Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness

The real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of...

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Main Authors: Yuli Xu, Zicheng Liu, Jingren Lin, Jintao Zhao, Nguyen Duc Hoa, Nguyen Van Hieu, Alexander A. Ganeev, Victoria Chuchina, Abolghasem Jouyban, Daxiang Cui, Ying Wang, Han Jin
Format: Article
Language:English
Published: MDPI AG 2023-09-01
Series:Sensors
Subjects:
Online Access:https://www.mdpi.com/1424-8220/23/19/8109
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author Yuli Xu
Zicheng Liu
Jingren Lin
Jintao Zhao
Nguyen Duc Hoa
Nguyen Van Hieu
Alexander A. Ganeev
Victoria Chuchina
Abolghasem Jouyban
Daxiang Cui
Ying Wang
Han Jin
author_facet Yuli Xu
Zicheng Liu
Jingren Lin
Jintao Zhao
Nguyen Duc Hoa
Nguyen Van Hieu
Alexander A. Ganeev
Victoria Chuchina
Abolghasem Jouyban
Daxiang Cui
Ying Wang
Han Jin
author_sort Yuli Xu
collection DOAJ
description The real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of volatile molecules. Nevertheless, the ambient environment of low temperature (normally below 4 °C) and high humidity (90% R.H.), as well as poor selectivity in sensing gas species remain the challenge. In this research, an integrated smart gas-tracking device is designed and fabricated. By applying pump voltage on the yttria-stabilized zirconia (YSZ) membrane, the oxygen concentration in the testing chamber can be manually tailored. Due to the working principle of the sensor following the mixed potential behavior, distinct differences in sensitivity and selectivity are observed for the sensor that operated at different oxygen concentrations. Typically, the sensor gives satisfactory selectivity to H<sub>2</sub>S, NH<sub>3</sub>, and C<sub>2</sub>H<sub>5</sub>OH at the oxygen concentrations of 10%, 30%, and 40%, respectively. In addition, an acceptable response/recovery rate (within 24 s) is also confirmed. Finally, a refrigerator prototype that includes the smart gas sensor is built, and satisfactory performance in discriminating food freshness status of fresh or semi-fresh is verified for the proposed refrigerator prototype. In conclusion, these aforementioned promising results suggest that the proposed integrated smart gas sensor could be a potential candidate for alarming food spoilage.
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spelling doaj.art-d5d97a963d7d4254b5414f4ee15e060d2023-11-19T15:02:51ZengMDPI AGSensors1424-82202023-09-012319810910.3390/s23198109Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food FreshnessYuli Xu0Zicheng Liu1Jingren Lin2Jintao Zhao3Nguyen Duc Hoa4Nguyen Van Hieu5Alexander A. Ganeev6Victoria Chuchina7Abolghasem Jouyban8Daxiang Cui9Ying Wang10Han Jin11Institute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInternational Training Institute for Material Science, Hanoi University of Science and Technology, Hanoi 100000, VietnamFaculty of Electrical and Electronic Engineering, Phenikaa University, Hanoi 100000, VietnamDepartment of Chemistry, St Petersburg University, 7/9 Universitetskaya Emb., St. Petersburg 199034, RussiaDepartment of Chemistry, St Petersburg University, 7/9 Universitetskaya Emb., St. Petersburg 199034, RussiaPharmaceutical Analysis Research Center, Faculty of Pharmacy, Tabriz University of Medical Sciences, Tabriz 51368, IranInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaChengdu Environmental Investment Group Co., Ltd., Building 1, Tianfushijia, No. 1000 Jincheng Street, Chengdu 610000, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaThe real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of volatile molecules. Nevertheless, the ambient environment of low temperature (normally below 4 °C) and high humidity (90% R.H.), as well as poor selectivity in sensing gas species remain the challenge. In this research, an integrated smart gas-tracking device is designed and fabricated. By applying pump voltage on the yttria-stabilized zirconia (YSZ) membrane, the oxygen concentration in the testing chamber can be manually tailored. Due to the working principle of the sensor following the mixed potential behavior, distinct differences in sensitivity and selectivity are observed for the sensor that operated at different oxygen concentrations. Typically, the sensor gives satisfactory selectivity to H<sub>2</sub>S, NH<sub>3</sub>, and C<sub>2</sub>H<sub>5</sub>OH at the oxygen concentrations of 10%, 30%, and 40%, respectively. In addition, an acceptable response/recovery rate (within 24 s) is also confirmed. Finally, a refrigerator prototype that includes the smart gas sensor is built, and satisfactory performance in discriminating food freshness status of fresh or semi-fresh is verified for the proposed refrigerator prototype. In conclusion, these aforementioned promising results suggest that the proposed integrated smart gas sensor could be a potential candidate for alarming food spoilage.https://www.mdpi.com/1424-8220/23/19/8109artificially tailored selectivitysmart gas sensoryttria-stabilized zirconia (YSZ)volatile compoundsfood freshness
spellingShingle Yuli Xu
Zicheng Liu
Jingren Lin
Jintao Zhao
Nguyen Duc Hoa
Nguyen Van Hieu
Alexander A. Ganeev
Victoria Chuchina
Abolghasem Jouyban
Daxiang Cui
Ying Wang
Han Jin
Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
Sensors
artificially tailored selectivity
smart gas sensor
yttria-stabilized zirconia (YSZ)
volatile compounds
food freshness
title Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
title_full Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
title_fullStr Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
title_full_unstemmed Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
title_short Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
title_sort integrated smart gas tracking device with artificially tailored selectivity for real time monitoring food freshness
topic artificially tailored selectivity
smart gas sensor
yttria-stabilized zirconia (YSZ)
volatile compounds
food freshness
url https://www.mdpi.com/1424-8220/23/19/8109
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