Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)

While water and sulfuric acid droplets are the main component of stratospheric aerosols, measurements performed for about 30 years have shown that non-sulfate particles (NSPs) are also present. Such particles, released from the Earth mainly through volcanic eruptions, pollution or biomass burning, o...

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Main Authors: Jean-Baptiste Renard, Gwenaël Berthet, Anny-Chantal Levasseur-Regourd, Sergey Beresnev, Alain Miffre, Patrick Rairoux, Damien Vignelles, Fabrice Jégou
Format: Article
Language:English
Published: MDPI AG 2020-09-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/11/10/1031
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author Jean-Baptiste Renard
Gwenaël Berthet
Anny-Chantal Levasseur-Regourd
Sergey Beresnev
Alain Miffre
Patrick Rairoux
Damien Vignelles
Fabrice Jégou
author_facet Jean-Baptiste Renard
Gwenaël Berthet
Anny-Chantal Levasseur-Regourd
Sergey Beresnev
Alain Miffre
Patrick Rairoux
Damien Vignelles
Fabrice Jégou
author_sort Jean-Baptiste Renard
collection DOAJ
description While water and sulfuric acid droplets are the main component of stratospheric aerosols, measurements performed for about 30 years have shown that non-sulfate particles (NSPs) are also present. Such particles, released from the Earth mainly through volcanic eruptions, pollution or biomass burning, or coming from space, present a wide variety of compositions, sizes, and shapes. To better understand the origin of NSPs, we have performed measurements with the Light Optical Aerosol Counter (LOAC) during 151 flights under weather balloons in the 2013–2019 period reaching altitudes up to 35 km. Coupled with previous counting measurements conducted over the 2004–2011 period, the LOAC measurements indicate the presence of stratospheric layers of enhanced concentrations associated with NSPs, with a bimodal vertical repartition ranging between 17 and 30 km altitude. Such enhancements are not correlated with permanent meteor shower events. They may be linked to dynamical and photophoretic effects lifting and sustaining particles coming from the Earth. Besides, large particles, up to several tens of μm, were detected and present decreasing concentrations with increasing altitudes. All these particles can originate from Earth but also from meteoroid disintegrations and from the interplanetary dust cloud and comets.
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spelling doaj.art-df5b52a19db74e3cada13c6190e31d662023-11-20T15:04:27ZengMDPI AGAtmosphere2073-44332020-09-011110103110.3390/atmos11101031Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)Jean-Baptiste Renard0Gwenaël Berthet1Anny-Chantal Levasseur-Regourd2Sergey Beresnev3Alain Miffre4Patrick Rairoux5Damien Vignelles6Fabrice Jégou7LPC2E-CNRS-CNES, F-45071 Orléans, FranceLPC2E-CNRS-CNES, F-45071 Orléans, FranceLATMOS-CNRS-CNES, Campus Pierre et Marie Curie, Sorbonne Université, F-75252 Paris, FranceInstitute of Natural Sciences and Mathematics, Ural Federal University, 620083 Ekaterinburg, RussiaInstitut Lumière Matière, University Claude Bernard Lyon 1, CNRS, F-69622 Villeurbanne, FranceInstitut Lumière Matière, University Claude Bernard Lyon 1, CNRS, F-69622 Villeurbanne, FranceLPC2E-CNRS-CNES, F-45071 Orléans, FranceLPC2E-CNRS-CNES, F-45071 Orléans, FranceWhile water and sulfuric acid droplets are the main component of stratospheric aerosols, measurements performed for about 30 years have shown that non-sulfate particles (NSPs) are also present. Such particles, released from the Earth mainly through volcanic eruptions, pollution or biomass burning, or coming from space, present a wide variety of compositions, sizes, and shapes. To better understand the origin of NSPs, we have performed measurements with the Light Optical Aerosol Counter (LOAC) during 151 flights under weather balloons in the 2013–2019 period reaching altitudes up to 35 km. Coupled with previous counting measurements conducted over the 2004–2011 period, the LOAC measurements indicate the presence of stratospheric layers of enhanced concentrations associated with NSPs, with a bimodal vertical repartition ranging between 17 and 30 km altitude. Such enhancements are not correlated with permanent meteor shower events. They may be linked to dynamical and photophoretic effects lifting and sustaining particles coming from the Earth. Besides, large particles, up to several tens of μm, were detected and present decreasing concentrations with increasing altitudes. All these particles can originate from Earth but also from meteoroid disintegrations and from the interplanetary dust cloud and comets.https://www.mdpi.com/2073-4433/11/10/1031non-sulfate stratospheric aerosolscountingtypologyballoon
spellingShingle Jean-Baptiste Renard
Gwenaël Berthet
Anny-Chantal Levasseur-Regourd
Sergey Beresnev
Alain Miffre
Patrick Rairoux
Damien Vignelles
Fabrice Jégou
Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
Atmosphere
non-sulfate stratospheric aerosols
counting
typology
balloon
title Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
title_full Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
title_fullStr Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
title_full_unstemmed Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
title_short Origins and Spatial Distribution of Non-Pure Sulfate Particles (NSPs) in the Stratosphere Detected by the Balloon-Borne Light Optical Aerosols Counter (LOAC)
title_sort origins and spatial distribution of non pure sulfate particles nsps in the stratosphere detected by the balloon borne light optical aerosols counter loac
topic non-sulfate stratospheric aerosols
counting
typology
balloon
url https://www.mdpi.com/2073-4433/11/10/1031
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