Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles

Emerging as a light, flexible and highly thermally conductive material, graphene-based membranes have attracted extensive attention in thermal management field. However, the preparation of high-quality graphene-based membranes usually involves complex processes and thermal annealing at ultra-high te...

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Main Authors: Jing Li, Jialiang Liu, Jinshui Liu, Jinfeng Lai, Yuxun Chen, Wenjun Li
Format: Article
Language:English
Published: MDPI AG 2021-12-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/11/12/3392
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author Jing Li
Jialiang Liu
Jinshui Liu
Jinfeng Lai
Yuxun Chen
Wenjun Li
author_facet Jing Li
Jialiang Liu
Jinshui Liu
Jinfeng Lai
Yuxun Chen
Wenjun Li
author_sort Jing Li
collection DOAJ
description Emerging as a light, flexible and highly thermally conductive material, graphene-based membranes have attracted extensive attention in thermal management field. However, the preparation of high-quality graphene-based membranes usually involves complex processes and thermal annealing at ultra-high temperature, which limits their large-scale application in thermal management field. In our study, reduced graphene oxide-Ni-hydroxypropyl methyl cellulose (RGO-Ni-HPMC) composite membrane was prepared from catalytic pyrolysis of hydroxypropyl methyl cellulose (HPMC) with Ni nanoparticles to generate multilayer graphene and form phonon transport channels between adjacent graphene layers. Further, our study shows that the RGO-Ni-HPMC composite membrane has a good heat dissipation effect at the hot spots at high temperature. The average temperature of hot spots is reduced by 11.5 °C. It is expected to solve the heat dissipation problem of high-power electronic equipment.
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spelling doaj.art-e0e1e9e9216a4ffbaf4a19e4c77b62702023-11-23T09:51:58ZengMDPI AGNanomaterials2079-49912021-12-011112339210.3390/nano11123392Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni NanoparticlesJing Li0Jialiang Liu1Jinshui Liu2Jinfeng Lai3Yuxun Chen4Wenjun Li5School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, ChinaSchool of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, ChinaSchool of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, ChinaSchool of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, ChinaSchool of Mechanical and Automotive Engineering, South China University of Technology, Guangzhou 510641, ChinaBeijing Headquarters of Space Vehicle, Beijing 100086, ChinaEmerging as a light, flexible and highly thermally conductive material, graphene-based membranes have attracted extensive attention in thermal management field. However, the preparation of high-quality graphene-based membranes usually involves complex processes and thermal annealing at ultra-high temperature, which limits their large-scale application in thermal management field. In our study, reduced graphene oxide-Ni-hydroxypropyl methyl cellulose (RGO-Ni-HPMC) composite membrane was prepared from catalytic pyrolysis of hydroxypropyl methyl cellulose (HPMC) with Ni nanoparticles to generate multilayer graphene and form phonon transport channels between adjacent graphene layers. Further, our study shows that the RGO-Ni-HPMC composite membrane has a good heat dissipation effect at the hot spots at high temperature. The average temperature of hot spots is reduced by 11.5 °C. It is expected to solve the heat dissipation problem of high-power electronic equipment.https://www.mdpi.com/2079-4991/11/12/3392oxidized graphenethermal conductivityhydroxypropyl methyl celluloseNi nanoparticles
spellingShingle Jing Li
Jialiang Liu
Jinshui Liu
Jinfeng Lai
Yuxun Chen
Wenjun Li
Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
Nanomaterials
oxidized graphene
thermal conductivity
hydroxypropyl methyl cellulose
Ni nanoparticles
title Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
title_full Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
title_fullStr Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
title_full_unstemmed Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
title_short Graphene-Based Composite Membrane Prepared from Solid Carbon Source Catalyzed by Ni Nanoparticles
title_sort graphene based composite membrane prepared from solid carbon source catalyzed by ni nanoparticles
topic oxidized graphene
thermal conductivity
hydroxypropyl methyl cellulose
Ni nanoparticles
url https://www.mdpi.com/2079-4991/11/12/3392
work_keys_str_mv AT jingli graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles
AT jialiangliu graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles
AT jinshuiliu graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles
AT jinfenglai graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles
AT yuxunchen graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles
AT wenjunli graphenebasedcompositemembranepreparedfromsolidcarbonsourcecatalyzedbyninanoparticles