Z-Scan theory for thin film measurements: Validation of a model beyond the standard approach using ITO and HfO2

The Z-Scan technique is an easy and widespread approach to evaluate the nonlinear optical coefficient of materials. However, the evaluation of the same coefficients for thin films requires complex experimental setups that allow to remove the contributions of the substrate. Here, we propose a simple,...

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Bibliographic Details
Main Authors: Andrea Tognazzi, Paolo Franceschini, Thi Ngoc Lam Tran, Alessandro Chiasera, Maria Antonietta Vincenti, Alfonso Carmelo Cino, Neset Akozbek, Michael Scalora, Costantino De Angelis
Format: Article
Language:English
Published: Elsevier 2023-07-01
Series:Optical Materials: X
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2590147823000165
Description
Summary:The Z-Scan technique is an easy and widespread approach to evaluate the nonlinear optical coefficient of materials. However, the evaluation of the same coefficients for thin films requires complex experimental setups that allow to remove the contributions of the substrate. Here, we propose a simple, yet effective, theoretical approach that allows to include the substrate contribution to the focusing effect when scanning along the propagation axis. The proposed method therefore removes the need of complex experimental setups and paves the way for a simpler retrieval of optical properties of complex nanostructures.
ISSN:2590-1478