Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy

We investigate the quantum confinement effects on excitons in several types of strain-free GaAs/Al<inline-formula> <math display="inline"> <semantics> <msub> <mrow></mrow> <mrow> <mn>0.3</mn> </mrow> </msub> </semantics&g...

Full description

Bibliographic Details
Main Authors: Inah Yeo, Doukyun Kim, Kyu-Tae Lee, Jong Su Kim, Jin Dong Song, Chul-Hong Park, Il Ki Han
Format: Article
Language:English
Published: MDPI AG 2020-07-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/10/7/1301
_version_ 1827713794523004928
author Inah Yeo
Doukyun Kim
Kyu-Tae Lee
Jong Su Kim
Jin Dong Song
Chul-Hong Park
Il Ki Han
author_facet Inah Yeo
Doukyun Kim
Kyu-Tae Lee
Jong Su Kim
Jin Dong Song
Chul-Hong Park
Il Ki Han
author_sort Inah Yeo
collection DOAJ
description We investigate the quantum confinement effects on excitons in several types of strain-free GaAs/Al<inline-formula> <math display="inline"> <semantics> <msub> <mrow></mrow> <mrow> <mn>0.3</mn> </mrow> </msub> </semantics> </math> </inline-formula>Ga<inline-formula> <math display="inline"> <semantics> <msub> <mrow></mrow> <mrow> <mn>0.7</mn> </mrow> </msub> </semantics> </math> </inline-formula>As droplet epitaxy (DE) quantum dots (QDs). By performing comparative analyses of energy-dispersive X-ray spectroscopy with the aid of a three-dimensional (3D) envelope-function model, we elucidate the individual quantum confinement characteristics of the QD band structures with respect to their composition profiles and the asymmetries of their geometrical shapes. By precisely controlling the exciton oscillator strength in strain-free QDs, we envisage the possibility of tailoring light-matter interactions to implement fully integrated quantum photonics based on QD single-photon sources (SPSs).
first_indexed 2024-03-10T18:43:00Z
format Article
id doaj.art-d30db3ecea1748e8823a3f25a199dd50
institution Directory Open Access Journal
issn 2079-4991
language English
last_indexed 2024-03-10T18:43:00Z
publishDate 2020-07-01
publisher MDPI AG
record_format Article
series Nanomaterials
spelling doaj.art-d30db3ecea1748e8823a3f25a199dd502023-11-20T05:42:47ZengMDPI AGNanomaterials2079-49912020-07-01107130110.3390/nano10071301Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet EpitaxyInah Yeo0Doukyun Kim1Kyu-Tae Lee2Jong Su Kim3Jin Dong Song4Chul-Hong Park5Il Ki Han6Dielectrics and Advanced Matter Physics Research Center, Pusan National University, Busan 46241, KoreaDielectrics and Advanced Matter Physics Research Center, Pusan National University, Busan 46241, KoreaNanophotonics Research Center, Korea Institute of Science and Technology, Seoul 02792, KoreaDepartment of Physics, Yeungnam University, Gyeonsan 38541, KoreaPost-Silicon Semiconductor Institute, Korea Institute of Science and Technology, Seoul 02792, KoreaDielectrics and Advanced Matter Physics Research Center, Pusan National University, Busan 46241, KoreaNanophotonics Research Center, Korea Institute of Science and Technology, Seoul 02792, KoreaWe investigate the quantum confinement effects on excitons in several types of strain-free GaAs/Al<inline-formula> <math display="inline"> <semantics> <msub> <mrow></mrow> <mrow> <mn>0.3</mn> </mrow> </msub> </semantics> </math> </inline-formula>Ga<inline-formula> <math display="inline"> <semantics> <msub> <mrow></mrow> <mrow> <mn>0.7</mn> </mrow> </msub> </semantics> </math> </inline-formula>As droplet epitaxy (DE) quantum dots (QDs). By performing comparative analyses of energy-dispersive X-ray spectroscopy with the aid of a three-dimensional (3D) envelope-function model, we elucidate the individual quantum confinement characteristics of the QD band structures with respect to their composition profiles and the asymmetries of their geometrical shapes. By precisely controlling the exciton oscillator strength in strain-free QDs, we envisage the possibility of tailoring light-matter interactions to implement fully integrated quantum photonics based on QD single-photon sources (SPSs).https://www.mdpi.com/2079-4991/10/7/1301droplet epitaxystrain-free quantum dotTEM-EDS
spellingShingle Inah Yeo
Doukyun Kim
Kyu-Tae Lee
Jong Su Kim
Jin Dong Song
Chul-Hong Park
Il Ki Han
Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
Nanomaterials
droplet epitaxy
strain-free quantum dot
TEM-EDS
title Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
title_full Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
title_fullStr Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
title_full_unstemmed Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
title_short Comparative Chemico-Physical Analyses of Strain-Free GaAs/Al<sub>0.3</sub>Ga<sub>0.7</sub>As Quantum Dots Grown by Droplet Epitaxy
title_sort comparative chemico physical analyses of strain free gaas al sub 0 3 sub ga sub 0 7 sub as quantum dots grown by droplet epitaxy
topic droplet epitaxy
strain-free quantum dot
TEM-EDS
url https://www.mdpi.com/2079-4991/10/7/1301
work_keys_str_mv AT inahyeo comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT doukyunkim comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT kyutaelee comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT jongsukim comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT jindongsong comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT chulhongpark comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy
AT ilkihan comparativechemicophysicalanalysesofstrainfreegaasalsub03subgasub07subasquantumdotsgrownbydropletepitaxy