Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor

Understanding the dynamics of a quantum bit’s environment is essential for the realization of practical systems for quantum information processing and metrology. We use single nitrogen-vacancy (NV) centers in diamond to study the dynamics of a disordered spin ensemble at the diamond surface. Specifi...

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Main Authors: Bo L. Dwyer, Lila V.H. Rodgers, Elana K. Urbach, Dolev Bluvstein, Sorawis Sangtawesin, Hengyun Zhou, Yahia Nassab, Mattias Fitzpatrick, Zhiyang Yuan, Kristiaan De Greve, Eric L. Peterson, Helena Knowles, Tamara Sumarac, Jyh-Pin Chou, Adam Gali, V.V. Dobrovitski, Mikhail D. Lukin, Nathalie P. de Leon
Format: Article
Language:English
Published: American Physical Society 2022-12-01
Series:PRX Quantum
Online Access:http://doi.org/10.1103/PRXQuantum.3.040328
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author Bo L. Dwyer
Lila V.H. Rodgers
Elana K. Urbach
Dolev Bluvstein
Sorawis Sangtawesin
Hengyun Zhou
Yahia Nassab
Mattias Fitzpatrick
Zhiyang Yuan
Kristiaan De Greve
Eric L. Peterson
Helena Knowles
Tamara Sumarac
Jyh-Pin Chou
Adam Gali
V.V. Dobrovitski
Mikhail D. Lukin
Nathalie P. de Leon
author_facet Bo L. Dwyer
Lila V.H. Rodgers
Elana K. Urbach
Dolev Bluvstein
Sorawis Sangtawesin
Hengyun Zhou
Yahia Nassab
Mattias Fitzpatrick
Zhiyang Yuan
Kristiaan De Greve
Eric L. Peterson
Helena Knowles
Tamara Sumarac
Jyh-Pin Chou
Adam Gali
V.V. Dobrovitski
Mikhail D. Lukin
Nathalie P. de Leon
author_sort Bo L. Dwyer
collection DOAJ
description Understanding the dynamics of a quantum bit’s environment is essential for the realization of practical systems for quantum information processing and metrology. We use single nitrogen-vacancy (NV) centers in diamond to study the dynamics of a disordered spin ensemble at the diamond surface. Specifically, we reduce the density of “dark” surface spins to interrogate their contribution to the decoherence of shallow NV center spin qubits. When the average surface spin spacing exceeds the NV center depth, we find that the surface spin contribution to the NV center free induction decay can be described by a stretched exponential with variable power n. We show that these observations are consistent with a model in which the spatial positions of the surface spins are fixed for each measurement, but some of them reconfigure between measurements. In particular, we observe a depth-dependent critical time associated with a dynamical transition from Gaussian (n=2) decay to n=2/3, and show that this transition arises from the competition between the small decay contributions of many distant spins and strong coupling to a few proximal spins at the surface. These observations demonstrate the potential of a local sensor for understanding complex systems and elucidate pathways for improving and controlling spin qubits at the surface.
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spelling doaj.art-d253cb825abd4820a1327efe965ce3782022-12-22T03:00:10ZengAmerican Physical SocietyPRX Quantum2691-33992022-12-013404032810.1103/PRXQuantum.3.040328Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum SensorBo L. DwyerLila V.H. RodgersElana K. UrbachDolev BluvsteinSorawis SangtawesinHengyun ZhouYahia NassabMattias FitzpatrickZhiyang YuanKristiaan De GreveEric L. PetersonHelena KnowlesTamara SumaracJyh-Pin ChouAdam GaliV.V. DobrovitskiMikhail D. LukinNathalie P. de LeonUnderstanding the dynamics of a quantum bit’s environment is essential for the realization of practical systems for quantum information processing and metrology. We use single nitrogen-vacancy (NV) centers in diamond to study the dynamics of a disordered spin ensemble at the diamond surface. Specifically, we reduce the density of “dark” surface spins to interrogate their contribution to the decoherence of shallow NV center spin qubits. When the average surface spin spacing exceeds the NV center depth, we find that the surface spin contribution to the NV center free induction decay can be described by a stretched exponential with variable power n. We show that these observations are consistent with a model in which the spatial positions of the surface spins are fixed for each measurement, but some of them reconfigure between measurements. In particular, we observe a depth-dependent critical time associated with a dynamical transition from Gaussian (n=2) decay to n=2/3, and show that this transition arises from the competition between the small decay contributions of many distant spins and strong coupling to a few proximal spins at the surface. These observations demonstrate the potential of a local sensor for understanding complex systems and elucidate pathways for improving and controlling spin qubits at the surface.http://doi.org/10.1103/PRXQuantum.3.040328
spellingShingle Bo L. Dwyer
Lila V.H. Rodgers
Elana K. Urbach
Dolev Bluvstein
Sorawis Sangtawesin
Hengyun Zhou
Yahia Nassab
Mattias Fitzpatrick
Zhiyang Yuan
Kristiaan De Greve
Eric L. Peterson
Helena Knowles
Tamara Sumarac
Jyh-Pin Chou
Adam Gali
V.V. Dobrovitski
Mikhail D. Lukin
Nathalie P. de Leon
Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
PRX Quantum
title Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
title_full Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
title_fullStr Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
title_full_unstemmed Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
title_short Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
title_sort probing spin dynamics on diamond surfaces using a single quantum sensor
url http://doi.org/10.1103/PRXQuantum.3.040328
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