Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons
Vibration-cavity polaritons are mixed states produced by strong coupling between a vibrational mode and an optical cavity. Here, the authors show that these polaritons can coherently exchange energy and exhibit drastically altered transient spectra and dynamics compared to uncoupled vibrations.
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Format: | Article |
Language: | English |
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Nature Portfolio
2016-11-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/ncomms13504 |
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author | A. D. Dunkelberger B. T. Spann K. P. Fears B. S. Simpkins J. C. Owrutsky |
author_facet | A. D. Dunkelberger B. T. Spann K. P. Fears B. S. Simpkins J. C. Owrutsky |
author_sort | A. D. Dunkelberger |
collection | DOAJ |
description | Vibration-cavity polaritons are mixed states produced by strong coupling between a vibrational mode and an optical cavity. Here, the authors show that these polaritons can coherently exchange energy and exhibit drastically altered transient spectra and dynamics compared to uncoupled vibrations. |
first_indexed | 2024-12-23T02:01:26Z |
format | Article |
id | doaj.art-ded2189e558547ebbb6d70804ede8c4f |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-23T02:01:26Z |
publishDate | 2016-11-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-ded2189e558547ebbb6d70804ede8c4f2022-12-21T18:03:58ZengNature PortfolioNature Communications2041-17232016-11-017111010.1038/ncomms13504Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritonsA. D. Dunkelberger0B. T. Spann1K. P. Fears2B. S. Simpkins3J. C. Owrutsky4Chemistry Division, National Research Council Postdoctoral Associate, U. S. Naval Research Laboratory, Washington, District of ColumbiaChemistry Division, National Research Council Postdoctoral Associate, U. S. Naval Research Laboratory, Washington, District of ColumbiaChemistry Division, Naval Research LaboratoryChemistry Division, Naval Research LaboratoryChemistry Division, Naval Research LaboratoryVibration-cavity polaritons are mixed states produced by strong coupling between a vibrational mode and an optical cavity. Here, the authors show that these polaritons can coherently exchange energy and exhibit drastically altered transient spectra and dynamics compared to uncoupled vibrations.https://doi.org/10.1038/ncomms13504 |
spellingShingle | A. D. Dunkelberger B. T. Spann K. P. Fears B. S. Simpkins J. C. Owrutsky Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons Nature Communications |
title | Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons |
title_full | Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons |
title_fullStr | Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons |
title_full_unstemmed | Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons |
title_short | Modified relaxation dynamics and coherent energy exchange in coupled vibration-cavity polaritons |
title_sort | modified relaxation dynamics and coherent energy exchange in coupled vibration cavity polaritons |
url | https://doi.org/10.1038/ncomms13504 |
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