Stratospheric ozone in the post-CFC era

Vertical and latitudinal changes in the stratospheric ozone in the post-chlorofluorocarbon (CFC) era are investigated using simulations of the recent past and the 21st century with a coupled chemistry-climate model. Model results reveal that, in the 2060s when the stratospheric halogen loading is pr...

Full description

Bibliographic Details
Main Authors: F. Li, R. S. Stolarski, P. A. Newman
Format: Article
Language:English
Published: Copernicus Publications 2009-03-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/9/2207/2009/acp-9-2207-2009.pdf
_version_ 1818002274742435840
author F. Li
R. S. Stolarski
P. A. Newman
author_facet F. Li
R. S. Stolarski
P. A. Newman
author_sort F. Li
collection DOAJ
description Vertical and latitudinal changes in the stratospheric ozone in the post-chlorofluorocarbon (CFC) era are investigated using simulations of the recent past and the 21st century with a coupled chemistry-climate model. Model results reveal that, in the 2060s when the stratospheric halogen loading is projected to return to its 1980 values, the extratropical column ozone is significantly higher than that in 1975–1984, but the tropical column ozone does not recover to 1980 values. Upper and lower stratospheric ozone changes in the post-CFC era have very different patterns. Above 15 hPa ozone increases almost latitudinally uniformly by 6 Dobson Unit (DU), whereas below 15 hPa ozone decreases in the tropics by 8 DU and increases in the extratropics by up to 16 DU. The upper stratospheric ozone increase is a photochemical response to greenhouse gas induced strong cooling, and the lower stratospheric ozone changes are consistent with enhanced mean advective transport due to a stronger Brewer-Dobson circulation. The model results suggest that the strengthening of the Brewer-Dobson circulation plays a crucial role in ozone recovery and ozone distributions in the post-CFC era.
first_indexed 2024-04-14T03:44:34Z
format Article
id doaj.art-d2ea32f1d34947c8b6f93725c92ff870
institution Directory Open Access Journal
issn 1680-7316
1680-7324
language English
last_indexed 2024-04-14T03:44:34Z
publishDate 2009-03-01
publisher Copernicus Publications
record_format Article
series Atmospheric Chemistry and Physics
spelling doaj.art-d2ea32f1d34947c8b6f93725c92ff8702022-12-22T02:14:22ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242009-03-019622072213Stratospheric ozone in the post-CFC eraF. LiR. S. StolarskiP. A. NewmanVertical and latitudinal changes in the stratospheric ozone in the post-chlorofluorocarbon (CFC) era are investigated using simulations of the recent past and the 21st century with a coupled chemistry-climate model. Model results reveal that, in the 2060s when the stratospheric halogen loading is projected to return to its 1980 values, the extratropical column ozone is significantly higher than that in 1975–1984, but the tropical column ozone does not recover to 1980 values. Upper and lower stratospheric ozone changes in the post-CFC era have very different patterns. Above 15 hPa ozone increases almost latitudinally uniformly by 6 Dobson Unit (DU), whereas below 15 hPa ozone decreases in the tropics by 8 DU and increases in the extratropics by up to 16 DU. The upper stratospheric ozone increase is a photochemical response to greenhouse gas induced strong cooling, and the lower stratospheric ozone changes are consistent with enhanced mean advective transport due to a stronger Brewer-Dobson circulation. The model results suggest that the strengthening of the Brewer-Dobson circulation plays a crucial role in ozone recovery and ozone distributions in the post-CFC era.http://www.atmos-chem-phys.net/9/2207/2009/acp-9-2207-2009.pdf
spellingShingle F. Li
R. S. Stolarski
P. A. Newman
Stratospheric ozone in the post-CFC era
Atmospheric Chemistry and Physics
title Stratospheric ozone in the post-CFC era
title_full Stratospheric ozone in the post-CFC era
title_fullStr Stratospheric ozone in the post-CFC era
title_full_unstemmed Stratospheric ozone in the post-CFC era
title_short Stratospheric ozone in the post-CFC era
title_sort stratospheric ozone in the post cfc era
url http://www.atmos-chem-phys.net/9/2207/2009/acp-9-2207-2009.pdf
work_keys_str_mv AT fli stratosphericozoneinthepostcfcera
AT rsstolarski stratosphericozoneinthepostcfcera
AT panewman stratosphericozoneinthepostcfcera