Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing

Abstract Nonlinear optics provides a means to bridge between different electromagnetic frequencies, enabling communication between visible, infrared, and terahertz bands through χ (2) and higher-order nonlinear optical processes. However, precisely modulating nonlinear optical waves in 3D space rema...

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Main Authors: Pengcheng Chen, Xiaoyi Xu, Tianxin Wang, Chao Zhou, Dunzhao Wei, Jianan Ma, Junjie Guo, Xuejing Cui, Xiaoyan Cheng, Chenzhu Xie, Shuang Zhang, Shining Zhu, Min Xiao, Yong Zhang
Format: Article
Language:English
Published: Nature Portfolio 2023-09-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-41350-2
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author Pengcheng Chen
Xiaoyi Xu
Tianxin Wang
Chao Zhou
Dunzhao Wei
Jianan Ma
Junjie Guo
Xuejing Cui
Xiaoyan Cheng
Chenzhu Xie
Shuang Zhang
Shining Zhu
Min Xiao
Yong Zhang
author_facet Pengcheng Chen
Xiaoyi Xu
Tianxin Wang
Chao Zhou
Dunzhao Wei
Jianan Ma
Junjie Guo
Xuejing Cui
Xiaoyan Cheng
Chenzhu Xie
Shuang Zhang
Shining Zhu
Min Xiao
Yong Zhang
author_sort Pengcheng Chen
collection DOAJ
description Abstract Nonlinear optics provides a means to bridge between different electromagnetic frequencies, enabling communication between visible, infrared, and terahertz bands through χ (2) and higher-order nonlinear optical processes. However, precisely modulating nonlinear optical waves in 3D space remains a significant challenge, severely limiting the ability to directly manipulate optical information across different wavelength bands. Here, we propose and experimentally demonstrate a three-dimensional (3D) χ (2)-super-pixel hologram with nanometer resolution in lithium niobate crystals, capable of performing advanced processing tasks. In our design, each pixel consists of properly arranged nanodomain structures capable of completely and dynamically manipulating the complex-amplitude of nonlinear waves. Fabricated by femtosecond laser writing, the nonlinear hologram features a pixel diameter of 500 nm and a pixel density of approximately 25000 pixels-per-inch (PPI), reaching far beyond the state of the art. In our experiments, we successfully demonstrate the novel functions of the hologram to process near-infrared (NIR) information at visible wavelengths, including dynamic 3D nonlinear holographic imaging and frequency-up-converted image recognition. Our scheme provides a promising nano-optic platform for high-capacity optical storage and multi-functional information processing across different wavelength ranges.
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spelling doaj.art-d5c5218116894470a04c022e0a7458232023-11-20T10:00:35ZengNature PortfolioNature Communications2041-17232023-09-011411910.1038/s41467-023-41350-2Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processingPengcheng Chen0Xiaoyi Xu1Tianxin Wang2Chao Zhou3Dunzhao Wei4Jianan Ma5Junjie Guo6Xuejing Cui7Xiaoyan Cheng8Chenzhu Xie9Shuang Zhang10Shining Zhu11Min Xiao12Yong Zhang13National Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversitySchool of Physics, Sun Yat-sen UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityDepartment of Physics, The University of Hong KongNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, School of Physics, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityAbstract Nonlinear optics provides a means to bridge between different electromagnetic frequencies, enabling communication between visible, infrared, and terahertz bands through χ (2) and higher-order nonlinear optical processes. However, precisely modulating nonlinear optical waves in 3D space remains a significant challenge, severely limiting the ability to directly manipulate optical information across different wavelength bands. Here, we propose and experimentally demonstrate a three-dimensional (3D) χ (2)-super-pixel hologram with nanometer resolution in lithium niobate crystals, capable of performing advanced processing tasks. In our design, each pixel consists of properly arranged nanodomain structures capable of completely and dynamically manipulating the complex-amplitude of nonlinear waves. Fabricated by femtosecond laser writing, the nonlinear hologram features a pixel diameter of 500 nm and a pixel density of approximately 25000 pixels-per-inch (PPI), reaching far beyond the state of the art. In our experiments, we successfully demonstrate the novel functions of the hologram to process near-infrared (NIR) information at visible wavelengths, including dynamic 3D nonlinear holographic imaging and frequency-up-converted image recognition. Our scheme provides a promising nano-optic platform for high-capacity optical storage and multi-functional information processing across different wavelength ranges.https://doi.org/10.1038/s41467-023-41350-2
spellingShingle Pengcheng Chen
Xiaoyi Xu
Tianxin Wang
Chao Zhou
Dunzhao Wei
Jianan Ma
Junjie Guo
Xuejing Cui
Xiaoyan Cheng
Chenzhu Xie
Shuang Zhang
Shining Zhu
Min Xiao
Yong Zhang
Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
Nature Communications
title Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
title_full Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
title_fullStr Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
title_full_unstemmed Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
title_short Laser nanoprinting of 3D nonlinear holograms beyond 25000 pixels-per-inch for inter-wavelength-band information processing
title_sort laser nanoprinting of 3d nonlinear holograms beyond 25000 pixels per inch for inter wavelength band information processing
url https://doi.org/10.1038/s41467-023-41350-2
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