Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes

This paper describes a way to implement a transparent electrode for symmetrical emission from the bottom and top sides of transparent organic light-emitting diodes (TOLEDs). An ultrathin (~6 nm) and smooth Ag film was achieved by using the pretreatment of using oxygen plasma prior to deposition of a...

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Main Authors: Illhwan Lee, Sungjun Kim, Jae Yong Park, Sungjoo Kim, Hyung Won Cho, Juyoung Ham, Seungo Gim, Kisoo Kim, Kihyon Hong, Jong-Lam Lee
Format: Article
Language:English
Published: IEEE 2018-01-01
Series:IEEE Photonics Journal
Subjects:
Online Access:https://ieeexplore.ieee.org/document/8332474/
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author Illhwan Lee
Sungjun Kim
Jae Yong Park
Sungjoo Kim
Hyung Won Cho
Juyoung Ham
Seungo Gim
Kisoo Kim
Kihyon Hong
Jong-Lam Lee
author_facet Illhwan Lee
Sungjun Kim
Jae Yong Park
Sungjoo Kim
Hyung Won Cho
Juyoung Ham
Seungo Gim
Kisoo Kim
Kihyon Hong
Jong-Lam Lee
author_sort Illhwan Lee
collection DOAJ
description This paper describes a way to implement a transparent electrode for symmetrical emission from the bottom and top sides of transparent organic light-emitting diodes (TOLEDs). An ultrathin (~6 nm) and smooth Ag film was achieved by using the pretreatment of using oxygen plasma prior to deposition of a nanoscale-thin Ag film on glass. The treatment increased the surface energy, thereby enhancing the wettability of the Ag on glass substrate and consequently leading to the formation of thin and unifrom Ag film with high optical transmittance T ~ 76% and low sheet resistance RS &lt;; 15 &#x03A9; &#x25A1;<sup>-1</sup>. Using this scheme, a highly transparent glass/Ag/WO3 structure with T = 85.6%, and RS = 9.3 &#x03A9; &#x25A1;<sup>-1</sup> was designed (ITO: 83.1%, 10 &#x03A9; &#x25A1;<sup>-1</sup>). We conducted finite-domain time-difference simulation for this glass/Ag/WO3 electrode to design a weak microcavity structure that retained the transparency and emitting properties. This optimized structure of TOLEDs (Ag = 6 nm) showed higher T = 73.84% than those of ITO devices (T = 73.19%), and can induce the weak microcavity effect, resuting in improved electroluminescent properties and increased the luminance value from 38.25 to 56.25 cd A<sup>-1</sup> at 25 mA cm<sup>-2</sup>.
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spelling doaj.art-d7983f44e98342c3acae1d9637a609202022-12-21T21:35:54ZengIEEEIEEE Photonics Journal1943-06552018-01-0110311010.1109/JPHOT.2018.28237598332474Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag ElectrodesIllhwan Lee0Sungjun Kim1Jae Yong Park2Sungjoo Kim3Hyung Won Cho4Juyoung Ham5Seungo Gim6Kisoo Kim7Kihyon Hong8Jong-Lam Lee9https://orcid.org/0000-0003-4502-9758Department of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaDepartment of Materials Science and Engineering, Pohang University of Science and Technology, Pohang, South KoreaThis paper describes a way to implement a transparent electrode for symmetrical emission from the bottom and top sides of transparent organic light-emitting diodes (TOLEDs). An ultrathin (~6 nm) and smooth Ag film was achieved by using the pretreatment of using oxygen plasma prior to deposition of a nanoscale-thin Ag film on glass. The treatment increased the surface energy, thereby enhancing the wettability of the Ag on glass substrate and consequently leading to the formation of thin and unifrom Ag film with high optical transmittance T ~ 76% and low sheet resistance RS &lt;; 15 &#x03A9; &#x25A1;<sup>-1</sup>. Using this scheme, a highly transparent glass/Ag/WO3 structure with T = 85.6%, and RS = 9.3 &#x03A9; &#x25A1;<sup>-1</sup> was designed (ITO: 83.1%, 10 &#x03A9; &#x25A1;<sup>-1</sup>). We conducted finite-domain time-difference simulation for this glass/Ag/WO3 electrode to design a weak microcavity structure that retained the transparency and emitting properties. This optimized structure of TOLEDs (Ag = 6 nm) showed higher T = 73.84% than those of ITO devices (T = 73.19%), and can induce the weak microcavity effect, resuting in improved electroluminescent properties and increased the luminance value from 38.25 to 56.25 cd A<sup>-1</sup> at 25 mA cm<sup>-2</sup>.https://ieeexplore.ieee.org/document/8332474/Organic light-emitting diodetransparentultra-thinbi-directionalmicro-cavity.
spellingShingle Illhwan Lee
Sungjun Kim
Jae Yong Park
Sungjoo Kim
Hyung Won Cho
Juyoung Ham
Seungo Gim
Kisoo Kim
Kihyon Hong
Jong-Lam Lee
Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
IEEE Photonics Journal
Organic light-emitting diode
transparent
ultra-thin
bi-directional
micro-cavity.
title Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
title_full Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
title_fullStr Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
title_full_unstemmed Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
title_short Symmetrical Emission Transparent Organic Light-Emitting Diodes With Ultrathin Ag Electrodes
title_sort symmetrical emission transparent organic light emitting diodes with ultrathin ag electrodes
topic Organic light-emitting diode
transparent
ultra-thin
bi-directional
micro-cavity.
url https://ieeexplore.ieee.org/document/8332474/
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