Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols

As an important fraction of light-absorbing particles, black carbon (BC) has a significant warming effect, despite accounting for a small proportion of total aerosols. A comprehensive investigation was conducted on the characteristics of atmospheric aerosols and BC particles over Wuhan, China. Mass...

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Main Authors: Yingying Ma, Ruonan Fan, Shikuan Jin, Xin Ma, Ming Zhang, Wei Gong, Boming Liu, Yifan Shi, Yiqun Zhang, Hui Li
Format: Article
Language:English
Published: MDPI AG 2021-09-01
Series:Remote Sensing
Subjects:
Online Access:https://www.mdpi.com/2072-4292/13/18/3620
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author Yingying Ma
Ruonan Fan
Shikuan Jin
Xin Ma
Ming Zhang
Wei Gong
Boming Liu
Yifan Shi
Yiqun Zhang
Hui Li
author_facet Yingying Ma
Ruonan Fan
Shikuan Jin
Xin Ma
Ming Zhang
Wei Gong
Boming Liu
Yifan Shi
Yiqun Zhang
Hui Li
author_sort Yingying Ma
collection DOAJ
description As an important fraction of light-absorbing particles, black carbon (BC) has a significant warming effect, despite accounting for a small proportion of total aerosols. A comprehensive investigation was conducted on the characteristics of atmospheric aerosols and BC particles over Wuhan, China. Mass concentration, optical properties, and radiative forcing of total aerosols and BC were estimated using multi-source observation data. Results showed that the BC concentration monthly mean varied from 2.19 to 5.33 μg m<sup>−3</sup>. The BC aerosol optical depth (AOD) maximum monthly mean (0.026) occurred in winter, whereas the maximum total AOD (1.75) occurred in summer. Under polluted-air conditions, both aerosol radiative forcing (ARF) and BC radiative forcing (BCRF) at the bottom of the atmosphere (BOA) were strongest in summer, with values of −83.01 and −11.22 W m<sup>−2</sup>, respectively. In summer, ARF at BOA on polluted-air days was more than two-fold that on clean-air days. In addition, compared with clean-air days, BCRF at BOA on polluted-air days was increased by 76% and 73% in summer and winter, respectively. The results indicate an important influence of particulate air pollution on ARF and BCRF. Furthermore, the average contribution of BCRF to ARF was 13.8%, even though the proportion of BC in PM<sub>2.5</sub> was only 5.1%.
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spelling doaj.art-d6e51684caeb4d5c94e5db27812eae302023-11-22T15:05:45ZengMDPI AGRemote Sensing2072-42922021-09-011318362010.3390/rs13183620Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric AerosolsYingying Ma0Ruonan Fan1Shikuan Jin2Xin Ma3Ming Zhang4Wei Gong5Boming Liu6Yifan Shi7Yiqun Zhang8Hui Li9State Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaHubei Key Laboratory of Critical Zone Evolution, School of Geography and Information Engineering, China University of Geosciences, Wuhan 430074, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaSchool of Mathematics and Statistics, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaState Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, ChinaAs an important fraction of light-absorbing particles, black carbon (BC) has a significant warming effect, despite accounting for a small proportion of total aerosols. A comprehensive investigation was conducted on the characteristics of atmospheric aerosols and BC particles over Wuhan, China. Mass concentration, optical properties, and radiative forcing of total aerosols and BC were estimated using multi-source observation data. Results showed that the BC concentration monthly mean varied from 2.19 to 5.33 μg m<sup>−3</sup>. The BC aerosol optical depth (AOD) maximum monthly mean (0.026) occurred in winter, whereas the maximum total AOD (1.75) occurred in summer. Under polluted-air conditions, both aerosol radiative forcing (ARF) and BC radiative forcing (BCRF) at the bottom of the atmosphere (BOA) were strongest in summer, with values of −83.01 and −11.22 W m<sup>−2</sup>, respectively. In summer, ARF at BOA on polluted-air days was more than two-fold that on clean-air days. In addition, compared with clean-air days, BCRF at BOA on polluted-air days was increased by 76% and 73% in summer and winter, respectively. The results indicate an important influence of particulate air pollution on ARF and BCRF. Furthermore, the average contribution of BCRF to ARF was 13.8%, even though the proportion of BC in PM<sub>2.5</sub> was only 5.1%.https://www.mdpi.com/2072-4292/13/18/3620aerosol optical propertyair pollutionblack carbonOPACradiative forcingSBDART
spellingShingle Yingying Ma
Ruonan Fan
Shikuan Jin
Xin Ma
Ming Zhang
Wei Gong
Boming Liu
Yifan Shi
Yiqun Zhang
Hui Li
Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
Remote Sensing
aerosol optical property
air pollution
black carbon
OPAC
radiative forcing
SBDART
title Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
title_full Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
title_fullStr Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
title_full_unstemmed Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
title_short Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols
title_sort black carbon over wuhan china seasonal variations in its optical properties radiative forcing and contribution to atmospheric aerosols
topic aerosol optical property
air pollution
black carbon
OPAC
radiative forcing
SBDART
url https://www.mdpi.com/2072-4292/13/18/3620
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