Simulation of the dielectric response of piezoelectric ceramics

We have analyzed the complex permittivity of a porous (10 volume % of pores) sodium-lithium niobate ceramic with the results of computer simulation. The calculation was based on the Cole–Cole formula, which took into account the presence of various mechanisms of relaxation processes in the low-frequ...

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Main Authors: N.E. Malysheva, E.V. Dyakova, O.V. Malyshkina
Format: Article
Language:Russian
Published: Tver State University 2023-12-01
Series:Физико-химические аспекты изучения кластеров, наноструктур и наноматериалов
Subjects:
Online Access:https://physchemaspects.ru/2023/doi-10-26456-pcascnn-2023-15-481/?lang=en
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author N.E. Malysheva
E.V. Dyakova
O.V. Malyshkina
author_facet N.E. Malysheva
E.V. Dyakova
O.V. Malyshkina
author_sort N.E. Malysheva
collection DOAJ
description We have analyzed the complex permittivity of a porous (10 volume % of pores) sodium-lithium niobate ceramic with the results of computer simulation. The calculation was based on the Cole–Cole formula, which took into account the presence of various mechanisms of relaxation processes in the low-frequency (linear dispersion) and mid-frequency regions, an additional term from the Debye formula was added to take into account the mixed polarization, and a term taking into account the damping factor was added for resonant-type polarization. The simulation was carried out with and without the conductivity taken into account. To take into account the contribution of conductivity to the dynamic dielectric response, the expression σ* = (ε″ + iε′)ε0ω was used. It is shown that the linear part of the frequency dependence in the range from 50 Hz to 1 MHz is equally well described both with and without conductivity. At the same time, the behavior of the dielectric response of piezoelectric ceramics in the high-frequency region, where resonance effects are observed, and the low-frequency region, where volume-charge polarization predominates, is much better described taking into account the contribution of conductivity to the dielectric response of the system.
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spelling doaj.art-da6b4629278c47fdbee1b754dc0dc65c2023-12-03T11:46:33ZrusTver State UniversityФизико-химические аспекты изучения кластеров, наноструктур и наноматериалов2226-44422658-43602023-12-011548149410.26456/pcascnn/2023.15.481Simulation of the dielectric response of piezoelectric ceramics N.E. Malysheva0E.V. Dyakova1O.V. Malyshkina2Military Academy of Air and Space Defence named after Marshal of the Soviet Union G.K. Zhukov, Tver, RussiaTver State University, Tver, RussiaTver State University, Tver, RussiaWe have analyzed the complex permittivity of a porous (10 volume % of pores) sodium-lithium niobate ceramic with the results of computer simulation. The calculation was based on the Cole–Cole formula, which took into account the presence of various mechanisms of relaxation processes in the low-frequency (linear dispersion) and mid-frequency regions, an additional term from the Debye formula was added to take into account the mixed polarization, and a term taking into account the damping factor was added for resonant-type polarization. The simulation was carried out with and without the conductivity taken into account. To take into account the contribution of conductivity to the dynamic dielectric response, the expression σ* = (ε″ + iε′)ε0ω was used. It is shown that the linear part of the frequency dependence in the range from 50 Hz to 1 MHz is equally well described both with and without conductivity. At the same time, the behavior of the dielectric response of piezoelectric ceramics in the high-frequency region, where resonance effects are observed, and the low-frequency region, where volume-charge polarization predominates, is much better described taking into account the contribution of conductivity to the dielectric response of the system. https://physchemaspects.ru/2023/doi-10-26456-pcascnn-2023-15-481/?lang=enpiezoelectric ceramicscomplex permittivitycomplex conductivitydielectric spectroscopy
spellingShingle N.E. Malysheva
E.V. Dyakova
O.V. Malyshkina
Simulation of the dielectric response of piezoelectric ceramics
Физико-химические аспекты изучения кластеров, наноструктур и наноматериалов
piezoelectric ceramics
complex permittivity
complex conductivity
dielectric spectroscopy
title Simulation of the dielectric response of piezoelectric ceramics
title_full Simulation of the dielectric response of piezoelectric ceramics
title_fullStr Simulation of the dielectric response of piezoelectric ceramics
title_full_unstemmed Simulation of the dielectric response of piezoelectric ceramics
title_short Simulation of the dielectric response of piezoelectric ceramics
title_sort simulation of the dielectric response of piezoelectric ceramics
topic piezoelectric ceramics
complex permittivity
complex conductivity
dielectric spectroscopy
url https://physchemaspects.ru/2023/doi-10-26456-pcascnn-2023-15-481/?lang=en
work_keys_str_mv AT nemalysheva simulationofthedielectricresponseofpiezoelectricceramics
AT evdyakova simulationofthedielectricresponseofpiezoelectricceramics
AT ovmalyshkina simulationofthedielectricresponseofpiezoelectricceramics