Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications

Southwest Florida is one of the most rapidly growing regions of the United States and has been impacted over the past decade with water-quality issues and some associated health problems. The ionic ratios of the dust measured in southwest Florida vary significantly from those on the Florida east coa...

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Main Authors: Razvan Barcan, Zoie R. Kassis, Christopher M. Teaf, Ashley Danley-Thomson, Douglas J. Covert, Thomas M. Missimer
Format: Article
Language:English
Published: MDPI AG 2023-01-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/14/1/102
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author Razvan Barcan
Zoie R. Kassis
Christopher M. Teaf
Ashley Danley-Thomson
Douglas J. Covert
Thomas M. Missimer
author_facet Razvan Barcan
Zoie R. Kassis
Christopher M. Teaf
Ashley Danley-Thomson
Douglas J. Covert
Thomas M. Missimer
author_sort Razvan Barcan
collection DOAJ
description Southwest Florida is one of the most rapidly growing regions of the United States and has been impacted over the past decade with water-quality issues and some associated health problems. The ionic ratios of the dust measured in southwest Florida vary significantly from those on the Florida east coast and in the Caribbean. The metals concentrations reported herein are enriched in potassium and calcium from local sources. Atmospheric deposition of metals and nutrients appears to have potential impacts on both indirect health problems and environmental issues of concern, particularly harmful algal blooms. However, no significant past research has been performed on measurement of the concentration of either metals including the micronutrient iron or nutrient concentrations occurring in atmospheric dry and wet fallout in southwest Florida. Measurements of the composition of key metals and nutrients were made over a one-year period. Concentrations of total phosphorus in the dust ranged from 0–80.5 mg/kg with an average of 4 mg/kg and in rainfall from 1–15.8 чg/L with an average of 4 mg/kg. Nitrate ranged from 0–746 чg/L with an average of 114.4 чg/L in rainfall in a soluble form, and from 1.3 to 718 mg/kg with an average of 209.9 mg/kg in an insoluble form. Ammonia was measured to range from 1.4 to 658 mg/kg with an average of 101.4 mg/kg in rainfall. Iron was found in the dust at concentrations ranging from 0–81 mg/kg with an average of 3.8 mg/kg and in rainfall from 0–125.7 mg/kg with an average of 3.0 mg/kg. While the measured nutrient and iron concentrations are not likely to initiate a harmful algal bloom, they are likely to sustain an existing bloom. Global climate change may exacerbate the atmospheric aerosol issue by increased wind speeds over Africa associated with longer term drought conditions caused by atmospheric temperature increases.
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spelling doaj.art-da4d6399401647d3a382d49fa17579292023-11-30T21:09:25ZengMDPI AGAtmosphere2073-44332023-01-0114110210.3390/atmos14010102Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health ImplicationsRazvan Barcan0Zoie R. Kassis1Christopher M. Teaf2Ashley Danley-Thomson3Douglas J. Covert4Thomas M. Missimer5U.A. Whitaker College of Engineering, Florida Gulf Coast University, 10501 FGCU Boulevard South, Fort Myers, FL 33965-6565, USAU.A. Whitaker College of Engineering, Florida Gulf Coast University, 10501 FGCU Boulevard South, Fort Myers, FL 33965-6565, USAInstitute of Science & Public Affairs, Florida State University, Tallahassee, FL 32306, USADepartment of Bioengineering, Civil and Environmental Engineering, U.A. Whitaker Engineering, Florida Gulf Coast University, 10501 FGCU Boulevard South, Fort Myers, FL 33965-6565, USAHazardous Substance and Waste Management Research, Inc., 2976 Wellington Circle West, Tallahassee, FL 32309, USAU.A. Whitaker College of Engineering, Florida Gulf Coast University, 10501 FGCU Boulevard South, Fort Myers, FL 33965-6565, USASouthwest Florida is one of the most rapidly growing regions of the United States and has been impacted over the past decade with water-quality issues and some associated health problems. The ionic ratios of the dust measured in southwest Florida vary significantly from those on the Florida east coast and in the Caribbean. The metals concentrations reported herein are enriched in potassium and calcium from local sources. Atmospheric deposition of metals and nutrients appears to have potential impacts on both indirect health problems and environmental issues of concern, particularly harmful algal blooms. However, no significant past research has been performed on measurement of the concentration of either metals including the micronutrient iron or nutrient concentrations occurring in atmospheric dry and wet fallout in southwest Florida. Measurements of the composition of key metals and nutrients were made over a one-year period. Concentrations of total phosphorus in the dust ranged from 0–80.5 mg/kg with an average of 4 mg/kg and in rainfall from 1–15.8 чg/L with an average of 4 mg/kg. Nitrate ranged from 0–746 чg/L with an average of 114.4 чg/L in rainfall in a soluble form, and from 1.3 to 718 mg/kg with an average of 209.9 mg/kg in an insoluble form. Ammonia was measured to range from 1.4 to 658 mg/kg with an average of 101.4 mg/kg in rainfall. Iron was found in the dust at concentrations ranging from 0–81 mg/kg with an average of 3.8 mg/kg and in rainfall from 0–125.7 mg/kg with an average of 3.0 mg/kg. While the measured nutrient and iron concentrations are not likely to initiate a harmful algal bloom, they are likely to sustain an existing bloom. Global climate change may exacerbate the atmospheric aerosol issue by increased wind speeds over Africa associated with longer term drought conditions caused by atmospheric temperature increases.https://www.mdpi.com/2073-4433/14/1/102atmospheric dustdust chemistryenvironmental impactshealth implicationsclimate changeSouthwest Florida
spellingShingle Razvan Barcan
Zoie R. Kassis
Christopher M. Teaf
Ashley Danley-Thomson
Douglas J. Covert
Thomas M. Missimer
Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
Atmosphere
atmospheric dust
dust chemistry
environmental impacts
health implications
climate change
Southwest Florida
title Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
title_full Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
title_fullStr Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
title_full_unstemmed Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
title_short Dry and Wet Atmospheric Deposition Composition in Southwest Florida: Environmental and Health Implications
title_sort dry and wet atmospheric deposition composition in southwest florida environmental and health implications
topic atmospheric dust
dust chemistry
environmental impacts
health implications
climate change
Southwest Florida
url https://www.mdpi.com/2073-4433/14/1/102
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AT ashleydanleythomson dryandwetatmosphericdepositioncompositioninsouthwestfloridaenvironmentalandhealthimplications
AT douglasjcovert dryandwetatmosphericdepositioncompositioninsouthwestfloridaenvironmentalandhealthimplications
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