Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS

We demonstrate that the conductivity of graphene on thin-film polymer substrates can be accurately determined by reflection-mode air-plasma-based THz time-domain spectroscopy (THz-TDS). The phase uncertainty issue associated with reflection measurements is discussed, and our implementation is valida...

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Main Authors: Binbin Zhou, Mattias Rasmussen, Patrick Rebsdorf Whelan, Jie Ji, Abhay Shivayogimath, Peter Bøggild, Peter Uhd Jepsen
Format: Article
Language:English
Published: MDPI AG 2023-03-01
Series:Sensors
Subjects:
Online Access:https://www.mdpi.com/1424-8220/23/7/3669
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author Binbin Zhou
Mattias Rasmussen
Patrick Rebsdorf Whelan
Jie Ji
Abhay Shivayogimath
Peter Bøggild
Peter Uhd Jepsen
author_facet Binbin Zhou
Mattias Rasmussen
Patrick Rebsdorf Whelan
Jie Ji
Abhay Shivayogimath
Peter Bøggild
Peter Uhd Jepsen
author_sort Binbin Zhou
collection DOAJ
description We demonstrate that the conductivity of graphene on thin-film polymer substrates can be accurately determined by reflection-mode air-plasma-based THz time-domain spectroscopy (THz-TDS). The phase uncertainty issue associated with reflection measurements is discussed, and our implementation is validated by convincing agreement with graphene electrical properties extracted from more conventional transmission-mode measurements. Both the reflection and transmission THz-TDS measurements reveal strong non-linear and instantaneous conductivity depletion across an ultra-broad bandwidth (1–9 THz) under relatively high incident THz electrical field strengths (up to 1050 kV/cm).
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spelling doaj.art-df473ef79d58425e92888212d18015ec2023-11-17T17:35:59ZengMDPI AGSensors1424-82202023-03-01237366910.3390/s23073669Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDSBinbin Zhou0Mattias Rasmussen1Patrick Rebsdorf Whelan2Jie Ji3Abhay Shivayogimath4Peter Bøggild5Peter Uhd Jepsen6Department of Electrical and Photonics Engineering, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Electrical and Photonics Engineering, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Physics, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Physics, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Physics, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Physics, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkDepartment of Electrical and Photonics Engineering, Technical University of Denmark, 2800 Kongens Lyngby, DenmarkWe demonstrate that the conductivity of graphene on thin-film polymer substrates can be accurately determined by reflection-mode air-plasma-based THz time-domain spectroscopy (THz-TDS). The phase uncertainty issue associated with reflection measurements is discussed, and our implementation is validated by convincing agreement with graphene electrical properties extracted from more conventional transmission-mode measurements. Both the reflection and transmission THz-TDS measurements reveal strong non-linear and instantaneous conductivity depletion across an ultra-broad bandwidth (1–9 THz) under relatively high incident THz electrical field strengths (up to 1050 kV/cm).https://www.mdpi.com/1424-8220/23/7/3669grapheneAC conductivityTHz time-domain spectroscopyreflection spectroscopy
spellingShingle Binbin Zhou
Mattias Rasmussen
Patrick Rebsdorf Whelan
Jie Ji
Abhay Shivayogimath
Peter Bøggild
Peter Uhd Jepsen
Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
Sensors
graphene
AC conductivity
THz time-domain spectroscopy
reflection spectroscopy
title Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
title_full Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
title_fullStr Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
title_full_unstemmed Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
title_short Non-Linear Conductivity Response of Graphene on Thin-Film PET Characterized by Transmission and Reflection Air-Plasma THz-TDS
title_sort non linear conductivity response of graphene on thin film pet characterized by transmission and reflection air plasma thz tds
topic graphene
AC conductivity
THz time-domain spectroscopy
reflection spectroscopy
url https://www.mdpi.com/1424-8220/23/7/3669
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