Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials

Abstract For pursuing the ambitious goals in the burgeoning electric vehicles, portable electronic devices, and energy storage sectors, Li‐ion batteries (LIBs) are considered as one of the most promising electrochemical power sources because of their high energy density and moderate cost. Particular...

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Main Authors: Yiyao Han, Xiaozheng Zhou, Ruyi Fang, Chengwei Lu, Kun Wang, Yongping Gan, Xinping He, Jun Zhang, Hui Huang, Wenkui Zhang, Xinhui Xia, Yang Xia
Format: Article
Language:English
Published: Wiley 2023-03-01
Series:Carbon Neutralization
Subjects:
Online Access:https://doi.org/10.1002/cnl2.49
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author Yiyao Han
Xiaozheng Zhou
Ruyi Fang
Chengwei Lu
Kun Wang
Yongping Gan
Xinping He
Jun Zhang
Hui Huang
Wenkui Zhang
Xinhui Xia
Yang Xia
author_facet Yiyao Han
Xiaozheng Zhou
Ruyi Fang
Chengwei Lu
Kun Wang
Yongping Gan
Xinping He
Jun Zhang
Hui Huang
Wenkui Zhang
Xinhui Xia
Yang Xia
author_sort Yiyao Han
collection DOAJ
description Abstract For pursuing the ambitious goals in the burgeoning electric vehicles, portable electronic devices, and energy storage sectors, Li‐ion batteries (LIBs) are considered as one of the most promising electrochemical power sources because of their high energy density and moderate cost. Particularly, the improvement of battery materials and recycling of spent LIBs are receiving great attention since the sustainable approaches for the synthesis, modification, and recycling of battery materials are the crucial factors to the successful large‐scale implementation of LIBs. In this regard, supercritical carbon dioxide (SC‐CO2), which possesses many merits, such as environmentally friendly, low‐cost, individual chemical environment, and especially its unique physical properties, has been employed as solvent and reaction medium in the synthesis and modification of diverse functional materials. In this review, we mainly aim at compiling the applications of SC‐CO2 technology in the synthesis and modification of electrode materials as well as the recycling of LIBs. First, the unique properties and principles of SC‐CO2 technology are highlighted. Second, the latest progresses of the electrode materials design and recycling with the assistance of SC‐CO2 technique are summarized. Finally, the challenges, future directions, and perspectives on the design and development of battery materials and battery recycling by SC‐CO2 technology are proposed.
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spelling doaj.art-e17238ed9b4b46d1a23901b9700fefdd2023-05-11T17:25:26ZengWileyCarbon Neutralization2769-33252023-03-012216918510.1002/cnl2.49Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materialsYiyao Han0Xiaozheng Zhou1Ruyi Fang2Chengwei Lu3Kun Wang4Yongping Gan5Xinping He6Jun Zhang7Hui Huang8Wenkui Zhang9Xinhui Xia10Yang Xia11College of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaCollege of Materials Science and Engineering Zhejiang University of Technology Hangzhou ChinaAbstract For pursuing the ambitious goals in the burgeoning electric vehicles, portable electronic devices, and energy storage sectors, Li‐ion batteries (LIBs) are considered as one of the most promising electrochemical power sources because of their high energy density and moderate cost. Particularly, the improvement of battery materials and recycling of spent LIBs are receiving great attention since the sustainable approaches for the synthesis, modification, and recycling of battery materials are the crucial factors to the successful large‐scale implementation of LIBs. In this regard, supercritical carbon dioxide (SC‐CO2), which possesses many merits, such as environmentally friendly, low‐cost, individual chemical environment, and especially its unique physical properties, has been employed as solvent and reaction medium in the synthesis and modification of diverse functional materials. In this review, we mainly aim at compiling the applications of SC‐CO2 technology in the synthesis and modification of electrode materials as well as the recycling of LIBs. First, the unique properties and principles of SC‐CO2 technology are highlighted. Second, the latest progresses of the electrode materials design and recycling with the assistance of SC‐CO2 technique are summarized. Finally, the challenges, future directions, and perspectives on the design and development of battery materials and battery recycling by SC‐CO2 technology are proposed.https://doi.org/10.1002/cnl2.49battery recyclingelectrode modificationlithium‐ion batteriesmaterials synthesissupercritical carbon dioxide
spellingShingle Yiyao Han
Xiaozheng Zhou
Ruyi Fang
Chengwei Lu
Kun Wang
Yongping Gan
Xinping He
Jun Zhang
Hui Huang
Wenkui Zhang
Xinhui Xia
Yang Xia
Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
Carbon Neutralization
battery recycling
electrode modification
lithium‐ion batteries
materials synthesis
supercritical carbon dioxide
title Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
title_full Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
title_fullStr Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
title_full_unstemmed Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
title_short Supercritical carbon dioxide technology in synthesis, modification, and recycling of battery materials
title_sort supercritical carbon dioxide technology in synthesis modification and recycling of battery materials
topic battery recycling
electrode modification
lithium‐ion batteries
materials synthesis
supercritical carbon dioxide
url https://doi.org/10.1002/cnl2.49
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