Epitaxial HfTe2 Dirac semimetal in the 2D limit

One monolayer semimetallic HfTe2 thin films are grown on three substrates with different electronic properties in order to study the substrate effect on the electronic structure of the HfTe2 epilayer. Angle resolved photoelectron spectroscopy measurements indicate that the band features are identica...

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Main Authors: Polychronis Tsipas, Panagiotis Pappas, Evgenia Symeonidou, Sotirios Fragkos, Christina Zacharaki, Evangelia Xenogiannopoulou, Nikitas Siannas, Athanasios Dimoulas
Format: Article
Language:English
Published: AIP Publishing LLC 2021-10-01
Series:APL Materials
Online Access:http://dx.doi.org/10.1063/5.0065839
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author Polychronis Tsipas
Panagiotis Pappas
Evgenia Symeonidou
Sotirios Fragkos
Christina Zacharaki
Evangelia Xenogiannopoulou
Nikitas Siannas
Athanasios Dimoulas
author_facet Polychronis Tsipas
Panagiotis Pappas
Evgenia Symeonidou
Sotirios Fragkos
Christina Zacharaki
Evangelia Xenogiannopoulou
Nikitas Siannas
Athanasios Dimoulas
author_sort Polychronis Tsipas
collection DOAJ
description One monolayer semimetallic HfTe2 thin films are grown on three substrates with different electronic properties in order to study the substrate effect on the electronic structure of the HfTe2 epilayer. Angle resolved photoelectron spectroscopy measurements indicate that the band features are identical in all three cases, providing evidence that the HfTe2 epilayer does not interact with any of the substrates to form hybridized bands and any band feature originates from the HfTe2 material itself. However, a shift of HfTe2 energy bands is observed among the three cases, which is attributed to substrate electron doping. This paves the way for accessing the Dirac point of HfTe2 Dirac semimetal, which is located about ∼0.2 to 0.3 eV above the Fermi level in the case of suspended HfTe2 in a non-destructive way.
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spelling doaj.art-e2e14b9374484c48b005528f37d07b9e2022-12-21T19:11:50ZengAIP Publishing LLCAPL Materials2166-532X2021-10-01910101103101103-610.1063/5.0065839Epitaxial HfTe2 Dirac semimetal in the 2D limitPolychronis Tsipas0Panagiotis Pappas1Evgenia Symeonidou2Sotirios Fragkos3Christina Zacharaki4Evangelia Xenogiannopoulou5Nikitas Siannas6Athanasios Dimoulas7Institute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceInstitute of Nanoscience and Nanotechnology, National Center for Scientific Research “Demokritos”, 15310 Athens, GreeceOne monolayer semimetallic HfTe2 thin films are grown on three substrates with different electronic properties in order to study the substrate effect on the electronic structure of the HfTe2 epilayer. Angle resolved photoelectron spectroscopy measurements indicate that the band features are identical in all three cases, providing evidence that the HfTe2 epilayer does not interact with any of the substrates to form hybridized bands and any band feature originates from the HfTe2 material itself. However, a shift of HfTe2 energy bands is observed among the three cases, which is attributed to substrate electron doping. This paves the way for accessing the Dirac point of HfTe2 Dirac semimetal, which is located about ∼0.2 to 0.3 eV above the Fermi level in the case of suspended HfTe2 in a non-destructive way.http://dx.doi.org/10.1063/5.0065839
spellingShingle Polychronis Tsipas
Panagiotis Pappas
Evgenia Symeonidou
Sotirios Fragkos
Christina Zacharaki
Evangelia Xenogiannopoulou
Nikitas Siannas
Athanasios Dimoulas
Epitaxial HfTe2 Dirac semimetal in the 2D limit
APL Materials
title Epitaxial HfTe2 Dirac semimetal in the 2D limit
title_full Epitaxial HfTe2 Dirac semimetal in the 2D limit
title_fullStr Epitaxial HfTe2 Dirac semimetal in the 2D limit
title_full_unstemmed Epitaxial HfTe2 Dirac semimetal in the 2D limit
title_short Epitaxial HfTe2 Dirac semimetal in the 2D limit
title_sort epitaxial hfte2 dirac semimetal in the 2d limit
url http://dx.doi.org/10.1063/5.0065839
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