Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy

We report the frequency stabilization of an external cavity diode laser (ECDL) to a reference molecular iodine (I<sub>2</sub>) transition at 13,531.18 cm<sup>−1</sup> (739.03382 nm). Using the Modulation Transfer Spectroscopy (MTS) method for the highly sensitive detection of...

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Main Authors: Lakhi Sharma, Atish Roy, Subhasis Panja, Subhadeep De
Format: Article
Language:English
Published: MDPI AG 2023-05-01
Series:Atoms
Subjects:
Online Access:https://www.mdpi.com/2218-2004/11/5/83
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author Lakhi Sharma
Atish Roy
Subhasis Panja
Subhadeep De
author_facet Lakhi Sharma
Atish Roy
Subhasis Panja
Subhadeep De
author_sort Lakhi Sharma
collection DOAJ
description We report the frequency stabilization of an external cavity diode laser (ECDL) to a reference molecular iodine (I<sub>2</sub>) transition at 13,531.18 cm<sup>−1</sup> (739.03382 nm). Using the Modulation Transfer Spectroscopy (MTS) method for the highly sensitive detection of weak absorption signals, the Doppler-free absorption peaks of I<sub>2</sub> corresponding to the hot band transition R(78) (1–11) are resolved. The ECDL’s frequency is stabilized with respect to one of the lines lying within the reference absorption band. For this, the iodine vapor cell is heated to 450 °C and the corresponding circularly polarized pump and probe beam powers are maintained at 10 mW and 1 mW, respectively, to avoid power broadening. The short (100 ms) and long-term (50 h) linewidths of the frequency stabilized laser are measured to be 0.75(3) MHz and 0.5(2) MHz, respectively, whereas the natural linewidth of the specific I<sub>2</sub>-transitions lie within a range of tens of MHz.
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spelling doaj.art-d6616c7ef3d04c2d8b63ade63b543a8d2023-11-18T00:26:46ZengMDPI AGAtoms2218-20042023-05-011158310.3390/atoms11050083Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer SpectroscopyLakhi Sharma0Atish Roy1Subhasis Panja2Subhadeep De3CSIR—National Physical Laboratory, Dr. K. S. Krishnan Marg, New Delhi 110012, IndiaCSIR—National Physical Laboratory, Dr. K. S. Krishnan Marg, New Delhi 110012, IndiaCSIR—National Physical Laboratory, Dr. K. S. Krishnan Marg, New Delhi 110012, IndiaInter-University Centre for Astronomy and Astrophysics (IUCAA), Post Bag 4, Pune 411007, IndiaWe report the frequency stabilization of an external cavity diode laser (ECDL) to a reference molecular iodine (I<sub>2</sub>) transition at 13,531.18 cm<sup>−1</sup> (739.03382 nm). Using the Modulation Transfer Spectroscopy (MTS) method for the highly sensitive detection of weak absorption signals, the Doppler-free absorption peaks of I<sub>2</sub> corresponding to the hot band transition R(78) (1–11) are resolved. The ECDL’s frequency is stabilized with respect to one of the lines lying within the reference absorption band. For this, the iodine vapor cell is heated to 450 °C and the corresponding circularly polarized pump and probe beam powers are maintained at 10 mW and 1 mW, respectively, to avoid power broadening. The short (100 ms) and long-term (50 h) linewidths of the frequency stabilized laser are measured to be 0.75(3) MHz and 0.5(2) MHz, respectively, whereas the natural linewidth of the specific I<sub>2</sub>-transitions lie within a range of tens of MHz.https://www.mdpi.com/2218-2004/11/5/83frequency stabilizationmodulation transfer spectroscopyatomic clockfrequency metrologyfour-wave mixingsaturated absorption spectroscopy
spellingShingle Lakhi Sharma
Atish Roy
Subhasis Panja
Subhadeep De
Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
Atoms
frequency stabilization
modulation transfer spectroscopy
atomic clock
frequency metrology
four-wave mixing
saturated absorption spectroscopy
title Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
title_full Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
title_fullStr Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
title_full_unstemmed Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
title_short Stabilizing Frequency of a Diode Laser to a Reference Transition of Molecular Iodine through Modulation Transfer Spectroscopy
title_sort stabilizing frequency of a diode laser to a reference transition of molecular iodine through modulation transfer spectroscopy
topic frequency stabilization
modulation transfer spectroscopy
atomic clock
frequency metrology
four-wave mixing
saturated absorption spectroscopy
url https://www.mdpi.com/2218-2004/11/5/83
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AT atishroy stabilizingfrequencyofadiodelasertoareferencetransitionofmoleculariodinethroughmodulationtransferspectroscopy
AT subhasispanja stabilizingfrequencyofadiodelasertoareferencetransitionofmoleculariodinethroughmodulationtransferspectroscopy
AT subhadeepde stabilizingfrequencyofadiodelasertoareferencetransitionofmoleculariodinethroughmodulationtransferspectroscopy