Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries

Abstract Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composite...

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Main Authors: Zhengqing Ye, Ying Jiang, Li Li, Feng Wu, Renjie Chen
Format: Article
Language:English
Published: SpringerOpen 2021-10-01
Series:Nano-Micro Letters
Subjects:
Online Access:https://doi.org/10.1007/s40820-021-00726-z
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author Zhengqing Ye
Ying Jiang
Li Li
Feng Wu
Renjie Chen
author_facet Zhengqing Ye
Ying Jiang
Li Li
Feng Wu
Renjie Chen
author_sort Zhengqing Ye
collection DOAJ
description Abstract Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.
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spelling doaj.art-e35d4932baad40928e5cd4d650e307432022-12-21T20:45:58ZengSpringerOpenNano-Micro Letters2311-67062150-55512021-10-0113113710.1007/s40820-021-00726-zRational Design of MOF-Based Materials for Next-Generation Rechargeable BatteriesZhengqing Ye0Ying Jiang1Li Li2Feng Wu3Renjie Chen4Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of TechnologyAbstract Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.https://doi.org/10.1007/s40820-021-00726-zMetal–organic frameworksMOF compositesMOF derivativesMOF composite derivativesBatteries
spellingShingle Zhengqing Ye
Ying Jiang
Li Li
Feng Wu
Renjie Chen
Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
Nano-Micro Letters
Metal–organic frameworks
MOF composites
MOF derivatives
MOF composite derivatives
Batteries
title Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
title_full Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
title_fullStr Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
title_full_unstemmed Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
title_short Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries
title_sort rational design of mof based materials for next generation rechargeable batteries
topic Metal–organic frameworks
MOF composites
MOF derivatives
MOF composite derivatives
Batteries
url https://doi.org/10.1007/s40820-021-00726-z
work_keys_str_mv AT zhengqingye rationaldesignofmofbasedmaterialsfornextgenerationrechargeablebatteries
AT yingjiang rationaldesignofmofbasedmaterialsfornextgenerationrechargeablebatteries
AT lili rationaldesignofmofbasedmaterialsfornextgenerationrechargeablebatteries
AT fengwu rationaldesignofmofbasedmaterialsfornextgenerationrechargeablebatteries
AT renjiechen rationaldesignofmofbasedmaterialsfornextgenerationrechargeablebatteries