Two-Dimensional Electronic Spectroscopy of a Model Dimer System

Two-dimensional spectra of a dimer were measured to determine the timescale for electronic decoherence at room temperature. Anti-correlated beats in the crosspeaks were observed only during the period corresponding to the measured homogeneous lifetime.

Bibliographic Details
Main Authors: Prokhorenko V.I., Murphy R.S., Johnson P.J.M., Halpin A., Miller R.J.D.
Format: Article
Language:English
Published: EDP Sciences 2013-03-01
Series:EPJ Web of Conferences
Online Access:http://dx.doi.org/10.1051/epjconf/20134105032
Description
Summary:Two-dimensional spectra of a dimer were measured to determine the timescale for electronic decoherence at room temperature. Anti-correlated beats in the crosspeaks were observed only during the period corresponding to the measured homogeneous lifetime.
ISSN:2100-014X