Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons

In this work we present an extensive experimental and theoretical investigation of different regimes of strong field light–matter interaction for cavity-driven quantum dot (QD) cavity systems. The electric field enhancement inside a high-Q micropillar cavity facilitates exceptionally strong interact...

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Main Authors: F Hargart, K Roy-Choudhury, T John, S L Portalupi, C Schneider, S Höfling, M Kamp, S Hughes, P Michler
Format: Article
Language:English
Published: IOP Publishing 2016-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/aa5198
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author F Hargart
K Roy-Choudhury
T John
S L Portalupi
C Schneider
S Höfling
M Kamp
S Hughes
P Michler
author_facet F Hargart
K Roy-Choudhury
T John
S L Portalupi
C Schneider
S Höfling
M Kamp
S Hughes
P Michler
author_sort F Hargart
collection DOAJ
description In this work we present an extensive experimental and theoretical investigation of different regimes of strong field light–matter interaction for cavity-driven quantum dot (QD) cavity systems. The electric field enhancement inside a high-Q micropillar cavity facilitates exceptionally strong interaction with few cavity photons, enabling the simultaneous investigation for a wide range of QD-laser detuning. In case of a resonant drive, the formation of dressed states and a Mollow triplet sideband splitting of up to 45 μ eV is measured for a mean cavity photon number $\langle {n}_{c}\rangle \leqslant 1$ . In the asymptotic limit of the linear AC Stark effect we systematically investigate the power and detuning dependence of more than 400 QDs. Some QD-cavity systems exhibit an unexpected anomalous Stark shift, which can be explained by an extended dressed 4-level QD model. We provide a detailed analysis of the QD-cavity systems properties enabling this novel effect. The experimental results are successfully reproduced using a polaron master equation approach for the QD-cavity system, which includes the driving laser field, exciton-cavity and exciton-phonon interactions.
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spelling doaj.art-d373a16b0e894d07a103ad93e0a2f22c2023-08-08T14:34:26ZengIOP PublishingNew Journal of Physics1367-26302016-01-01181212303110.1088/1367-2630/aa5198Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photonsF Hargart0K Roy-Choudhury1T John2S L Portalupi3C Schneider4S Höfling5M Kamp6S Hughes7P Michler8Institut für Halbleiteroptik und Funktionelle Grenzflächen, Center for Integrated Quantum Science and Technology ( IQ ST ) and SCoPE, Universität Stuttgart , Allmandring 3, D-70569 Stuttgart, GermanyDepartment of Physics, Engineering Physics and Astronomy, Queen’s University , Kingston, Ontario, K7L 3N6, CanadaInstitut für Halbleiteroptik und Funktionelle Grenzflächen, Center for Integrated Quantum Science and Technology ( IQ ST ) and SCoPE, Universität Stuttgart , Allmandring 3, D-70569 Stuttgart, GermanyInstitut für Halbleiteroptik und Funktionelle Grenzflächen, Center for Integrated Quantum Science and Technology ( IQ ST ) and SCoPE, Universität Stuttgart , Allmandring 3, D-70569 Stuttgart, GermanyTechnische Physik and Wilhelm Conrad Röntgen Research Center for Complex Material Systems, Physikalisches Institut, Universität Würzburg , Am Hubland, D-97074 Würzburg, GermanyTechnische Physik and Wilhelm Conrad Röntgen Research Center for Complex Material Systems, Physikalisches Institut, Universität Würzburg , Am Hubland, D-97074 Würzburg, Germany; SUPA, School of Physics and Astronomy, University of St. Andrews , St. Andrews KY16 9SS, UKTechnische Physik and Wilhelm Conrad Röntgen Research Center for Complex Material Systems, Physikalisches Institut, Universität Würzburg , Am Hubland, D-97074 Würzburg, GermanyDepartment of Physics, Engineering Physics and Astronomy, Queen’s University , Kingston, Ontario, K7L 3N6, CanadaInstitut für Halbleiteroptik und Funktionelle Grenzflächen, Center for Integrated Quantum Science and Technology ( IQ ST ) and SCoPE, Universität Stuttgart , Allmandring 3, D-70569 Stuttgart, GermanyIn this work we present an extensive experimental and theoretical investigation of different regimes of strong field light–matter interaction for cavity-driven quantum dot (QD) cavity systems. The electric field enhancement inside a high-Q micropillar cavity facilitates exceptionally strong interaction with few cavity photons, enabling the simultaneous investigation for a wide range of QD-laser detuning. In case of a resonant drive, the formation of dressed states and a Mollow triplet sideband splitting of up to 45 μ eV is measured for a mean cavity photon number $\langle {n}_{c}\rangle \leqslant 1$ . In the asymptotic limit of the linear AC Stark effect we systematically investigate the power and detuning dependence of more than 400 QDs. Some QD-cavity systems exhibit an unexpected anomalous Stark shift, which can be explained by an extended dressed 4-level QD model. We provide a detailed analysis of the QD-cavity systems properties enabling this novel effect. The experimental results are successfully reproduced using a polaron master equation approach for the QD-cavity system, which includes the driving laser field, exciton-cavity and exciton-phonon interactions.https://doi.org/10.1088/1367-2630/aa5198quantum dotslight–matter interactionAC Stark effectdressed states78.67.Hc42.50.Hz
spellingShingle F Hargart
K Roy-Choudhury
T John
S L Portalupi
C Schneider
S Höfling
M Kamp
S Hughes
P Michler
Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
New Journal of Physics
quantum dots
light–matter interaction
AC Stark effect
dressed states
78.67.Hc
42.50.Hz
title Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
title_full Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
title_fullStr Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
title_full_unstemmed Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
title_short Probing different regimes of strong field light–matter interaction with semiconductor quantum dots and few cavity photons
title_sort probing different regimes of strong field light matter interaction with semiconductor quantum dots and few cavity photons
topic quantum dots
light–matter interaction
AC Stark effect
dressed states
78.67.Hc
42.50.Hz
url https://doi.org/10.1088/1367-2630/aa5198
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AT kroychoudhury probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT tjohn probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT slportalupi probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT cschneider probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT shofling probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT mkamp probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT shughes probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons
AT pmichler probingdifferentregimesofstrongfieldlightmatterinteractionwithsemiconductorquantumdotsandfewcavityphotons