One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model

Non-thermal plasma (NTP) technologies can be used to treat a variety of gaseous pollutants, and extensive research has been carried out worldwide because of its high purification efficiency, low dependence on temperature, and other advantages. NO and SO<sub>2</sub> are the main gaseous p...

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Main Authors: Chao Zhang, Lixin Yang
Format: Article
Language:English
Published: MDPI AG 2018-11-01
Series:Energies
Subjects:
Online Access:https://www.mdpi.com/1996-1073/11/12/3249
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author Chao Zhang
Lixin Yang
author_facet Chao Zhang
Lixin Yang
author_sort Chao Zhang
collection DOAJ
description Non-thermal plasma (NTP) technologies can be used to treat a variety of gaseous pollutants, and extensive research has been carried out worldwide because of its high purification efficiency, low dependence on temperature, and other advantages. NO and SO<sub>2</sub> are the main gaseous pollutants in coal-fired flue gas. The plasma dynamics for desulfurization and denitrification is a hot topic in the field of NTP pollutant control technologies. In this paper, a one-dimensional fluid model for the simultaneous desulfurization and denitrification of flue gas by negative direct current (DC) corona discharge was established based on the traditional zero-dimensional chemical kinetic model. The simplified wire-cylindrical electrodes configuration and numerical simulation conditions are similar to the working process of electrostatic precipitators. The results obtained by the finite element method show that the removal efficiency of NO and SO<sub>2</sub> is remarkable in the region with a radius of less than one centimeter around the high-voltage electrode, and the effective purification area expands with the increase of the discharge voltage. There are different removal pathways for NO at different positions in the removal region, while the removal of SO<sub>2</sub> is mainly dependent on the oxidation by OH.
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spelling doaj.art-dc11db02d9ea41f4ac80304f973940992022-12-22T02:54:10ZengMDPI AGEnergies1996-10732018-11-011112324910.3390/en11123249en11123249One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid ModelChao Zhang0Lixin Yang1Beijing Key Laboratory of Flow and Heat Transfer of Phase Changing in Micro and Small Scale, Beijing Jiaotong University, Beijing 100044, ChinaBeijing Key Laboratory of Flow and Heat Transfer of Phase Changing in Micro and Small Scale, Beijing Jiaotong University, Beijing 100044, ChinaNon-thermal plasma (NTP) technologies can be used to treat a variety of gaseous pollutants, and extensive research has been carried out worldwide because of its high purification efficiency, low dependence on temperature, and other advantages. NO and SO<sub>2</sub> are the main gaseous pollutants in coal-fired flue gas. The plasma dynamics for desulfurization and denitrification is a hot topic in the field of NTP pollutant control technologies. In this paper, a one-dimensional fluid model for the simultaneous desulfurization and denitrification of flue gas by negative direct current (DC) corona discharge was established based on the traditional zero-dimensional chemical kinetic model. The simplified wire-cylindrical electrodes configuration and numerical simulation conditions are similar to the working process of electrostatic precipitators. The results obtained by the finite element method show that the removal efficiency of NO and SO<sub>2</sub> is remarkable in the region with a radius of less than one centimeter around the high-voltage electrode, and the effective purification area expands with the increase of the discharge voltage. There are different removal pathways for NO at different positions in the removal region, while the removal of SO<sub>2</sub> is mainly dependent on the oxidation by OH.https://www.mdpi.com/1996-1073/11/12/3249one-dimensional fluid modelchemical kinetic modelnon-thermal plasmadesulfurizationdenitrification
spellingShingle Chao Zhang
Lixin Yang
One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
Energies
one-dimensional fluid model
chemical kinetic model
non-thermal plasma
desulfurization
denitrification
title One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
title_full One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
title_fullStr One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
title_full_unstemmed One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
title_short One-Dimensional Simulation of Synergistic Desulfurization and Denitrification Processes for Electrostatic Precipitators Based on a Fluid-Chemical Reaction Hybrid Model
title_sort one dimensional simulation of synergistic desulfurization and denitrification processes for electrostatic precipitators based on a fluid chemical reaction hybrid model
topic one-dimensional fluid model
chemical kinetic model
non-thermal plasma
desulfurization
denitrification
url https://www.mdpi.com/1996-1073/11/12/3249
work_keys_str_mv AT chaozhang onedimensionalsimulationofsynergisticdesulfurizationanddenitrificationprocessesforelectrostaticprecipitatorsbasedonafluidchemicalreactionhybridmodel
AT lixinyang onedimensionalsimulationofsynergisticdesulfurizationanddenitrificationprocessesforelectrostaticprecipitatorsbasedonafluidchemicalreactionhybridmodel