Tackling realistic Li+ flux for high-energy lithium metal batteries
The low conductivity of LiF disturbs Li+ diffusion across solid electrolyte interphase (SEI) and induces Li+ transfer-driven dendritic growth. Herein, the authors establish a mechanistic model to decipher how the SEI affects realistic Li plating in high-fluorine electrolytes.
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2022-09-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-33151-w |
| _version_ | 1828148117085618176 |
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| author | Shuoqing Zhang Ruhong Li Nan Hu Tao Deng Suting Weng Zunchun Wu Di Lu Haikuo Zhang Junbo Zhang Xuefeng Wang Lixin Chen Liwu Fan Xiulin Fan |
| author_facet | Shuoqing Zhang Ruhong Li Nan Hu Tao Deng Suting Weng Zunchun Wu Di Lu Haikuo Zhang Junbo Zhang Xuefeng Wang Lixin Chen Liwu Fan Xiulin Fan |
| author_sort | Shuoqing Zhang |
| collection | DOAJ |
| description | The low conductivity of LiF disturbs Li+ diffusion across solid electrolyte interphase (SEI) and induces Li+ transfer-driven dendritic growth. Herein, the authors establish a mechanistic model to decipher how the SEI affects realistic Li plating in high-fluorine electrolytes. |
| first_indexed | 2024-04-11T21:10:19Z |
| format | Article |
| id | doaj.art-d5865733ac244489bfb6a01f378dd20f |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-11T21:10:19Z |
| publishDate | 2022-09-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-d5865733ac244489bfb6a01f378dd20f2022-12-22T04:03:03ZengNature PortfolioNature Communications2041-17232022-09-0113111210.1038/s41467-022-33151-wTackling realistic Li+ flux for high-energy lithium metal batteriesShuoqing Zhang0Ruhong Li1Nan Hu2Tao Deng3Suting Weng4Zunchun Wu5Di Lu6Haikuo Zhang7Junbo Zhang8Xuefeng Wang9Lixin Chen10Liwu Fan11Xiulin Fan12State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, School of Energy Engineering, Zhejiang UniversityDepartment of Chemical and Biomolecular Engineering, University of MarylandBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, School of Energy Engineering, Zhejiang UniversityState Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityThe low conductivity of LiF disturbs Li+ diffusion across solid electrolyte interphase (SEI) and induces Li+ transfer-driven dendritic growth. Herein, the authors establish a mechanistic model to decipher how the SEI affects realistic Li plating in high-fluorine electrolytes.https://doi.org/10.1038/s41467-022-33151-w |
| spellingShingle | Shuoqing Zhang Ruhong Li Nan Hu Tao Deng Suting Weng Zunchun Wu Di Lu Haikuo Zhang Junbo Zhang Xuefeng Wang Lixin Chen Liwu Fan Xiulin Fan Tackling realistic Li+ flux for high-energy lithium metal batteries Nature Communications |
| title | Tackling realistic Li+ flux for high-energy lithium metal batteries |
| title_full | Tackling realistic Li+ flux for high-energy lithium metal batteries |
| title_fullStr | Tackling realistic Li+ flux for high-energy lithium metal batteries |
| title_full_unstemmed | Tackling realistic Li+ flux for high-energy lithium metal batteries |
| title_short | Tackling realistic Li+ flux for high-energy lithium metal batteries |
| title_sort | tackling realistic li flux for high energy lithium metal batteries |
| url | https://doi.org/10.1038/s41467-022-33151-w |
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