Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness
The real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of...
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MDPI AG
2023-09-01
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author | Yuli Xu Zicheng Liu Jingren Lin Jintao Zhao Nguyen Duc Hoa Nguyen Van Hieu Alexander A. Ganeev Victoria Chuchina Abolghasem Jouyban Daxiang Cui Ying Wang Han Jin |
author_facet | Yuli Xu Zicheng Liu Jingren Lin Jintao Zhao Nguyen Duc Hoa Nguyen Van Hieu Alexander A. Ganeev Victoria Chuchina Abolghasem Jouyban Daxiang Cui Ying Wang Han Jin |
author_sort | Yuli Xu |
collection | DOAJ |
description | The real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of volatile molecules. Nevertheless, the ambient environment of low temperature (normally below 4 °C) and high humidity (90% R.H.), as well as poor selectivity in sensing gas species remain the challenge. In this research, an integrated smart gas-tracking device is designed and fabricated. By applying pump voltage on the yttria-stabilized zirconia (YSZ) membrane, the oxygen concentration in the testing chamber can be manually tailored. Due to the working principle of the sensor following the mixed potential behavior, distinct differences in sensitivity and selectivity are observed for the sensor that operated at different oxygen concentrations. Typically, the sensor gives satisfactory selectivity to H<sub>2</sub>S, NH<sub>3</sub>, and C<sub>2</sub>H<sub>5</sub>OH at the oxygen concentrations of 10%, 30%, and 40%, respectively. In addition, an acceptable response/recovery rate (within 24 s) is also confirmed. Finally, a refrigerator prototype that includes the smart gas sensor is built, and satisfactory performance in discriminating food freshness status of fresh or semi-fresh is verified for the proposed refrigerator prototype. In conclusion, these aforementioned promising results suggest that the proposed integrated smart gas sensor could be a potential candidate for alarming food spoilage. |
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spelling | doaj.art-d5d97a963d7d4254b5414f4ee15e060d2023-11-19T15:02:51ZengMDPI AGSensors1424-82202023-09-012319810910.3390/s23198109Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food FreshnessYuli Xu0Zicheng Liu1Jingren Lin2Jintao Zhao3Nguyen Duc Hoa4Nguyen Van Hieu5Alexander A. Ganeev6Victoria Chuchina7Abolghasem Jouyban8Daxiang Cui9Ying Wang10Han Jin11Institute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaInternational Training Institute for Material Science, Hanoi University of Science and Technology, Hanoi 100000, VietnamFaculty of Electrical and Electronic Engineering, Phenikaa University, Hanoi 100000, VietnamDepartment of Chemistry, St Petersburg University, 7/9 Universitetskaya Emb., St. Petersburg 199034, RussiaDepartment of Chemistry, St Petersburg University, 7/9 Universitetskaya Emb., St. Petersburg 199034, RussiaPharmaceutical Analysis Research Center, Faculty of Pharmacy, Tabriz University of Medical Sciences, Tabriz 51368, IranInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaChengdu Environmental Investment Group Co., Ltd., Building 1, Tianfushijia, No. 1000 Jincheng Street, Chengdu 610000, ChinaInstitute of Micro-Nano Science and Technology, School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, ChinaThe real-time monitoring of food freshness in refrigerators is of significant importance in detecting potential food spoiling and preventing serious health issues. One method that is commonly reported and has received substantial attention is the discrimination of food freshness via the tracking of volatile molecules. Nevertheless, the ambient environment of low temperature (normally below 4 °C) and high humidity (90% R.H.), as well as poor selectivity in sensing gas species remain the challenge. In this research, an integrated smart gas-tracking device is designed and fabricated. By applying pump voltage on the yttria-stabilized zirconia (YSZ) membrane, the oxygen concentration in the testing chamber can be manually tailored. Due to the working principle of the sensor following the mixed potential behavior, distinct differences in sensitivity and selectivity are observed for the sensor that operated at different oxygen concentrations. Typically, the sensor gives satisfactory selectivity to H<sub>2</sub>S, NH<sub>3</sub>, and C<sub>2</sub>H<sub>5</sub>OH at the oxygen concentrations of 10%, 30%, and 40%, respectively. In addition, an acceptable response/recovery rate (within 24 s) is also confirmed. Finally, a refrigerator prototype that includes the smart gas sensor is built, and satisfactory performance in discriminating food freshness status of fresh or semi-fresh is verified for the proposed refrigerator prototype. In conclusion, these aforementioned promising results suggest that the proposed integrated smart gas sensor could be a potential candidate for alarming food spoilage.https://www.mdpi.com/1424-8220/23/19/8109artificially tailored selectivitysmart gas sensoryttria-stabilized zirconia (YSZ)volatile compoundsfood freshness |
spellingShingle | Yuli Xu Zicheng Liu Jingren Lin Jintao Zhao Nguyen Duc Hoa Nguyen Van Hieu Alexander A. Ganeev Victoria Chuchina Abolghasem Jouyban Daxiang Cui Ying Wang Han Jin Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness Sensors artificially tailored selectivity smart gas sensor yttria-stabilized zirconia (YSZ) volatile compounds food freshness |
title | Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness |
title_full | Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness |
title_fullStr | Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness |
title_full_unstemmed | Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness |
title_short | Integrated Smart Gas Tracking Device with Artificially Tailored Selectivity for Real-Time Monitoring Food Freshness |
title_sort | integrated smart gas tracking device with artificially tailored selectivity for real time monitoring food freshness |
topic | artificially tailored selectivity smart gas sensor yttria-stabilized zirconia (YSZ) volatile compounds food freshness |
url | https://www.mdpi.com/1424-8220/23/19/8109 |
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