Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy

We demonstrate large nonlinear terahertz responses in the gaps of metamaterial split ring resonators in several materials and use nonlinear THz transmission and THz-pump/THz-probe spectroscopy to study the nonlinear responses and dynamics. We use the field enhancement in the SRR gaps to initiate hig...

Full description

Bibliographic Details
Main Authors: Zhang X., Perkins B. G., Brandt N. C., Sternbach A., Strikwerda A. C., Zhang J., Fan K., Liu M., Hwang H. Y., Averitt R. D., Nelson K. A.
Format: Article
Language:English
Published: EDP Sciences 2013-03-01
Series:EPJ Web of Conferences
Online Access:http://dx.doi.org/10.1051/epjconf/20134109005
_version_ 1818892827392737280
author Zhang X.
Perkins B. G.
Brandt N. C.
Sternbach A.
Strikwerda A. C.
Zhang J.
Fan K.
Liu M.
Hwang H. Y.
Averitt R. D.
Nelson K. A.
author_facet Zhang X.
Perkins B. G.
Brandt N. C.
Sternbach A.
Strikwerda A. C.
Zhang J.
Fan K.
Liu M.
Hwang H. Y.
Averitt R. D.
Nelson K. A.
author_sort Zhang X.
collection DOAJ
description We demonstrate large nonlinear terahertz responses in the gaps of metamaterial split ring resonators in several materials and use nonlinear THz transmission and THz-pump/THz-probe spectroscopy to study the nonlinear responses and dynamics. We use the field enhancement in the SRR gaps to initiate high-field phenomena at lower incident fields. In vanadium dioxide, we drive the insulator-to-metal phase transition with high-field THz radiation. The film conductivity increases by over two orders of magnitude and the phase transition occurs on a several picosecond timescale. In gallium arsenide, we observe high-field transport phenomena, including mobility saturation and impact ionization. The carrier density increases by up to ten orders of magnitude at high fields. At the highest fields, we demonstrate THz-induced damage in both vanadium dioxide and gallium arsenide.
first_indexed 2024-12-19T18:02:53Z
format Article
id doaj.art-dc7b77970f7144afa274f1a7185cde3e
institution Directory Open Access Journal
issn 2100-014X
language English
last_indexed 2024-12-19T18:02:53Z
publishDate 2013-03-01
publisher EDP Sciences
record_format Article
series EPJ Web of Conferences
spelling doaj.art-dc7b77970f7144afa274f1a7185cde3e2022-12-21T20:11:33ZengEDP SciencesEPJ Web of Conferences2100-014X2013-03-01410900510.1051/epjconf/20134109005Metamaterial-Enhanced Nonlinear Terahertz SpectroscopyZhang X.Perkins B. G.Brandt N. C.Sternbach A.Strikwerda A. C.Zhang J.Fan K.Liu M.Hwang H. Y.Averitt R. D.Nelson K. A.We demonstrate large nonlinear terahertz responses in the gaps of metamaterial split ring resonators in several materials and use nonlinear THz transmission and THz-pump/THz-probe spectroscopy to study the nonlinear responses and dynamics. We use the field enhancement in the SRR gaps to initiate high-field phenomena at lower incident fields. In vanadium dioxide, we drive the insulator-to-metal phase transition with high-field THz radiation. The film conductivity increases by over two orders of magnitude and the phase transition occurs on a several picosecond timescale. In gallium arsenide, we observe high-field transport phenomena, including mobility saturation and impact ionization. The carrier density increases by up to ten orders of magnitude at high fields. At the highest fields, we demonstrate THz-induced damage in both vanadium dioxide and gallium arsenide.http://dx.doi.org/10.1051/epjconf/20134109005
spellingShingle Zhang X.
Perkins B. G.
Brandt N. C.
Sternbach A.
Strikwerda A. C.
Zhang J.
Fan K.
Liu M.
Hwang H. Y.
Averitt R. D.
Nelson K. A.
Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
EPJ Web of Conferences
title Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
title_full Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
title_fullStr Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
title_full_unstemmed Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
title_short Metamaterial-Enhanced Nonlinear Terahertz Spectroscopy
title_sort metamaterial enhanced nonlinear terahertz spectroscopy
url http://dx.doi.org/10.1051/epjconf/20134109005
work_keys_str_mv AT zhangx metamaterialenhancednonlinearterahertzspectroscopy
AT perkinsbg metamaterialenhancednonlinearterahertzspectroscopy
AT brandtnc metamaterialenhancednonlinearterahertzspectroscopy
AT sternbacha metamaterialenhancednonlinearterahertzspectroscopy
AT strikwerdaac metamaterialenhancednonlinearterahertzspectroscopy
AT zhangj metamaterialenhancednonlinearterahertzspectroscopy
AT fank metamaterialenhancednonlinearterahertzspectroscopy
AT lium metamaterialenhancednonlinearterahertzspectroscopy
AT hwanghy metamaterialenhancednonlinearterahertzspectroscopy
AT averittrd metamaterialenhancednonlinearterahertzspectroscopy
AT nelsonka metamaterialenhancednonlinearterahertzspectroscopy