Critical behavior and magnetocaloric effect in VI_{3}

Layered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI_{3} single crystals. The critical exponents β=0.244(5) with a c...

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Main Authors: Yu Liu (刘育), Milinda Abeykoon, C. Petrovic
Format: Article
Language:English
Published: American Physical Society 2020-01-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.013013
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author Yu Liu (刘育)
Milinda Abeykoon
C. Petrovic
author_facet Yu Liu (刘育)
Milinda Abeykoon
C. Petrovic
author_sort Yu Liu (刘育)
collection DOAJ
description Layered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI_{3} single crystals. The critical exponents β=0.244(5) with a critical temperature T_{c}=50.10(2)K and γ=1.028(12) with T_{c}=49.97(5)K are obtained from the modified Arrott plot, whereas δ=5.24(2) is obtained from a critical isotherm analysis at T_{c}=50K. The magnetic entropy change −ΔS_{M}(T,H) features a maximum at T_{c}, i.e., −ΔS_{M}^{max}∼2.64(2.27)Jkg^{−1}K^{−1} with out-of-plane (in-plane) field change of 5 T. This is consistent with −ΔS_{M}^{max}∼2.80Jkg^{−1}K^{−1} deduced from heat capacity and the corresponding adiabatic temperature change ΔT_{ad}∼0.96K with out-of-plane field change of 5 T. The critical analysis suggests that the ferromagnetic phase transition in VI_{3} is situated close to a three- to two-dimensional critical point. The rescaled ΔS_{M}(T,H) curves collapse onto a universal curve, confirming a second-order type of the magnetic transition and reliability of the obtained critical exponents.
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spelling doaj.art-e485ef3c6586414daf6cb348ed53f1432024-04-12T16:48:19ZengAmerican Physical SocietyPhysical Review Research2643-15642020-01-012101301310.1103/PhysRevResearch.2.013013Critical behavior and magnetocaloric effect in VI_{3}Yu Liu (刘育)Milinda AbeykoonC. PetrovicLayered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI_{3} single crystals. The critical exponents β=0.244(5) with a critical temperature T_{c}=50.10(2)K and γ=1.028(12) with T_{c}=49.97(5)K are obtained from the modified Arrott plot, whereas δ=5.24(2) is obtained from a critical isotherm analysis at T_{c}=50K. The magnetic entropy change −ΔS_{M}(T,H) features a maximum at T_{c}, i.e., −ΔS_{M}^{max}∼2.64(2.27)Jkg^{−1}K^{−1} with out-of-plane (in-plane) field change of 5 T. This is consistent with −ΔS_{M}^{max}∼2.80Jkg^{−1}K^{−1} deduced from heat capacity and the corresponding adiabatic temperature change ΔT_{ad}∼0.96K with out-of-plane field change of 5 T. The critical analysis suggests that the ferromagnetic phase transition in VI_{3} is situated close to a three- to two-dimensional critical point. The rescaled ΔS_{M}(T,H) curves collapse onto a universal curve, confirming a second-order type of the magnetic transition and reliability of the obtained critical exponents.http://doi.org/10.1103/PhysRevResearch.2.013013
spellingShingle Yu Liu (刘育)
Milinda Abeykoon
C. Petrovic
Critical behavior and magnetocaloric effect in VI_{3}
Physical Review Research
title Critical behavior and magnetocaloric effect in VI_{3}
title_full Critical behavior and magnetocaloric effect in VI_{3}
title_fullStr Critical behavior and magnetocaloric effect in VI_{3}
title_full_unstemmed Critical behavior and magnetocaloric effect in VI_{3}
title_short Critical behavior and magnetocaloric effect in VI_{3}
title_sort critical behavior and magnetocaloric effect in vi 3
url http://doi.org/10.1103/PhysRevResearch.2.013013
work_keys_str_mv AT yuliuliúyù criticalbehaviorandmagnetocaloriceffectinvi3
AT milindaabeykoon criticalbehaviorandmagnetocaloriceffectinvi3
AT cpetrovic criticalbehaviorandmagnetocaloriceffectinvi3