Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface

Nanostructured plasmonic surfaces have been the subject of many biosensing applications exploiting surface-enhanced fluorescence in the last few years. For this reason, we investigated the refractive index dependence of the coupling mechanism between the plasmonic modes and the fluorescence processe...

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Main Authors: Francesco Floris, Margherita Angelini, Eliana Manobianco, Paola Pellacani, Franco Marabelli
Format: Article
Language:English
Published: MDPI AG 2023-05-01
Series:Materials Proceedings
Subjects:
Online Access:https://www.mdpi.com/2673-4605/14/1/41
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author Francesco Floris
Margherita Angelini
Eliana Manobianco
Paola Pellacani
Franco Marabelli
author_facet Francesco Floris
Margherita Angelini
Eliana Manobianco
Paola Pellacani
Franco Marabelli
author_sort Francesco Floris
collection DOAJ
description Nanostructured plasmonic surfaces have been the subject of many biosensing applications exploiting surface-enhanced fluorescence in the last few years. For this reason, we investigated the refractive index dependence of the coupling mechanism between the plasmonic modes and the fluorescence processes. The results show that the fluorescence emission spectral shape is controlled by the plasmonic field distribution, together with the enhancement of its signal. By altering the refractive index at the plasmonic active surface, the resonance conditions of the plasmonic modes change, resulting in a reshaping of fluorescence emission and a different spectral distribution of the largest enhancement regions.
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spelling doaj.art-db1dd64ef5d845a3ad0bb1783793fd772023-11-19T11:46:55ZengMDPI AGMaterials Proceedings2673-46052023-05-011414110.3390/IOCN2023-14529Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic SurfaceFrancesco Floris0Margherita Angelini1Eliana Manobianco2Paola Pellacani3Franco Marabelli4Department of Physics, University of Pavia, Via Bassi 6, 27100 Pavia, ItalyDepartment of Physics, University of Pavia, Via Bassi 6, 27100 Pavia, ItalyPlasmore S.r.l, Via Vittorio Emanuele II 4, 27100 Pavia, ItalyPlasmore S.r.l, Via Vittorio Emanuele II 4, 27100 Pavia, ItalyDepartment of Physics, University of Pavia, Via Bassi 6, 27100 Pavia, ItalyNanostructured plasmonic surfaces have been the subject of many biosensing applications exploiting surface-enhanced fluorescence in the last few years. For this reason, we investigated the refractive index dependence of the coupling mechanism between the plasmonic modes and the fluorescence processes. The results show that the fluorescence emission spectral shape is controlled by the plasmonic field distribution, together with the enhancement of its signal. By altering the refractive index at the plasmonic active surface, the resonance conditions of the plasmonic modes change, resulting in a reshaping of fluorescence emission and a different spectral distribution of the largest enhancement regions.https://www.mdpi.com/2673-4605/14/1/41fluorescencesurface plasmon resonanceelectric field coupling mechanismoptical characterizationFDTD simulation
spellingShingle Francesco Floris
Margherita Angelini
Eliana Manobianco
Paola Pellacani
Franco Marabelli
Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
Materials Proceedings
fluorescence
surface plasmon resonance
electric field coupling mechanism
optical characterization
FDTD simulation
title Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
title_full Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
title_fullStr Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
title_full_unstemmed Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
title_short Fluorescence Enhancement Dependence on Refractive Index Variation in a Nanostructured Plasmonic Surface
title_sort fluorescence enhancement dependence on refractive index variation in a nanostructured plasmonic surface
topic fluorescence
surface plasmon resonance
electric field coupling mechanism
optical characterization
FDTD simulation
url https://www.mdpi.com/2673-4605/14/1/41
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AT elianamanobianco fluorescenceenhancementdependenceonrefractiveindexvariationinananostructuredplasmonicsurface
AT paolapellacani fluorescenceenhancementdependenceonrefractiveindexvariationinananostructuredplasmonicsurface
AT francomarabelli fluorescenceenhancementdependenceonrefractiveindexvariationinananostructuredplasmonicsurface