Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic

This study was carried out to provide a novel solution to treat drinking water at household levels, specifically removing arsenic (As) and faecal coliforms (microbes). In the current investigation, a synergistic iron-loaded zeolites and ozonation process (O<sub>3</sub>/Fe-ZA) was used fo...

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Main Authors: Amir Ikhlaq, Rida Fatima, Umair Yaqub Qazi, Rahat Javaid, Asia Akram, Sami Ibn Shamsah, Fei Qi
Format: Article
Language:English
Published: MDPI AG 2021-03-01
Series:Catalysts
Subjects:
Online Access:https://www.mdpi.com/2073-4344/11/3/373
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author Amir Ikhlaq
Rida Fatima
Umair Yaqub Qazi
Rahat Javaid
Asia Akram
Sami Ibn Shamsah
Fei Qi
author_facet Amir Ikhlaq
Rida Fatima
Umair Yaqub Qazi
Rahat Javaid
Asia Akram
Sami Ibn Shamsah
Fei Qi
author_sort Amir Ikhlaq
collection DOAJ
description This study was carried out to provide a novel solution to treat drinking water at household levels, specifically removing arsenic (As) and faecal coliforms (microbes). In the current investigation, a synergistic iron-loaded zeolites and ozonation process (O<sub>3</sub>/Fe-ZA) was used for the first time in a modified batch reactor to remove coliform bacteria and arsenic in tap water. Moreover, the study utilizes the human health risk assessment model to confirm the health risk due to As intake in drinking water. The risk assessment study revealed a health risk threat among the residents suffering from the adverse effects of As through its intake in drinking water. Furthermore, the results also suggested that the O<sub>3</sub>/Fe-ZA process significantly removes faecal coliforms and As, when compared with single ozonation processes. Additionally, the ozone dose 0.2 mg/min and Fe-ZA dose of 10 g (in the O<sub>3</sub>/Fe-ZA process) gives the maximum removal efficiency of 100% within 15 min for faecal coliform removal. In 30 min, the removal efficiency of 88.4% was achieved at the ozone dose of 0.5 mg/min and 93% removal efficiency was achieved using 10 g Fe-ZA for the removal of As in the O<sub>3</sub>/Fe-ZA process. Hence, it was concluded that the O<sub>3</sub>/Fe-ZA process may be regarded as an effective method for removing faecal coliforms and As from drinking water compared to the single ozonation processes.
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spelling doaj.art-def3d55ad63d4393b0bd00761cb67e4e2023-11-21T10:12:02ZengMDPI AGCatalysts2073-43442021-03-0111337310.3390/catal11030373Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and ArsenicAmir Ikhlaq0Rida Fatima1Umair Yaqub Qazi2Rahat Javaid3Asia Akram4Sami Ibn Shamsah5Fei Qi6Institute of Environmental Engineering and Research, University of Engineering and Technology, Lahore 54890, PakistanInstitute of Environmental Engineering and Research, University of Engineering and Technology, Lahore 54890, PakistanDepartment of Chemistry, College of Science, University of Hafr Al Batin, Hafr Al Batin 39524, Saudi ArabiaRenewable Energy Research Center, Fukushima Renewable Energy Institute, National Institute of Advanced Industrial Science and Technology, Koriyama 963-0298, JapanDepartment of Chemistry, University of Management and Technology, Johar Town, Lahore 54770, PakistanDepartment of Mechanical Engineering, College of Engineering, University of Hafr Al Batin, Hafr Al Batin 31991, Saudi ArabiaBeijing Key Lab for Source Control Technology of Water Pollution, College of Environmental Science and Engineering, Beijing Forestry University, Beijing 100083, ChinaThis study was carried out to provide a novel solution to treat drinking water at household levels, specifically removing arsenic (As) and faecal coliforms (microbes). In the current investigation, a synergistic iron-loaded zeolites and ozonation process (O<sub>3</sub>/Fe-ZA) was used for the first time in a modified batch reactor to remove coliform bacteria and arsenic in tap water. Moreover, the study utilizes the human health risk assessment model to confirm the health risk due to As intake in drinking water. The risk assessment study revealed a health risk threat among the residents suffering from the adverse effects of As through its intake in drinking water. Furthermore, the results also suggested that the O<sub>3</sub>/Fe-ZA process significantly removes faecal coliforms and As, when compared with single ozonation processes. Additionally, the ozone dose 0.2 mg/min and Fe-ZA dose of 10 g (in the O<sub>3</sub>/Fe-ZA process) gives the maximum removal efficiency of 100% within 15 min for faecal coliform removal. In 30 min, the removal efficiency of 88.4% was achieved at the ozone dose of 0.5 mg/min and 93% removal efficiency was achieved using 10 g Fe-ZA for the removal of As in the O<sub>3</sub>/Fe-ZA process. Hence, it was concluded that the O<sub>3</sub>/Fe-ZA process may be regarded as an effective method for removing faecal coliforms and As from drinking water compared to the single ozonation processes.https://www.mdpi.com/2073-4344/11/3/373arsenicfaecal coliformsozonationFe-Zeolite Adrinking water
spellingShingle Amir Ikhlaq
Rida Fatima
Umair Yaqub Qazi
Rahat Javaid
Asia Akram
Sami Ibn Shamsah
Fei Qi
Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
Catalysts
arsenic
faecal coliforms
ozonation
Fe-Zeolite A
drinking water
title Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
title_full Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
title_fullStr Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
title_full_unstemmed Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
title_short Combined Iron-Loaded Zeolites and Ozone-Based Process for the Purification of Drinking Water in a Novel Hybrid Reactor: Removal of Faecal Coliforms and Arsenic
title_sort combined iron loaded zeolites and ozone based process for the purification of drinking water in a novel hybrid reactor removal of faecal coliforms and arsenic
topic arsenic
faecal coliforms
ozonation
Fe-Zeolite A
drinking water
url https://www.mdpi.com/2073-4344/11/3/373
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