Direct observation of ultrafast singlet exciton fission in three dimensions

Here, the authors use quantitative ultrafast interferometric pump-probe microscopy to track photoexcitations with sub-10 nm spatial precision in three dimensions and 15 fs temporal resolution to study the spatiotemporal dynamics of singlet exciton fission in polycrystalline pentacene films.

Bibliographic Details
Main Authors: Arjun Ashoka, Nicolas Gauriot, Aswathy V. Girija, Nipun Sawhney, Alexander J. Sneyd, Kenji Watanabe, Takashi Taniguchi, Jooyoung Sung, Christoph Schnedermann, Akshay Rao
Format: Article
Language:English
Published: Nature Portfolio 2022-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-33647-5
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author Arjun Ashoka
Nicolas Gauriot
Aswathy V. Girija
Nipun Sawhney
Alexander J. Sneyd
Kenji Watanabe
Takashi Taniguchi
Jooyoung Sung
Christoph Schnedermann
Akshay Rao
author_facet Arjun Ashoka
Nicolas Gauriot
Aswathy V. Girija
Nipun Sawhney
Alexander J. Sneyd
Kenji Watanabe
Takashi Taniguchi
Jooyoung Sung
Christoph Schnedermann
Akshay Rao
author_sort Arjun Ashoka
collection DOAJ
description Here, the authors use quantitative ultrafast interferometric pump-probe microscopy to track photoexcitations with sub-10 nm spatial precision in three dimensions and 15 fs temporal resolution to study the spatiotemporal dynamics of singlet exciton fission in polycrystalline pentacene films.
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spelling doaj.art-d4739ce7f82e43e493f6bdb7fbe297862022-12-22T02:24:36ZengNature PortfolioNature Communications2041-17232022-10-011311810.1038/s41467-022-33647-5Direct observation of ultrafast singlet exciton fission in three dimensionsArjun Ashoka0Nicolas Gauriot1Aswathy V. Girija2Nipun Sawhney3Alexander J. Sneyd4Kenji Watanabe5Takashi Taniguchi6Jooyoung Sung7Christoph Schnedermann8Akshay Rao9Cavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeResearch Center for Functional Materials, National Institute for Materials ScienceInternational Center for Materials Nanoarchitectonics, National Institute for Materials ScienceDepartment of Emerging Materials Science, DGISTCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeHere, the authors use quantitative ultrafast interferometric pump-probe microscopy to track photoexcitations with sub-10 nm spatial precision in three dimensions and 15 fs temporal resolution to study the spatiotemporal dynamics of singlet exciton fission in polycrystalline pentacene films.https://doi.org/10.1038/s41467-022-33647-5
spellingShingle Arjun Ashoka
Nicolas Gauriot
Aswathy V. Girija
Nipun Sawhney
Alexander J. Sneyd
Kenji Watanabe
Takashi Taniguchi
Jooyoung Sung
Christoph Schnedermann
Akshay Rao
Direct observation of ultrafast singlet exciton fission in three dimensions
Nature Communications
title Direct observation of ultrafast singlet exciton fission in three dimensions
title_full Direct observation of ultrafast singlet exciton fission in three dimensions
title_fullStr Direct observation of ultrafast singlet exciton fission in three dimensions
title_full_unstemmed Direct observation of ultrafast singlet exciton fission in three dimensions
title_short Direct observation of ultrafast singlet exciton fission in three dimensions
title_sort direct observation of ultrafast singlet exciton fission in three dimensions
url https://doi.org/10.1038/s41467-022-33647-5
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