintronics. CrTe2, a 2D material with perpendicular magnetic anisotropy (PMA) and ferromagnetic transient temperature near room temperature, holds promise for various applications. However, the unde...

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Main Authors: Jin Wang, Yongkang Xu, Shuanghai Wang, Xingze Dai, Pengfei Yan, Jian Zhou, Ruifeng Wang, Yongbing Xu, Liang He
Format: Article
Language:English
Published: Wiley-VCH 2024-01-01
Series:Advanced Electronic Materials
Subjects:
Online Access:https://doi.org/10.1002/aelm.202300646
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author Jin Wang
Yongkang Xu
Shuanghai Wang
Xingze Dai
Pengfei Yan
Jian Zhou
Ruifeng Wang
Yongbing Xu
Liang He
author_facet Jin Wang
Yongkang Xu
Shuanghai Wang
Xingze Dai
Pengfei Yan
Jian Zhou
Ruifeng Wang
Yongbing Xu
Liang He
author_sort Jin Wang
collection DOAJ
description Abstract The rapid development of 2D magnetic materials has opened new possibilities in the field of spintronics. CrTe2, a 2D material with perpendicular magnetic anisotropy (PMA) and ferromagnetic transient temperature near room temperature, holds promise for various applications. However, the underlying mechanism responsible for its global magnetism remains unclear. This work focuses on investigating the magneto‐transport properties of ultra‐thin CrTe2 Field Effect Transistor (FET) under the influence of top gate biases. The application of gate voltage ranging from 25 to −15 V tunes its coercivity (HC) and Curie temperature (TC) (from 152 to 191 K). Notably, a linear correlation is observed between the TC and the hole concentration (np1/3) in the CrTe2 film, indicating the involvement of the Ruderman–Kittel–Kasuya–Yosida interaction. This experimental analysis sheds light on the mechanism of the CrTe2’s ferromagnetism and paves the way for future advancements and applications in this material.
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spelling doaj.art-d1528d87d3ab44cab03a53ab504bb1282024-01-10T06:50:59ZengWiley-VCHAdvanced Electronic Materials2199-160X2024-01-01101n/an/a10.1002/aelm.202300646Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin FilmsJin Wang0Yongkang Xu1Shuanghai Wang2Xingze Dai3Pengfei Yan4Jian Zhou5Ruifeng Wang6Yongbing Xu7Liang He8State Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaState Key Laboratory of Spintronics Devices and Technologies School of Electronic Science and Engineering Nanjing University Nanjing 210023 ChinaAbstract The rapid development of 2D magnetic materials has opened new possibilities in the field of spintronics. CrTe2, a 2D material with perpendicular magnetic anisotropy (PMA) and ferromagnetic transient temperature near room temperature, holds promise for various applications. However, the underlying mechanism responsible for its global magnetism remains unclear. This work focuses on investigating the magneto‐transport properties of ultra‐thin CrTe2 Field Effect Transistor (FET) under the influence of top gate biases. The application of gate voltage ranging from 25 to −15 V tunes its coercivity (HC) and Curie temperature (TC) (from 152 to 191 K). Notably, a linear correlation is observed between the TC and the hole concentration (np1/3) in the CrTe2 film, indicating the involvement of the Ruderman–Kittel–Kasuya–Yosida interaction. This experimental analysis sheds light on the mechanism of the CrTe2’s ferromagnetism and paves the way for future advancements and applications in this material.https://doi.org/10.1002/aelm.202300646CrTe2curie temperaturegate‐voltageRKKY interaction
spellingShingle Jin Wang
Yongkang Xu
Shuanghai Wang
Xingze Dai
Pengfei Yan
Jian Zhou
Ruifeng Wang
Yongbing Xu
Liang He
Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
Advanced Electronic Materials
CrTe2
curie temperature
gate‐voltage
RKKY interaction
title Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
title_full Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
title_fullStr Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
title_full_unstemmed Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
title_short Hole‐Mediated RKKY Interaction in 2D Ferromagnetic CrTe2 Ultra‐Thin Films
title_sort hole mediated rkky interaction in 2d ferromagnetic crte2 ultra thin films
topic CrTe2
curie temperature
gate‐voltage
RKKY interaction
url https://doi.org/10.1002/aelm.202300646
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AT shuanghaiwang holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT xingzedai holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT pengfeiyan holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT jianzhou holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT ruifengwang holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT yongbingxu holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms
AT lianghe holemediatedrkkyinteractionin2dferromagneticcrte2ultrathinfilms