Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}

Here, we propose an idea to realize noncollinear ferrimagnetic orders with a considerably high magnetization M and their coupling with an improper ferroelectric (FE) order in hexagonal LuFeO_{3} type systems which exhibit interesting topological orders. These magnetic and magnetoelectric phenomena a...

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Main Author: Hena Das
Format: Article
Language:English
Published: American Physical Society 2023-01-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.5.013007
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author Hena Das
author_facet Hena Das
author_sort Hena Das
collection DOAJ
description Here, we propose an idea to realize noncollinear ferrimagnetic orders with a considerably high magnetization M and their coupling with an improper ferroelectric (FE) order in hexagonal LuFeO_{3} type systems which exhibit interesting topological orders. These magnetic and magnetoelectric phenomena are driven by the antisymmetric Dzyaloshinskii-Moriya interactions between the magnetic ions and their coupling with the ferroelectricity. The proposed two-sublattice magnetic system, generated by a specific charge-ordered state, forms multiple energetically close, noncollinear ferrimagnetic orders. This offers a platform to manipulate the microscopic magnetic interactions and to trigger spin-reorientation (SR) transitions by various efficient means. The two-sublattice structure was realized in the hexagonal phase of LuFeO_{3} doped with electrons. The proposed electron-doped systems are expected to exhibit switchable electric polarization (P∼6–15 μC/cm^{2}), considerably high magnetization (M∼1.1–1.3μ_{B}/Fe), and magnetic transition near room temperature (∼275–290K). Based on the coupling between the magnetic interactions and the FE primary order parameter observed in this system, microscopic mechanisms to achieve electric field E induced SR transitions and 180^{∘} switching of the direction of M are discussed.
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spelling doaj.art-dfa595d2d1fa4f7485a158f4225efe7c2024-04-12T17:27:28ZengAmerican Physical SocietyPhysical Review Research2643-15642023-01-015101300710.1103/PhysRevResearch.5.013007Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}Hena DasHere, we propose an idea to realize noncollinear ferrimagnetic orders with a considerably high magnetization M and their coupling with an improper ferroelectric (FE) order in hexagonal LuFeO_{3} type systems which exhibit interesting topological orders. These magnetic and magnetoelectric phenomena are driven by the antisymmetric Dzyaloshinskii-Moriya interactions between the magnetic ions and their coupling with the ferroelectricity. The proposed two-sublattice magnetic system, generated by a specific charge-ordered state, forms multiple energetically close, noncollinear ferrimagnetic orders. This offers a platform to manipulate the microscopic magnetic interactions and to trigger spin-reorientation (SR) transitions by various efficient means. The two-sublattice structure was realized in the hexagonal phase of LuFeO_{3} doped with electrons. The proposed electron-doped systems are expected to exhibit switchable electric polarization (P∼6–15 μC/cm^{2}), considerably high magnetization (M∼1.1–1.3μ_{B}/Fe), and magnetic transition near room temperature (∼275–290K). Based on the coupling between the magnetic interactions and the FE primary order parameter observed in this system, microscopic mechanisms to achieve electric field E induced SR transitions and 180^{∘} switching of the direction of M are discussed.http://doi.org/10.1103/PhysRevResearch.5.013007
spellingShingle Hena Das
Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
Physical Review Research
title Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
title_full Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
title_fullStr Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
title_full_unstemmed Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
title_short Coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite LuFeO_{3}
title_sort coupling between improper ferroelectricity and ferrimagnetism in the hexagonal ferrite lufeo 3
url http://doi.org/10.1103/PhysRevResearch.5.013007
work_keys_str_mv AT henadas couplingbetweenimproperferroelectricityandferrimagnetisminthehexagonalferritelufeo3