Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures

Abstract Over the last decade, the possibility of realizing topological superconductivity (TSC) has generated much excitement. TSC can be created in electronic systems where the topological and superconducting orders coexist, motivating the continued exploration of candidate material platforms to th...

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Main Authors: Hemian Yi, Lun-Hui Hu, Yi-Fan Zhao, Ling-Jie Zhou, Zi-Jie Yan, Ruoxi Zhang, Wei Yuan, Zihao Wang, Ke Wang, Danielle Reifsnyder Hickey, Anthony R. Richardella, John Singleton, Laurel E. Winter, Xianxin Wu, Moses H. W. Chan, Nitin Samarth, Chao-Xing Liu, Cui-Zu Chang
Format: Article
Language:English
Published: Nature Portfolio 2023-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-42902-2
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author Hemian Yi
Lun-Hui Hu
Yi-Fan Zhao
Ling-Jie Zhou
Zi-Jie Yan
Ruoxi Zhang
Wei Yuan
Zihao Wang
Ke Wang
Danielle Reifsnyder Hickey
Anthony R. Richardella
John Singleton
Laurel E. Winter
Xianxin Wu
Moses H. W. Chan
Nitin Samarth
Chao-Xing Liu
Cui-Zu Chang
author_facet Hemian Yi
Lun-Hui Hu
Yi-Fan Zhao
Ling-Jie Zhou
Zi-Jie Yan
Ruoxi Zhang
Wei Yuan
Zihao Wang
Ke Wang
Danielle Reifsnyder Hickey
Anthony R. Richardella
John Singleton
Laurel E. Winter
Xianxin Wu
Moses H. W. Chan
Nitin Samarth
Chao-Xing Liu
Cui-Zu Chang
author_sort Hemian Yi
collection DOAJ
description Abstract Over the last decade, the possibility of realizing topological superconductivity (TSC) has generated much excitement. TSC can be created in electronic systems where the topological and superconducting orders coexist, motivating the continued exploration of candidate material platforms to this end. Here, we use molecular beam epitaxy (MBE) to synthesize heterostructures that host emergent interfacial superconductivity when a non-superconducting antiferromagnet (FeTe) is interfaced with a topological insulator (TI) (Bi, Sb)2Te3. By performing in-vacuo angle-resolved photoemission spectroscopy (ARPES) and ex-situ electrical transport measurements, we find that the superconducting transition temperature and the upper critical magnetic field are suppressed when the chemical potential approaches the Dirac point. We provide evidence to show that the observed interfacial superconductivity and its chemical potential dependence is the result of the competition between the Ruderman-Kittel-Kasuya-Yosida-type ferromagnetic coupling mediated by Dirac surface states and antiferromagnetic exchange couplings that generate the bicollinear antiferromagnetic order in the FeTe layer.
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spelling doaj.art-e46cfcc9403f494d974702d31c5a04582023-11-12T12:23:57ZengNature PortfolioNature Communications2041-17232023-11-011411910.1038/s41467-023-42902-2Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructuresHemian Yi0Lun-Hui Hu1Yi-Fan Zhao2Ling-Jie Zhou3Zi-Jie Yan4Ruoxi Zhang5Wei Yuan6Zihao Wang7Ke Wang8Danielle Reifsnyder Hickey9Anthony R. Richardella10John Singleton11Laurel E. Winter12Xianxin Wu13Moses H. W. Chan14Nitin Samarth15Chao-Xing Liu16Cui-Zu Chang17Department of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityMaterials Research Institute, The Pennsylvania State UniversityMaterials Research Institute, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityNational High Magnetic Field LaboratoryNational High Magnetic Field LaboratoryCAS Key Laboratory of Theoretical Physics, Institute of Theoretical Physics, Chinese Academy of SciencesDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityDepartment of Physics, The Pennsylvania State UniversityAbstract Over the last decade, the possibility of realizing topological superconductivity (TSC) has generated much excitement. TSC can be created in electronic systems where the topological and superconducting orders coexist, motivating the continued exploration of candidate material platforms to this end. Here, we use molecular beam epitaxy (MBE) to synthesize heterostructures that host emergent interfacial superconductivity when a non-superconducting antiferromagnet (FeTe) is interfaced with a topological insulator (TI) (Bi, Sb)2Te3. By performing in-vacuo angle-resolved photoemission spectroscopy (ARPES) and ex-situ electrical transport measurements, we find that the superconducting transition temperature and the upper critical magnetic field are suppressed when the chemical potential approaches the Dirac point. We provide evidence to show that the observed interfacial superconductivity and its chemical potential dependence is the result of the competition between the Ruderman-Kittel-Kasuya-Yosida-type ferromagnetic coupling mediated by Dirac surface states and antiferromagnetic exchange couplings that generate the bicollinear antiferromagnetic order in the FeTe layer.https://doi.org/10.1038/s41467-023-42902-2
spellingShingle Hemian Yi
Lun-Hui Hu
Yi-Fan Zhao
Ling-Jie Zhou
Zi-Jie Yan
Ruoxi Zhang
Wei Yuan
Zihao Wang
Ke Wang
Danielle Reifsnyder Hickey
Anthony R. Richardella
John Singleton
Laurel E. Winter
Xianxin Wu
Moses H. W. Chan
Nitin Samarth
Chao-Xing Liu
Cui-Zu Chang
Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
Nature Communications
title Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
title_full Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
title_fullStr Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
title_full_unstemmed Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
title_short Dirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
title_sort dirac fermion assisted interfacial superconductivity in epitaxial topological insulator iron chalcogenide heterostructures
url https://doi.org/10.1038/s41467-023-42902-2
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