Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter
Depositions of trace elements of air particulates in the atmosphere have gained much attention in recent times due to their environmental, climatic and health impacts. In the current study, trace elements of size-segregated rural and urban particulate matter (PM2.5 and PM2.5−10) were characterized u...
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| Format: | Article |
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Frontiers Media S.A.
2023-01-01
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| Series: | Frontiers in Environmental Science |
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| Online Access: | https://www.frontiersin.org/articles/10.3389/fenvs.2022.1082783/full |
| _version_ | 1797956556243861504 |
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| author | Abdallah M. A. Dawood Eric Akortia Sultan J. Alsufyani Gustav Gbeddy |
| author_facet | Abdallah M. A. Dawood Eric Akortia Sultan J. Alsufyani Gustav Gbeddy |
| author_sort | Abdallah M. A. Dawood |
| collection | DOAJ |
| description | Depositions of trace elements of air particulates in the atmosphere have gained much attention in recent times due to their environmental, climatic and health impacts. In the current study, trace elements of size-segregated rural and urban particulate matter (PM2.5 and PM2.5−10) were characterized using particle-induced X-ray emission method. Effects of dry deposition flux and Saharan dust intrusion on the elemental concentrations were determined. The mean elemental concentration in the rural fine PM ranged between 0.0002 ± 0.0002 μg m−3 (for Se) and 0.6658 ± 0.5816 μg m−3 (for S) whereas in the urban fine PM the concentration ranged between 0.0007 ± 0.0008 μg m−3 (for As) and 0.5869 ± 0.3429 μg m−3 (for Ca). In the coarse PM fraction, concentration ranged between 0.0001 ± 0.0001 μg m−3 (for Se) and 0.5886 ± 0.5343 μg m−3 (for Ca) at the rural site; and between 0.0002 ± 0.0002 μg m−3 (for Se) and 1.9201 ± 1.911 μg m−3 (for Ca) at the urban site. Mainly crustal elements (Al, Ca, Fe) and ‘pollution’ source element (S) recorded high and significant dry deposition fluxes across the two sites in both PM modes. Deposition flux was relatively higher in the coarse than in the fine PM mode. The average dry deposition flux estimated for fine and coarse PM at the rural and urban sites were 33.68 ± 57.19 μg m−2 day−1 and 47.71 ± 92.19 μg m−2 day−1; 36.66 ± 61.95 μg m−2 day−1 and 107.02 ± 237.71 μg m−2 day−1, respectively. Mainly crustal (Al, Ca, Fe) and “pollution” (S) element recorded high and significant dry deposition fluxes across the two sites and in the two PM modes. The impacts of dust on climate, air quality, and the environment in general have increased the need to better understand the dust flow system. In the current study, dust intruding the study area from the Sahara was analyzed using the NMMB/BSC dust model. The model’s output indicated that, the highest daily surface dust concentration was observed in the central and south-west of Turkey which corresponded with the peak period of Saharan dust transport to the Eastern Mediterranean in the month of March. |
| first_indexed | 2024-04-10T23:51:50Z |
| format | Article |
| id | doaj.art-e5842eeec362414fa17f4e848b660284 |
| institution | Directory Open Access Journal |
| issn | 2296-665X |
| language | English |
| last_indexed | 2024-04-10T23:51:50Z |
| publishDate | 2023-01-01 |
| publisher | Frontiers Media S.A. |
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| series | Frontiers in Environmental Science |
| spelling | doaj.art-e5842eeec362414fa17f4e848b6602842023-01-10T18:34:02ZengFrontiers Media S.A.Frontiers in Environmental Science2296-665X2023-01-011010.3389/fenvs.2022.10827831082783Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matterAbdallah M. A. Dawood0Eric Akortia1Sultan J. Alsufyani2Gustav Gbeddy3Radiation Protection Institute, Ghana Atomic Energy Commission, Accra, GhanaRadiation Protection Institute, Ghana Atomic Energy Commission, Accra, GhanaDepartment of Physics, College of Science, Taif University, Taif, Saudi ArabiaRadiation Protection Institute, Ghana Atomic Energy Commission, Accra, GhanaDepositions of trace elements of air particulates in the atmosphere have gained much attention in recent times due to their environmental, climatic and health impacts. In the current study, trace elements of size-segregated rural and urban particulate matter (PM2.5 and PM2.5−10) were characterized using particle-induced X-ray emission method. Effects of dry deposition flux and Saharan dust intrusion on the elemental concentrations were determined. The mean elemental concentration in the rural fine PM ranged between 0.0002 ± 0.0002 μg m−3 (for Se) and 0.6658 ± 0.5816 μg m−3 (for S) whereas in the urban fine PM the concentration ranged between 0.0007 ± 0.0008 μg m−3 (for As) and 0.5869 ± 0.3429 μg m−3 (for Ca). In the coarse PM fraction, concentration ranged between 0.0001 ± 0.0001 μg m−3 (for Se) and 0.5886 ± 0.5343 μg m−3 (for Ca) at the rural site; and between 0.0002 ± 0.0002 μg m−3 (for Se) and 1.9201 ± 1.911 μg m−3 (for Ca) at the urban site. Mainly crustal elements (Al, Ca, Fe) and ‘pollution’ source element (S) recorded high and significant dry deposition fluxes across the two sites in both PM modes. Deposition flux was relatively higher in the coarse than in the fine PM mode. The average dry deposition flux estimated for fine and coarse PM at the rural and urban sites were 33.68 ± 57.19 μg m−2 day−1 and 47.71 ± 92.19 μg m−2 day−1; 36.66 ± 61.95 μg m−2 day−1 and 107.02 ± 237.71 μg m−2 day−1, respectively. Mainly crustal (Al, Ca, Fe) and “pollution” (S) element recorded high and significant dry deposition fluxes across the two sites and in the two PM modes. The impacts of dust on climate, air quality, and the environment in general have increased the need to better understand the dust flow system. In the current study, dust intruding the study area from the Sahara was analyzed using the NMMB/BSC dust model. The model’s output indicated that, the highest daily surface dust concentration was observed in the central and south-west of Turkey which corresponded with the peak period of Saharan dust transport to the Eastern Mediterranean in the month of March.https://www.frontiersin.org/articles/10.3389/fenvs.2022.1082783/fullair particulate matterair pollutiondust intrusiontrace elementsdeposition flux |
| spellingShingle | Abdallah M. A. Dawood Eric Akortia Sultan J. Alsufyani Gustav Gbeddy Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter Frontiers in Environmental Science air particulate matter air pollution dust intrusion trace elements deposition flux |
| title | Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| title_full | Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| title_fullStr | Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| title_full_unstemmed | Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| title_short | Impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| title_sort | impact of dry deposition flux and dust intrusion phenomena on elemental concentrations of air particulate matter |
| topic | air particulate matter air pollution dust intrusion trace elements deposition flux |
| url | https://www.frontiersin.org/articles/10.3389/fenvs.2022.1082783/full |
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